Hostname: page-component-7b7567c8c-wxvwp Total loading time: 0 Render date: 2026-11-15T02:33:55.592Z Has data issue: false hasContentIssue false
  • English
  • Français

Field-Free Molecular Orientation Induced by a Single-Cycle THz Laser Pulse Train

Published online by Cambridge University Press:  31 August 2016

Xiao-Miao Zhang,
Jian Li,
Jie Yu and
Shu-Lin Cong
Xiao-Miao Zhang*
Affiliation:
School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024, China
Jian Li*
Affiliation:
School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024, China
Jie Yu*
Affiliation:
School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024, China
Shu-Lin Cong*
Affiliation:
School of Physics and Optoelectronic Technology, Dalian University of Technology, Dalian 116024, China
*
*Corresponding author. Email addresses:xiaomiaozhang@mail.dlut.edu.cn (X.-M. Zhang), dlut_lijian@mail.dlut.edu.cn (J. Li), yujie@dlut.edu.cn (J. Yu), shlcong@dlut.edu.cn (S.-L. Cong)
*Corresponding author. Email addresses:xiaomiaozhang@mail.dlut.edu.cn (X.-M. Zhang), dlut_lijian@mail.dlut.edu.cn (J. Li), yujie@dlut.edu.cn (J. Yu), shlcong@dlut.edu.cn (S.-L. Cong)
*Corresponding author. Email addresses:xiaomiaozhang@mail.dlut.edu.cn (X.-M. Zhang), dlut_lijian@mail.dlut.edu.cn (J. Li), yujie@dlut.edu.cn (J. Yu), shlcong@dlut.edu.cn (S.-L. Cong)
*Corresponding author. Email addresses:xiaomiaozhang@mail.dlut.edu.cn (X.-M. Zhang), dlut_lijian@mail.dlut.edu.cn (J. Li), yujie@dlut.edu.cn (J. Yu), shlcong@dlut.edu.cn (S.-L. Cong)

Abstract

Core share and HTML view are not available for this content. However, as you have access to this content, a full PDF is available via the 'Save PDF' action button.

We investigate theoretically the field-free orientation of CO molecules induced by a single-cycle THz laser pulse train. It is shown that the molecular orientation can be obviously enhanced by applying the pulse train. The laser intensity and pulse number have some effects on the molecular orientation. The high degree of field-free molecular orientation |⟨cosθ⟩|max=0.9246 is obtained at temperature T=0 K. The variations of the maximum orientation degree with the experimentally available pulse number and peak intensity are given. Temperature T has a considerable influence on the field-free molecular orientation. The maximal field-free molecular orientation at T=0, 10, 20 and 30 K for N=14 and E 0=1.8 MV/cm are |⟨cosθ⟩|max=0.9188, 0.7338, 0.6055 and 0.5154 in order, and the corresponding effective duration times of molecular orientation are Δt=0.759, 0.432, 0.297 and 0.117 ps.

Keywords

Single-cycle THz laser pulse trainpulse numbermolecular orientation

Information

Type
Research Article
Information
Communications in Computational Physics , Volume 20 , Issue 3 , September 2016, pp. 689 - 702
Copyright
Copyright © Global-Science Press 2016 

References

[1] Stapelfeldt, H. and Seideman, T., Colloquium: Aligning molecules with strong laser pulses, Rev. Mod. Phys., 75(2003) 543.CrossRefGoogle Scholar
[2] Stapelfeldt, H. and Hamilton, E., Nonadiabatic alignment by intense pulses. Concepts, theory, and directions, Adv. At. Mol. Opt. Phys., 52 (2005) 289–329.Google Scholar
[3] Kanai, T., Minemoto, S. and Sakai, H., Quantum interference during high-order harmonic generation from aligned molecules, Nature, 435(2005) 470–474.CrossRefGoogle ScholarPubMed
[4] Kanai, T., Minemoto, S. and Sakai, H., Ellipticity dependence of high-order harmonic generation from aligned molecules, Phys. Rev. Lett., 98(2007) 053002.Google ScholarPubMed
[5] Bian, X.-B. and Bandrauk, A. D., Orientation dependence of nonadiabatic molecular high-order-harmonic generation from resonant polar molecules, Phys. Rev. A, 86(2012) 053417.CrossRefGoogle Scholar
[6] Jin, Y., Tong, X. and Toshima, N., Anomalous alignment dependence of the third-order harmonic of H2 + ions in intense laser fields, Phys. Rev. A, 86(2012) 053418.CrossRefGoogle Scholar
[7] Bisgaard, C. Z., Clarkin, O. J., Wu, G., Lee, A. M. D., Geßner, O., Hayden, C. C. and Stolow, A., Time-Resolved Molecular Frame Dynamics of Fixed-in-Space CS2 Molecules, Science, 323(2009) 1464–1468.CrossRefGoogle ScholarPubMed
[8] Li, F., Hao, X.-Y. and Li, X.-G., Efficient Grid Treatment of the Time Dependent Schrödinger Equation for Laser-Driven Molecular Dynamics, Commun. Comput. Phys., 13(2013) 1389–1407.CrossRefGoogle Scholar
[9] Li, J.-L., Huang, Y., Xie, T., Chai, S. and Cong, S.-L., Formation of NaH Molecules in the Lowest Rovibrational Level of the Ground Electronic State via Short-Range Photoassociation, Commun. Comput. Phys., 17(2015) 79–92.CrossRefGoogle Scholar
[10] Hu, J., Han, K.-L. and He, G.-Z., Correlation Quantum Dynamics between an Electron and D2+ Molecule with Attosecond Resolution. Phys. Rev. Lett., 95(2005) 123001.CrossRefGoogle ScholarPubMed
[11] Yuan, K.-J., Sun, Z.-G., Cong, S.-L. and Lou, N.-Q., Selective excitation of the OClO molecule with femtosecond laser pulse. Phys. Rev. A, 72(2005) 052513.CrossRefGoogle Scholar
[12] Litvinyuk, I. V., Lee, K. F., Dooley, P. W., Rayner, D. M., Villeneuve, D. M. and Corkum, P. B., Alignment-dependent strong field ionization of molecules, Phys. Rev. Lett., 90(2003) 233003.CrossRefGoogle ScholarPubMed
[13] Lein, M., Molecular imaging using recolliding electrons, J. Phys. B, 40(2007) R135-R173.CrossRefGoogle Scholar
[14] Meckel, M., Comtois, D., Zeidler, D., Staudte, A., Pavičić, D., Bandulet, H. C., Pépin, H., Kieffer, J. C., Dörner, R., Villeneuve, D. M., Corkum, P. B., Laser-Induced Electron Tunneling and Diffraction, Science 320(2008) 1478–1482.CrossRefGoogle ScholarPubMed
[15] Küpper, J. et al, X-Ray Diffraction from Isolated and Strongly Aligned Gas-Phase Molecules with a Free-Electron Laser, Phys. Rev. Lett., 112(2014) 083002.CrossRefGoogle Scholar
[16] Lan, P.-F., Lu, P.-X., Cao, W., Li, Y.-H. and Wang, X.-L., Carrier-envelope phase-stabilized attosecond pulses from asymmetric molecules, Phys. Rev. A, 76(2007) 021801(R).CrossRefGoogle Scholar
[17] Chen, J., Cui, X., Zhou, S., Huang, B. and Jiang, X., Numerical simulations of femtosecond-laser-induced dynamic alignment of molecules in the high-frequency off-resonance regime, Laser Phys., 12(2006) 1672–1680.CrossRefGoogle Scholar
[18] Zeng, G.-P., Zhong, F.-J., Wu, C.-Y., Jiang, H.-B. and Gong, Q.-H., Field-free molecular alignment and its application, Laser Phys., 19(2009) 1691.CrossRefGoogle Scholar
[19] Molodenskiy, M. S. and Tikhonova, O. V., Rotational dynamics of a molecular ensemble in the presence of a strong laser field, Laser Phys., 17(2007) 401.CrossRefGoogle Scholar
[20] Wu, J., Cai, H., Peng, Y., Tong, Y.-Q., Couairon, A. and Zeng, H.-P., Control of femtosecond filamentation by field-free revivals of molecular alignment, Laser Phys., 19(2009) 1759–1768.CrossRefGoogle Scholar
[21] Rosca-Pruna, F. and Vrakking, M. J. J., Experimental Observation of Revival Structures in Picosecond Laser-Induced Alignment of I2 , Phys. Rev. Lett., 87(2001) 153902.CrossRefGoogle ScholarPubMed
[22] Hain, T. D., Moision, R.M. and Curtiss, T. J., Hexapole state-selection and orientation of asymmetric top molecules: CH2F2 , J. Chem. Phys., 111(1999) 6797.CrossRefGoogle Scholar
[23] Friedrich, B. and Herschbach, D. R., On the possibility of orienting rotationally cooled polar-molecules in an electric-field, Z. Phys. D, 18(1991) 153.CrossRefGoogle Scholar
[24] Friedrich, B. and Herschbach, D., Enhanced orientation of polar molecules by combined electrostatic and nonresonant induced dipole forces, J. Chem. Phys., 111(1999) 6157.CrossRefGoogle Scholar
[25] Friedrich, B. and Herschbach, D., Manipulating Molecules via Combined Static and Laser Fields, J. Phys. Chem. A, 103(1999) 10280.CrossRefGoogle Scholar
[26] Kitano, K., Ishii, N. and Itatani, J., High degree of molecular orientation by a combination of THz and femtosecond laser pulses, Phys. Rev. A, 84(2011) 053408.CrossRefGoogle Scholar
[27] Machholm, M. and Henriksen, N. E., Field-Free Orientation of Molecules, Phys. Rev. Lett., 87(2001) 193001.CrossRefGoogle ScholarPubMed
[28] Daems, D., Guérin, S., Sugny, D. and Jauslin, H. R., Efficient and Long-Lived Field-Free Orientation of Molecules by a Single Hybrid Short Pulse, Phys. Rev. lett., 94(2005) 153003.CrossRefGoogle ScholarPubMed
[29] Gershnabel, E., Averbukh, I. S. and Gordon, R. J., Enhanced molecular orientation induced by molecular antialignment, Phys. Rev. A, 74(2006) 053414.CrossRefGoogle Scholar
[30] Shu, C.-C., Yuan, K.-J., Hu, W.-H. and Cong, S.-L., Field-free molecular orientation with terahertz few-cycle pulses, J. Chem. Phys. 132(2010) 244311.CrossRefGoogle ScholarPubMed
[31] Qin, C.-C., Tang, Y., Wang, Y.-M. and Zhang, B., Field-free orientation of CO by a terahertz few-cycle pulse, Phys. Rev. A, 85(2012) 053415.CrossRefGoogle Scholar
[32] Kanai, T. and Sakai, H., Numerical simulations of molecular orientation using strong, non-resonant, two-color laser fields, J. Chem. Phys., 115(2001) 5492.CrossRefGoogle Scholar
[33] De, S. et al, Field-Free Orientation of CO Molecules by Femtosecond Two-Color Laser Fields, Phys. Rev. Lett., 103(2009) 153002.CrossRefGoogle ScholarPubMed
[34] Wu, J. and Zeng, H., Field-free molecular orientation control by two ultrashort dual-color laser pulses, Phys. Rev. A, 81(2010) 053401.CrossRefGoogle Scholar
[35] Muramatsu, M., Hita, M., Minemoto, S. and Sakai, H., Field-free molecular orientation by an intense nonresonant two-color laser field with a slow turn on and rapid turn off, Phys. Rev. A, 79(2009) 011403(R).CrossRefGoogle Scholar
[36] Liu, Y., Li, J., Yu, J. and Cong, S.-L., Field-free molecular orientation by two-color shaped laser pulse together with time-delayed THz laser pulse, Laser. Phys. Lett., 10(2013) 076001.CrossRefGoogle Scholar
[37] Zhang, S., Shi, J., Zhang, H., Jia, T., Wang, Z. and Sun, Z., Field-free molecular orientation by a multicolor laser field, Phys. Rev. A, 83(2011) 023416.Google Scholar
[38] Sheng, Z.-M., Wu, H.-C., Wang, W.-M., Chen, M., Dong, X.-G., Zheng, J. and Zhang, J., Simulation of High Power THz Emission from Laser Interaction with Tenuous Plasma and Gas Targets† , Commun. Comput. Phys., 4(2008) 1258–1278.Google Scholar
[39] Fleischer, S., Zhou, Y., Field, R.W. and Nelson, K. A., Molecular Orientation and Alignment by Intense Single-Cycle THz Pulses, Phys. Rev. Lett., 107(2011) 163603.CrossRefGoogle ScholarPubMed
[40] Shu, C.-C. and Henriksen, N. E., Field-free molecular orientation induced by single-cycle THz pulses: The role of resonance and quantum interference, Phys. Rev. A, 87(2013) 013408.CrossRefGoogle Scholar
[41] Huang, Y., Xie, T., Li, J., Yu, J. and Cong, S.-L., Efficiently field-free orientation of CO molecules by a femtosecond pulse and a THz pulse train, Laser Phys. 24(2014) 016002.CrossRefGoogle Scholar
[42] Ramakrishna, S. and Seideman, T., Intense Laser Alignment in Dissipative Media as a Route to Solvent Dynamics, Phys. Rev. Lett., 95(2005) 113001.CrossRefGoogle Scholar
[43] Ramakrishna, S. and Seideman, T., Disspative dynamics of laser induced nonadiabatic molecualr alignment, J. Chem. Phys., 124(2006) 034101.CrossRefGoogle Scholar