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Using Space-Time Correlations to Identify Transient Defects

Published online by Cambridge University Press:  19 February 2018

William Lowe  and
Jacob Eapen
William Lowe*
Affiliation:
Department of Nuclear Engineering, North Carolina State University, Raleigh, North Carolina 27695, U.S.A
Jacob Eapen
Affiliation:
Department of Nuclear Engineering, North Carolina State University, Raleigh, North Carolina 27695, U.S.A
*
*(Email: wclowe@ncsu.edu)
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Abstract

Atomistic simulations are employed to investigate the dynamical behavior of atoms in cubic silicon carbide (SiC) following a 5 keV radiation knock. Specifically, we have computed the time-resolved van Hove self-correlation function, Gs(r,t), separately for the silicon and carbon sub-lattices. Our goal is to probe the early radiation damage mechanisms using a dynamical methodology. The simulation results show that the carbon atoms engage in a dynamic hopping mechanism as the system recovers from the radiation knock. The silicon atoms, however, exhibit a strikingly different behaviour: the time variation of 4πr2Gs(r,t) indicates a dynamic tension between the crystalline and disordered regions of the Si sub-lattice. The power-law tail of the 4πr2Gs(r,t) correlation for silicon atoms suggests a scale-free self-organized critical (SOC) state – a possible precursor to the collapse of the Si sub-lattice.

Keywords

ceramicnuclear materialsradiation effects

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Type
Articles
Information
MRS Advances , Volume 3 , Issue 31: Energy and Sustainability , 2018 , pp. 1755 - 1760
Copyright
Copyright © Materials Research Society 2018 

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