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Buoyant miscible displacement flows in rectangular channels

Published online by Cambridge University Press:  10 August 2017

S. M. Taghavi*
Affiliation:
Department of Chemical Engineering, Université Laval, Québec, QC G1V 0A6, Canada
R. Mollaabbasi
Affiliation:
Department of Chemical Engineering, Université Laval, Québec, QC G1V 0A6, Canada
Y. St-Hilaire
Affiliation:
Department of Chemical Engineering, Université Laval, Québec, QC G1V 0A6, Canada
*
†Email address for correspondence: Seyed-Mohammad.Taghavi@gch.ulaval.ca

Abstract

Buoyant displacement flows of two miscible fluids in rectangular channels are studied, theoretically and experimentally. The scenario considered involves the displacement of a fluid by a slightly heavier one at nearly horizontal channel inclinations, where inertial effects are weak and laminar stratified flows may be expected. In the theoretical part, a lubrication approximation model is developed to simplify the displacement flow governing equations and furnish a semi-analytical solution for the heavy and light fluid flux functions. Three key dimensionless parameters govern the fluid flow motion, i.e. a buoyancy number, the viscosity ratio and the channel cross-section aspect ratio. When these parameters are specified, the reduced model can deliver the interface propagation in time, leading and trailing front heights, shapes and speeds, cross-sectional velocity fields, etc. In addition, the model can be exploited to provide various classifications such as single or multiple fronts as well as main displacement flow regimes at long times such as no sustained backflows, stationary interface flows and sustained backflows. Focusing on the variation of the buoyancy number, a large number of iso-viscous displacement experiments are performed in a square duct and the results are compared with those of the lubrication model. Qualitative displacement flow features observed in the theory and experiments are in good agreement, in particular, in terms of the main displacement flow regimes. The quantitative comparisons are also reasonable for small and moderate imposed displacement flow velocities. However, at large flow rates, a deviation of the experimental results from the model results is observed, which may be due to the presence of non-negligible inertial effects.

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Papers
Copyright
© 2017 Cambridge University Press 
Figure 0

Figure 1.Schematic of the displacement flow geometry considered.

Figure 1

Figure 2.Variation of $q_{H}$ versus $\unicode[STIX]{x1D6EC}$ for $h_{X}=0$ (note that $h_{X}=\unicode[STIX]{x2202}h/\unicode[STIX]{x2202}X$) and $\unicode[STIX]{x1D712}=50$, from the full model (circles), in comparison with the limiting cases: $q_{H}^{\unicode[STIX]{x1D6EC}\ll 1}$ (lines) and $q_{H}^{\unicode[STIX]{x1D6EC}\gg 1}$ (dashed lines). From (a–c) $m=0.1$, $m=1$ and $m=10$. In each graph, $h=0.2$, $h=0.4$ and $h=0.6$ from bottom to top.

Figure 2

Figure 3.Examples of contours of $q_{H}/\unicode[STIX]{x1D6EC}$, versus $h$ and $\unicode[STIX]{x1D6EC}$, for $\unicode[STIX]{x1D712}=30$ and $h_{X}=0$. From (a–c) $m=0.1$, $m=1$ and $m=10$.

Figure 3

Figure 4.Local flow reversal within the light fluid. Steady state velocity contours $u(y,z)$ versus $y$ and $2z/\unicode[STIX]{x1D6EC}$, plotted within the light fluid within half of the duct for $h=0.7$, $h_{X}=0$, $m=1$, $\unicode[STIX]{x1D712}=50$ and $\unicode[STIX]{x1D6EC}=1,~2,~4$ from (a–c). In each panel, the thick black line shows the zero contour line, where the light fluid velocity is zero. Below the thick line, the light fluid moves forward and above the thick line it moves backward against the mean imposed flow direction.

Figure 4

Figure 5.Examples of displacements for $\unicode[STIX]{x1D6EC}=m=1$ at $T=0,1,\ldots ,9,10$, with $\unicode[STIX]{x1D712}=0,100,200$ from (a) to (c). The dashed lines illustrate the front height predictions obtained from equation (4.3) for long times. The insets show the superimposition of the interface heights at long times when plotted versus $X/T$.

Figure 5

Figure 6.Heights and speeds of the $\text{leading}\backslash \text{trailing}$ fronts at long times for $\unicode[STIX]{x1D712}=0\backslash 50$ (solid line), $\unicode[STIX]{x1D712}=20\backslash 100$ (dashed line), $\unicode[STIX]{x1D712}=40\backslash 150$ (dash–dot line) and $\unicode[STIX]{x1D712}=60\backslash 200$ (dots); in each column, $m$ is fixed ($m=0.1,1,10$ from left to right). For the case of $\unicode[STIX]{x1D712}=20$, ${V_{f}^{\infty }|}_{\unicode[STIX]{x1D6EC}\gg 1}$ and ${h_{f}^{\infty }|}_{\unicode[STIX]{x1D6EC}\gg 1}$ are superposed as horizontal lines (also marked by arrows).

Figure 6

Figure 7.Parameter regime in the $(m-\unicode[STIX]{x1D712})$-plane where multiple fronts with finite heights are marked by shaded areas. Elsewhere there is only a single leading front with a finite height and a trailing front that is pinned to the upper wall. The cross-section aspect ratio increases from (a–c) $\unicode[STIX]{x1D6EC}=1,2,10$. The middle shaded area is where there exist forward-moving multiple fronts. The upper shaded area contains multiple fronts, among which at least one is a backward-moving trailing front.

Figure 7

Figure 8.(a) Front length scale, $\unicode[STIX]{x1D701}_{L}$, versus the viscosity ratio, $m$, for $\unicode[STIX]{x1D6EC}=10$ (▫), $\unicode[STIX]{x1D6EC}=1$ ($\circ$) and $\unicode[STIX]{x1D6EC}=0.1$ (▵). (b–d) Examples of the leading front shapes in the moving frame of reference at $\unicode[STIX]{x1D712}=0$ for $\unicode[STIX]{x1D6EC}=0.5$ (solid line), $\unicode[STIX]{x1D6EC}=1$ (dashed line) and $\unicode[STIX]{x1D6EC}=2$ (dash–dot line). The value of the viscosity ratio is changed in each panel: $m=0.1,1,10$ from left to right.

Figure 8

Figure 9.Numerical solution of the short-time behaviours for $\unicode[STIX]{x1D6EC}=1$, $\unicode[STIX]{x1D712}=0$ and $m=1$. (a) Interface evolution versus time for a very sharp initial slope of the interface ($h_{X}=-10^{3}$) for very short times, i.e. $T=[0,1,\ldots ,9,10]\times 5\times 10^{-5}$. (b) Variation of the trailing front velocity versus time. (c) Variation of the leading front velocity versus time. The dashed lines in panels (b) and (c) show respectively the long-time leading and trailing velocities, predicted by the method explained in § 4.2.

Figure 9

Figure 10.Variation of critical values versus $\unicode[STIX]{x1D6EC}$, for the stationary flow state, for $m=0.1$ (solid line), $m=1$ (dashed line) and $m=10$ (dash–dot line).

Figure 10

Table 1.Comparison of the critical values for the stationary interface condition, for two-layer displacements in typical flow geometries. The values of the critical buoyancy number ($\unicode[STIX]{x1D712}_{c}$) and the stationary layer thickness ($h_{c}$) are given for iso-viscous displacement flows ($m=1$) in near-horizontal inclinations. The values marked by ‘$\ast$’ are taken from Taghavi et al. (2011). In the definition of $\unicode[STIX]{x1D712}$ for different geometries, the pipe diameter or channel height has been used as the characteristic length scale.

Figure 11

Figure 11.Panel (a) shows a schematic view of our experimental apparatus. Panels (b–f) show the results for experiment $VI$. (b) Image sequence showing the evolution of a typical displacement. From top to bottom are shown images for $\hat{t}=1.8,3.6,\ldots ,16.2,18$ s. The field of view is $2450\times 12.5~\text{mm}^{2}$. (c) The extracted experimental interface evolution, for the same times as in panel (b). The inset shows the collapse of $h$ when plotted versus $x/t$. Horizontal dashed lines mark the front height at long times. (d) Variation of the leading front velocity with time. Dashed line shows $\hat{V}_{f}^{\infty }=93~\text{mm}~\text{s}^{-1}$. (e) Velocity contour results $(\text{mm}~\text{s}^{-1})$ at the UDV probe positions in line with the $\hat{z}$-axis fixed at $(\hat{x},{\hat{y}})\approx (894,16)$ (mm). From top to bottom the velocity contours correspond to $\hat{z}\approx -4,~0,+4$ (mm). (f) Velocity contour results ($\text{mm}~\text{s}^{-1}$) at the UDV probe positions in line with the ${\hat{y}}$-axis fixed at $(\hat{x},\hat{z})\approx (894,8)$ (mm). From top to bottom the velocity contours correspond to ${\hat{y}}\approx 4,~8,~12$ mm. Velocity contours are averaged in time over several consecutive velocity profiles.

Figure 12

Table 2.Dimensional and dimensionless experimental parameters ($\unicode[STIX]{x1D712}$ varies in the range 0–7082). The two fluids are (nearly) iso-viscous with $\hat{\unicode[STIX]{x1D708}}\approx 1~\text{mm}^{2}~\text{s}^{-1}$ as the common kinematic viscosity; therefore, $m\approx 1$. All the experiments are performed in a nearly square duct, with the cross-section area of $15.65\times 15.85$ mm$^{2}$; therefore, $\unicode[STIX]{x1D6EC}\approx 1.013$ is fixed in our experiments. Certain experiments labelled by Roman numerals will be referenced in the following figures.

Figure 13

Figure 12.Experimental datapoints marking viscous flows (●) and inertial flows (▫). Examples of spatio-temporal diagrams obtained for experiments $V$ and $VII$ are plotted as lower and upper insets, respectively. Dashed line marks the transition boundary using equation (5.1) for $h_{s}=0.6$.

Figure 14

Figure 13.Comparison between the leading front velocities obtained from the model and experiments. Datapoints correspond to experiments performed at $At=10^{-3}$ with $\unicode[STIX]{x1D6FD}=90^{\circ }$ (▪), $\unicode[STIX]{x1D6FD}=88^{\circ }$ (▴), $\unicode[STIX]{x1D6FD}=85^{\circ }$ (●) and $\unicode[STIX]{x1D6FD}=88^{\circ }$ ($\star$); $At=5\times 10^{-3}$ with $\unicode[STIX]{x1D6FD}=90^{\circ }$ ($\times$), $\unicode[STIX]{x1D6FD}=88^{\circ }$ ($+$), $\unicode[STIX]{x1D6FD}=85^{\circ }$ ($\ast$) and $\unicode[STIX]{x1D6FD}=82^{\circ }$ (); and $At=10^{-2}$ with $\unicode[STIX]{x1D6FD}=90^{\circ }$ (▾), $\unicode[STIX]{x1D6FD}=88^{\circ }$ (◂), $\unicode[STIX]{x1D6FD}=85^{\circ }$ (▸) and $\unicode[STIX]{x1D6FD}=82^{\circ }$ (♦). The dashed line indicates $Fr\times V_{f,model}^{\infty }=Fr\times V_{f,exp}^{\infty }$. The arrow marks $Fr\times V_{f,\exp }^{\infty }\approx 3.4$, which on average corresponds to $Fr\approx 2$.

Figure 15

Figure 14.Comparison between $h_{f}^{\infty }$ obtained from the model and experiments.

Figure 16

Figure 15.(a,c,e,g) Image sequences for various trailing front behaviours, where the red arrows mark the approximate position of the trailing front. The field of view is $2250\times 12.5$ mm$^{2}$. (b,d,f,h) Plots of the variation of the trailing front velocity versus time for the same flow parameters as in (a,c,e,g). (a) Sustained backflow in experiment $III$ for $\hat{t}=18$, $36,\ldots ,162$, $180$ s. (c) Stationary interface flow in experiment $IV$ for $\hat{t}=84$, $168,\ldots ,756$, $840$ s. (e) No sustained backflow (here a temporary backflow) in experiment $II$ for $\hat{t}=9.9$, $19.8,\ldots ,89.1$, $99$ s. (g) No sustained backflow (here an instantaneous displacement) in experiment $I$ for $\hat{t}=5.9$, $11.8,\ldots ,53.1$, $59$ s. Dashed lines represent $\hat{V}_{b}^{\infty }$ predicted by the model.

Figure 17

Figure 16.Comparison between $h_{b}^{\infty }$ and $V_{b}^{\infty }$ from the model and experiments, in the sustained-backflow regime.

Figure 18

Figure 17.Comparison between the lubrication predictions and the experimental results for the stationary interface flow condition. (a) Lines show the results in experiment $IV$ for $\hat{t}=$ 84, 168, 252, 336, 420, 504, 588, 672, 756, 840 s. Dashed line shows the lubrication model for $\unicode[STIX]{x1D712}_{c}=100.67$, $\unicode[STIX]{x1D6EC}=1.013$ and $m=1$. (b) Experimental results showing no sustained backflows (including instantaneous displacements ($+$), temporary backflows ($\ast$)), stationary interface flows (●) and sustained backflows ($\times$). The thick solid line shows $\unicode[STIX]{x1D712}_{c}=2Re\cos \unicode[STIX]{x1D6FD}/Fr^{2}=100.67$, which is the critical value obtained from the model for $\unicode[STIX]{x1D6EC}=1.013$ and $m=1$. Inertial flows are marked by the superposed rectangles. The horizontal dashed line (also highlighted by the arrow) marks $Re\cos \unicode[STIX]{x1D6FD}/Fr=50$.