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Thermotactic navigation of an artificial microswimmer near a plane wall

Published online by Cambridge University Press:  03 February 2023

Antarip Poddar*
Affiliation:
Department of Mechanical Engineering, Indian Institute of Technology (Indian School of Mines) Dhanbad, Jharkhand 826004, India
*
†Email address for correspondence: antarip@iitism.ac.in

Abstract

Despite significant advances in the field of man-made micro- and nanomotors, it remains a challenge to precisely control their motion in bounded environments. Here, we present a theoretical analysis of a thermally activated micromotor near a plane wall under the action of a background linear temperature field. The coupling between the autonomous and field-directed motions has been resolved using a combined analytical–numerical framework comprising general solutions in bispherical coordinates and the reciprocal theorem for creeping flows. Results reveal giant augmentation in swimming speeds, the controlling parameter zones for positive and negative thermotaxes and the flexibility of steering perpendicular to the field gradient for an isolated micromotor. Boundary-instigated thermo-fluidic modulations at different levels of confinements and preferential orientations cause directional switching of both the vertical translation and rotation parallel to the wall, thereby drastically altering the phase portraits of the swimmer dynamics. Contrasting trajectory characteristics, e.g. escape, attraction, are partitioned by unstable separatrices in the phase portraits, while competitive repulsion (attraction) after attraction (repulsion) characteristics emerge for different relative field strengths $\mathcal {S}$ and gradient orientations $\theta _T$. Below $\mathcal {S}=0.25$, highly counter-intuitive trajectories result when the micromotor is initially launched from an overlapping escape zone. Moreover, external-field-assisted microswimming can uniquely tune the directionality of wall-parallel translation, broadening the scope of dynamic regulation of self-propulsion. Thus, providing insights into a precisely controlled fuel-free actuation of micromotors near a physical obstacle, the present study stands as a step toward addressing the increasing demand for successful implementation of micromotors in futuristic clinical and environmental applications.

Information

Type
JFM Papers
Copyright
© The Author(s), 2023. Published by Cambridge University Press
Figure 0

Figure 1.Schematic of a thermally activated half-coated Janus particle near a conducting plane wall. The surrounding fluid medium is externally heated using a linearly varying temperature field $\tilde {T}_\infty$ along the direction $\boldsymbol {e}_T$. The green (cold) to orange (hot) coloured background denotes the variation of the external temperature field. Similarly, the orange and green colours on the particle denote the hot metallic cap and the cold uncoated halves of the particle surface, respectively. The symmetry axis of the Janus particle is oriented along $\boldsymbol {d}$. The plane conducting wall at $z=0$ has been marked with grey.

Figure 1

Figure 2.Velocity of the micromotor in the unbounded domain. (a) Regime diagram for positive and negative thermotaxes based on $V_{\parallel }$ in the $\mathcal {S}$–$\theta _T$ plane. Variations of (b) translational velocity magnitude $(|\boldsymbol {V}|)$, and (c) orientation of the velocity vector $({\rm \Delta} \theta _v)$ with the orientation angle of the background temperature field $(\theta _T)$ for different values of the strength number $(\mathcal {S})$. In (b), the dashed lines are ‘ext’ cases, and the marker lines are combined situations for the indicated $\mathcal {S}$.

Figure 2

Figure 3.Temperature distribution in and around the micromotor under externally applied temperature gradient. The colours denote a normalized temperature $\hat {\mathcal {T}} = \mathcal {T}/(\mathcal {T}_{max} - \mathcal {T}_{min})$, with the south-east end temperature set to zero for the imposed temperature field $( \mathcal {T}_{ref}(x=0,z=0) = 0 )$. The orientation of the external temperature gradient $(\theta _T)$ is varied as $0^{\circ },\ 315^{\circ },\ 270^{\circ }$ from top to bottom, while the dimensionless strength of the temperature gradient $( \mathcal {S})$ is varied as $0.01, 0.05, 0.1$ from left to right. The other parameters are $\theta _d=60^{\circ }$, and $\delta = 1$.

Figure 3

Figure 4.Temperature variation with the angular distance $\theta$ (shown as an inset) along the surface of the micromotor, starting from the top surface point where the $z$-axis intersects the swimmer periphery in the $x$–$z$ plane. Different values of the strength number $(\mathcal {S})$, orientation of the applied temperature gradient $(\theta _T)$ and distance of micromotor surface from the wall $(\delta )$ have been chosen. Other parameters and temperature reference remain the same as in figure 3.

Figure 4

Figure 5.(a) Surface temperature variation with the angle $\theta$ for different values of the strength number $(\mathcal {S})$. The orientation of the applied temperature gradient is $\theta _T=45^{\circ }$. Panels (b) and (c) show the direction of surface flow $(u_s)$ for self-propulsion and combined propulsion ($\mathcal {S}=0.1$, $\theta _T=45^{\circ }$), respectively. The coloured background encodes the variation of normalized temperature field $(\mathcal {T})$. The maximum and minimum temperature points in each case have been marked with yellow and light blue bubbles, respectively. In all three panels, distance from wall is kept constant at $\delta = 1$. (d) Surface temperature distribution for different $\delta$, $\mathcal {S}=0.1$ and $\theta _T=45^{\circ }$. In all the panels, $\theta _d=60^{\circ }$ has been taken. The reference (zero) temperature is set at the south-west corner.

Figure 5

Figure 6.(a) Variation of the vertical velocity component of the micromotor $(V_z)$ with the wall distance $(\delta )$ for $(\theta _d,\theta _T) = (60^{\circ },45^{\circ })$. (b) Surface plot of the critical wall distance $\delta _{cr}$ for $V_z=0$ in the $\mathcal {S}$–$\theta _T$ plane. Panel (c) shows plots similar to (a), but with a different parameter set $(\theta _d,\theta _T) = (150^{\circ },120^{\circ })$.

Figure 6

Figure 7.(a) Variation of the rotational velocity of the micromotor $(\varOmega _y)$ with the wall distance $(\delta )$ for $(\theta _d,\theta _T) = (60^{\circ },45^{\circ })$. (b) Surface plot showing signs of $\varOmega _y$ for distances $0.01 \le \delta \le 10$ in the $\mathcal {S}$–$\theta _T$ plane for $\theta _d= 60^{\circ }$.

Figure 7

Figure 8.Phase portrait for (a) self-propulsion only, (b) combined action of self- and passive propulsion with $\mathcal {S}=0.1, \theta _T=0^{\circ }$. (c) Sample trajectories with initial condition $z_0=4,\theta _{d,0}=80^{\circ }$. Other parameters in parts (i) and (ii) are similar to panels (a) and (b), respectively. (d) Minimum initial distance from the wall required to attain an escape state $\delta _{0,min}$ vs imposed field orientation $\theta _T$ for $\mathcal {S}=0.1$. It also shows the variation of the range of micromotor orientations ${\rm \Delta} \theta _d$ in the phase portrait (marked in panel (a)) for which only attraction states are possible.

Figure 8

Figure 9.(a) Phase portrait for combined propulsion with $\mathcal {S}=0.5, \theta _T=75^{\circ }$. (b) Sample trajectories with similar parameters and different initial conditions: (i) $z_0=3.2,\theta _{d,0}=54^{\circ }$ and (ii) $z_0=5.3,\theta _{d,0}=295^{\circ }$. The corresponding phase space trajectories have been shown with black lines in (a), where the initial locations are marked with red bubbles.

Figure 9

Figure 10.Phase portrait for combined propulsion with (a) $\mathcal {S}=0.5, \theta _T=120^{\circ }$. (b) A sample trajectory with similar parameters and initial conditions: $z_0=2.28,\theta _{d,0}=155^{\circ }$. The corresponding phase space trajectory has been shown with a black line in (a), where the initial location is marked with a red bubble.

Figure 10

Figure 11.Regime maps showing the observed swimming states for different combinations of the parameters $\mathcal {S}$ and $\theta _T$.

Figure 11

Figure 12.Surface plot for $V_x$ in the $\theta _d$–$h$ plane for (a) self-propulsion only and combined propulsion with (b) $\mathcal {S}=0.2, \theta _T=55^{\circ }$ and (c) $\mathcal {S}=0.5,\ \theta _T=55^{\circ }$. (d) Regime map showing the motion direction of the micromotor for different combinations of $\mathcal {S}$ and $\theta _T$.

Figure 12

Figure 13.Variation of velocity components of an inert particle under thermophoresis with the reciprocal of the centre distance from the wall $1/h$ for different relative thermal conductivities of the particle $\mathcal {K}$. Panels show (a) $V_{ext,x}/V_0$, (b) $\varOmega _{ext,y} /V_0$ and (c) $V_{ext,z}/V_0$, where $V_0$ denotes the dimensionless free-space thermophoretic velocity. Reported results of Keh & Chen (2003) and Chen (1999) have been shown with markers.