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A macrotransport equation for the Hele-Shaw flow of a concentrated suspension

Published online by Cambridge University Press:  09 August 2021

Sourojeet Chakraborty
Affiliation:
Chemical Engineering and Applied Chemistry, University of Toronto, Toronto, ON M5S 3E5, Canada
Arun Ramachandran*
Affiliation:
Chemical Engineering and Applied Chemistry, University of Toronto, Toronto, ON M5S 3E5, Canada
*
†Email address for correspondence: engrarun@gmail.com

Abstract

A depth-averaged, convection-dispersion equation is derived for the particle volume fraction distribution in the pressure-driven flow of a concentrated suspension of neutrally buoyant, non-colloidal particles between two parallel plates, by implementing a two-time-scale perturbation expansion of the suspension balance model (Nott & Brady, J. Fluid Mech., vol. 275, 1994, pp. 157–199) coupled with the constitutive equations of Zarraga et al. (J. Rheol., vol. 52, issue 2, 2000, pp. 185–220). The Taylor-dispersion coefficient in the macrotransport equation scales as $U_c^{\prime}B^{\prime 3}/a^{\prime 2}$, where $U_c^{\prime}$ is the characteristic depth-averaged velocity, $B^{\prime}$ is the half-depth of the channel and $a^{\prime}$ is the particle radius. Taylor dispersion relaxes gradients in the depth-averaged volume fraction along the local velocity vector. Perpendicular to the flow, however, only shear-induced migration can cause particle redistribution, leading to fluxes down gradients in volume fraction, shear rate and streamline curvature that scale as $U_c^{\prime}a^{\prime 2}/B^{\prime}$. To determine the velocity and particle distributions in Hele-Shaw suspension flows, one only needs to solve two coupled partial differential equations in the pressure and the depth-averaged volume fraction, achievable on commercially available solvers. Analogous to the macrotransport equation for suspension flow through a circular tube (Ramachandran, J. Fluid Mech., vol. 734, 2013, pp. 219–252), the evolution of the particle volume fraction distribution is dependent only on the total strain experienced by the suspension, and is independent of the suspension velocity scale. However, unlike the tube problem, a positive concentration gradient along the flow direction is susceptible to viscous miscible fingering. A linear stability analysis performed for a step increase in the volume fraction in the direction of flow with a velocity $U^{\prime}$ reveals that the growth rate and wavenumber corresponding to fastest growing mode scale as $U^{\prime}a^{\prime 2}/B^{\prime 3}$ and $a^{\prime 2/3}/B^{\prime 5/3}$, respectively.

Information

Type
JFM Papers
Copyright
© The Author(s), 2021. Published by Cambridge University Press
Figure 0

Figure 1. Schematic of the flow geometry.

Figure 1

Figure 2. Predictions of the zeroth-order profiles of (a) volume fraction ($\phi ^{(0)}$, (3.16)), (b) the function quantifying the in-plane velocity ($F$, (3.17)) and (c) the velocity along the thin direction ($\hat {Q}_1=Q_1//M$, (3.26)), as functions of the co-ordinate in the thin direction, $x_3$. The solid, dotted and dash–dotted curves are the results for depth-averaged volume fractions of 20 %, 30 % and 45 %. The inset in subfigure (a) provides a zoomed-in view of the volume fraction profiles near the centreline.

Figure 2

Figure 3. Predictions of the first-order profiles of (a) volume fraction ($Q_7$, (3.33)) and (b) the function quantifying the in-plane velocity, ($Q_{10}/M$, (3.35)), as functions of the co-ordinate in the thin direction, $x_3$. The solid, dotted and dash–dotted curves are the results for depth-averaged volume fractions of 20 %, 30 % and 45 %.

Figure 3

Figure 4. The functions appearing in the macrotransport equation: (a) the suspension mobility, $M (\bar {\phi })$ (3.20); (b) the flow-averaged volume fraction, $g (\bar {\phi })$ (3.49) (the dotted line is the parity line, equal to $\bar {\phi }$); (c) the reduced Taylor dispersivity, $h (\bar {\phi })$ (3.45); (d) the relative contributions of the volume fraction and velocity perturbations, $h_1 (\bar {\phi })$ (3.35) and $h_2 (\bar {\phi })$ (3.33), respectively, to the reduced Taylor dispersivity (note that $h=Q_{11}-Q_{12}$ (3.45)); (e) the prefactor of SIM$_1$, $q_A (\bar {\phi })$ (3.47); and (f) the prefactor of SIM$_2$, $q_B (\bar {\phi })$ (3.47).

Figure 4

Figure 5. The volume fraction dependence of the ratio of the shear-induced migration flux to the Taylor dispersion flux along the flow direction.

Figure 5

Figure 6. Simulation of the displacement of a 30 % suspension by a 50 % suspension in a Hele-Shaw expansion geometry using the macrotransport equations, (4.1) to (4.5), solved on COMSOL®. Subfigure (a) shows the details of the expansion geometry. A pressure difference of $\Delta P^{\prime }$ is applied between the left and right edges of the geometry. The length, time and velocity scales used to render the equations dimensionless are $B^{\prime 3}/a^{\prime 2}$, $B^{\prime 4}\mu _0^{\prime }/a^{\prime 4}\Delta P^{\prime }$ and $a^{\prime 2}\Delta P^{\prime }/(B^{\prime }\mu _0^{\prime })$. Subfigure (b) shows the initial volume fraction distribution, which contains a shock in the flow direction at $x_1=-5$. Subfigures (c–f) show the evolution of the volume fraction distribution predicted by the macrotransport equation, (4.1), at times $t=250,750,1500$ and 3000, respectively, for two cases: with Taylor dispersion in (4.1) turned off (top), and with Taylor dispersion turned on (bottom). It can be seen that with the inclusion of Taylor dispersion, the shock relaxes significantly more in the axial direction. The aspect ratio $B^{\prime }/a^{\prime }$ for the simulations was 20.

Figure 6

Figure 7. Simulation of the displacement of a 30 % suspension by a 50 % suspension in a radial Hele-Shaw geometry with inner and outer radii of $1$ and $10$ units, respectively. The macrotransport equations, (4.1) to (4.5), were solved in the simulations on COMSOL®. A radial pressure difference of $\Delta P^{\prime }$ is applied to drive the suspension flow outwards from the centre. The length, time and velocity scales used to render the equations dimensionless are $B^{\prime 3}/a^{\prime 2}$, $B^{\prime 4}\mu _0^{\prime }/a^{\prime 4}\Delta P^{\prime }$ and $a^{\prime 2}\Delta P^{\prime }/(B^{\prime }\mu _0^{\prime })$. The initial volume fraction distribution, $\phi |_{t=0}=0.4+0.1\tanh \left [10(r-2)\right ]$, shows a shock at a radial position, $r$, of $2$ units (see subfigure a). Subfigures (b,d) show the evolution of volume fraction distribution for $t=400$ and $t=1600$, respectively, when Taylor dispersion is turned off, while subfigures (c,e) show the results for the case when Taylor dispersion is included for the time stamps $t = 400$ and $t=1600$, respectively. As in figure 6, the relaxation of the shock in the radial direction is stronger when Taylor dispersion is included in the simulations. The aspect ratio $B^{\prime }/a^{\prime }$ for the simulations was 20.

Figure 7

Figure 8. Two canonical volume fraction profiles: (a) a step decrease and (b) a step increase in the depth-averaged volume fraction in the flow direction. Here $\bar {\phi }_-$ and $\bar {\phi }_+$ are the volume fractions upstream and downstream of the shock.

Figure 8

Table 1. The scaling relationships for the maximum growth rate $(\sigma _{m}^{\prime })$ and the wavenumbers corresponding to the maximum growth rate $(k_{m}^{\prime })$ and cut-off $(k_{c}^{\prime })$ for the miscible viscous fingering problem, in the limit, $D_\perp ^{\prime }/D_\parallel ^{\prime }\ll 1$.

Figure 9

Figure 9. Definition sketch for the linear stability analysis of the viscous miscible fingering problem for the Hele-Shaw flow of suspensions. The initial configuration comprises a suspension at a low volume fraction $\bar {\phi }_-$$(x_1<0)$ interfacing a suspension at a high volume fraction $\bar {\phi }_+$, $x_1>0$, in the form of a flat plane at $x_1=0$. The combination is displaced from left to right. Sinusoidal perturbations of the volume fraction, pressure and velocity fields are imposed at about the base configuration in the $x_2$ direction.

Figure 10

Figure 10. The dispersion relationship arising from a linear stability analysis of the macrotransport equation for a step increase in volume fraction in the flow direction from $\bar {\phi }_-=0.4$ to $\bar {\phi }_+=0.5$ (see figure 8b). The solid, dotted and dash–dotted curves are results for $B/a =$ 10, 40 and 100, respectively. The inset shows the same dispersion curves in the limit of small wavenumbers.

Figure 11

Figure 11. The maximum growth rate $\sigma _m^{\prime }$ (subfigure a), the wavenumber, $k_m^{\prime }$, corresponding to the maximum growth rate (subfigure b) and the cut-off wavenumber (subfigure c) as functions of the aspect ratio $B^{\prime }/a^{\prime }$ for $\bar {\phi }_-=0.4$ and $\bar {\phi }_+=0.5$.

Figure 12

Figure 12. The effect of volume fraction on the stability curve, $\sigma '$ vs $k'$. For the solid curve, $\bar {\phi }_-=0.4$ and $\bar {\phi }_+=0.5$, while for the dash–dotted curve, $\bar {\phi }_-=0.3$ and $\bar {\phi }_+=0.4$. For both curves, $B^{\prime }/a^{\prime }=40$. Larger volume fractions lead to higher growth rates and a larger range of wavenumbers for which perturbations are unstable.

Figure 13

Figure 13. The effect of the excess of the flow-averaged concentration $g$ over the area-averaged concentration $\bar {\phi }$ on the relationship between $\sigma '$ and $k'$; (a) $\bar {\phi }_-=0.4$ and $\bar {\phi }_+=0.5$, (b) $\bar {\phi }_-=0.3$ and $\bar {\phi }_+=0.4$. For both subfigures, $B^{\prime }/a^{\prime }=40$. In each subfigure, the dash–dotted line is the result of a simulation where $g$ was manually set to be equal to $\bar {\phi }$.

Figure 14

Figure 14. A picture explaining why the case of $U_s^{\prime }< U^{\prime }$ would lead to lower growth rates compared with the case of $U_s^{\prime }=U^{\prime }$. A low volume fraction suspension displaces a high volume fraction suspension from left to right.

Figure 15

Table 2. Symbols/variables used and their description.