1 Introduction
Fluid–particle suspensions are commonly encountered in nature (dust storms, snow avalanches, debris flows, slurries, etc.) and find important applications in many chemical process industries. While the effects of interstitial fluid on the dynamics of particles in dry granular flows can be neglected, the particle motion is affected by the viscous drag and other fluid forces in gas–solid or liquid–solid suspensions (Batchelor Reference Batchelor1970; Hinch Reference Hinch1977; Brady & Bossis Reference Brady and Bossis1988; Jackson Reference Jackson2000; Guazzelli & Morris Reference Guazzelli and Morris2011). The particle inertia can be quantified in terms of Stokes number defined as
where
$\dot{\unicode[STIX]{x1D6FE}}$
is the local shear rate and
$\unicode[STIX]{x1D70F}_{vis}$
is the viscous relaxation time of a single particle of mass
$m$
and diameter
$\unicode[STIX]{x1D70E}$
suspended in a gas of viscosity
$\unicode[STIX]{x1D707}_{g}$
and density
$\unicode[STIX]{x1D70C}_{g}$
. The estimate (1.1) of
$\unicode[STIX]{x1D70F}_{vis}$
follows from the assumption that the particle Reynolds number
$Re_{p}=\unicode[STIX]{x1D70C}_{g}\dot{\unicode[STIX]{x1D6FE}}\unicode[STIX]{x1D70E}^{2}/\unicode[STIX]{x1D707}_{g}\ll 1$
, a measure of the fluid inertia, is very small so that it experiences Stokes’ linear drag force. The connection of the dry rapid granular flow with inertial gas–solid suspension can be established via the Stokes number:
The dense-gas kinetic theory (Chapman & Cowling Reference Chapman and Cowling1970) has been extended to derive constitutive relations for rapid granular flows (Goldreich & Tremaine Reference Goldreich and Tremaine1978; Savage & Jeffrey Reference Savage and Jeffrey1981; Jenkins & Richman Reference Jenkins and Richman1985; Sela & Goldhirsch Reference Sela and Goldhirsch1998; Brey, Dufty & Santos Reference Brey, Dufty and Santos1999) as well as for gas–solid suspensions (Koch Reference Koch1990; Tsao & Koch Reference Tsao and Koch1995; Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996; Koch & Sangani Reference Koch and Sangani1999; Lun & Savage Reference Lun, Savage, Pöschel and Brilliantov2003; Garzo et al.
Reference Garzo, Tenneti, Subramaniam and Hrenya2012; Parmentier & Simonin Reference Parmentier and Simonin2012; Saha & Alam Reference Saha and Alam2017). The Grad-moment theory of Tsao & Koch (Reference Tsao and Koch1995), based on the well-known Grad’s moment expansion (Grad Reference Grad1949), can quantitatively predict the shear viscosity of a ‘dilute’ suspension of inelastic particles with restitution coefficient
$e\geqslant 0.8$
and Stokes number
$St=10$
(see figure 12c of Saha & Alam (Reference Saha and Alam2017)). However, the agreement between the theory of Tsao & Koch (Reference Tsao and Koch1995) and the simulation data for the particle-phase viscosity worsens significantly for (i) inelastic particles with
$e<0.8$
and (ii) smaller values of the Stokes number
$St<10$
. Regarding the non-Newtonian transport coefficients, the first normal-stress difference is well predicted by Tsao & Koch (Reference Tsao and Koch1995) at
$e\geqslant 0.5$
; however, their theory (with added nonlinear corrections as in Saha & Alam (Reference Saha and Alam2017)) underpredicts the second normal-stress difference by a factor of
$3$
or more over the whole range of restitution coefficient (see figure 12b of Saha & Alam (Reference Saha and Alam2017)). These discrepancies have been addressed in the recent anisotropic-moment theory of Saha & Alam (Reference Saha and Alam2017), who found excellent agreement of all transport coefficients with the simulation data for a ‘dilute’ gas–solid suspension over wide ranges of
$St$
and
$e$
.
Moving to ‘moderately dense’ suspensions, the analyses of transport coefficients predicted by the existing constitutive models (Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996; Garzo et al.
Reference Garzo, Tenneti, Subramaniam and Hrenya2012; Parmentier & Simonin Reference Parmentier and Simonin2012) confirmed that they hold only at Stokes numbers of
$St>O(10)$
even for elastically colliding particles (
$e=1$
). Moreover, the quantitative predictions of transport coefficients by the above models deteriorate markedly for inelastic (
$e\neq 1$
) particles in the rapid granular (
$St\rightarrow \infty$
) regime (Saha & Alam Reference Saha and Alam2016). Clearly, there is a need to develop a theory for non-dilute gas–solid suspensions of inelastic particles that can provide quantitative predictions of rheology over wide ranges of Stokes numbers and restitution coefficients since the current rheological models fair poorly (i) at
$St\leqslant O(10)$
for elastically colliding particles (
$e=1$
) as well as for (ii) highly inelastic particles (
$e\ll 1$
) at any
$St$
.
The following text, quoted from the concluding part of a review article (Koch & Hill Reference Koch and Hill2001), aptly summarizes the current status of theoretical models for inertial gas–solid suspensions: ‘Kinetic theories have been used to derive the averaged equations of motion of inertial gas–solid suspensions with
$Re_{p}\ll 1$
and
$St\geqslant O(1)$
.
$\ldots$
[F]urther analytical studies of the first effects of inertia for
$Re_{p}\ll 1$
and
$St\ll 1$
would help to develop the overall picture of inertial suspension behaviour.’ Focusing on low-Reynolds-number suspensions (
$Re_{p}\ll 1$
), our primary aim in this paper is to outline a theory for gas–solid suspensions that (i) bridges the two limits of Stokes numbers (
$1\ll St\rightarrow \infty$
), and (ii) encompasses both dilute and dense regimes (
$0<\unicode[STIX]{x1D708}<\unicode[STIX]{x1D708}_{f}\approx 0.5$
), and is such that (iii) the resulting constitutive relations for shear viscosity and two normal-stress differences should hold for highly inelastic particles (i.e.
$e\ll 1$
). The latter requirement calls for a non-Newtonian constitutive model going beyond the standard Navier–Stokes (NS) order models as pursued in our recent work (Saha & Alam Reference Saha and Alam2017) that dealt with a dilute gas–solid suspension.
Focusing on moderately dense gas–solid suspensions, we employ the Boltzmann–Enskog equation (§ 2) with a velocity-dependent acceleration term to account for the effective drag force on the particles offered by laminar gas flow – the underlying assumptions about hydrodynamic interactions are discussed in § 2. In § 3, the anisotropic Maxwellian is used as the single-particle distribution function to analyse the rheology of the dilute to dense suspension undergoing homogeneous shear flow. In addition, the Boltzmann–Enskog equation under homogeneous shearing condition is solved using the direct-simulation Monte Carlo (DSMC) method (§ 4.1), yielding information on the shear viscosity and two normal-stress differences and the anisotropies of the second-moment tensor. In §§ 4.1 and 4.2, the superiority of the present theory is demonstrated via comparisons of predicted transport coefficients with the simulation data for inelastic particles over a range of Stokes numbers. The limitations of the theory are discussed in § 5 with reference to (i) the possible impact of many-body hydrodynamic interactions (§ 5.1), (ii) the scaling of the stress in the zero-Stokes-number limit (§ 5.2), and (iii) the inertial effects (
$Re_{p}>0$
) on the predicted transport coefficients (§ 5.3).
2 Beyond Navier–Stokes hydrodynamics for a dense suspension
We consider the steady homogeneous shear flow of smooth inelastic spheres, each of mass
$m$
, material density
$\unicode[STIX]{x1D70C}_{p}$
and diameter
$\unicode[STIX]{x1D70E}$
, suspended in a Newtonian gas of density
$\unicode[STIX]{x1D70C}_{g}$
and viscosity
$\unicode[STIX]{x1D707}_{g}$
. In the absence of gravity and assuming the smallness of the particle Reynolds number,
$Re_{p}=\unicode[STIX]{x1D70C}_{g}\dot{\unicode[STIX]{x1D6FE}}\unicode[STIX]{x1D70E}^{2}/\unicode[STIX]{x1D707}_{g}\ll 1$
, the gas-phase velocity
$\boldsymbol{v}(\boldsymbol{x},t)$
can be determined from the Stokes equations of motion,
$\unicode[STIX]{x1D707}_{g}\unicode[STIX]{x1D6FB}^{2}\boldsymbol{v}=\unicode[STIX]{x1D735}p_{g}$
and
$\unicode[STIX]{x1D735}\boldsymbol{\cdot }\boldsymbol{v}=0$
, where
$p_{g}(\boldsymbol{x},t)$
refers to the gas pressure. For the particle phase, the single-particle distribution function
$f(\boldsymbol{c},\boldsymbol{x},t)$
satisfies the well-known Boltzmann–Enskog equation
where the effects of the gas phase on the particle dynamics is taken into account via the acceleration term,
$\text{d}\boldsymbol{c}/\text{d}t$
, on the left-hand side of (2.1) and
$\unicode[STIX]{x1D735}_{\boldsymbol{c}}$
is the divergence operator in the velocity space. It is assumed that the collision operator
$(\unicode[STIX]{x2202}f/\unicode[STIX]{x2202}t)_{coll}$
on the right-hand side of (2.1), which incorporates dense (excluded-volume) effects via the two-body interactions, remains unaffected by the gas phase. The latter assumption implies the validity of the standard collision rule for smooth spheres: the normal component of the relative velocity of a colliding pair of particles changes according to
$(\boldsymbol{g}^{\prime }\boldsymbol{\cdot }\boldsymbol{k})=-e(\boldsymbol{g}\boldsymbol{\cdot }\boldsymbol{k})$
, where
$\boldsymbol{g}=\boldsymbol{c}_{1}-\boldsymbol{c}_{2}$
and
$\boldsymbol{g}^{\prime }=\boldsymbol{c}_{1}^{\prime }-\boldsymbol{c}_{2}^{\prime }$
are the pre- and post-collisional relative velocities, respectively,
$\boldsymbol{k}\equiv \boldsymbol{k}_{12}=(\boldsymbol{x}_{2}-\boldsymbol{x}_{1})/|\boldsymbol{x}_{2}-\boldsymbol{x}_{1}|$
is the unit contact vector joining the centre of sphere 1 to that of sphere 2, and
$0\leqslant e\leqslant 1$
is the coefficient of restitution, which accounts for the dissipative nature of particle collisions.
The macroscopic or hydrodynamic fields for the particle phase are defined via
$n\langle \unicode[STIX]{x1D713}\rangle \equiv \int \unicode[STIX]{x1D713}f(\boldsymbol{c},\boldsymbol{x},t)\,\text{d}\boldsymbol{c}$
, which, for
$\unicode[STIX]{x1D713}=m$
, yields the mass density
$\unicode[STIX]{x1D70C}(\boldsymbol{x},t)\equiv mn(\boldsymbol{x},t)$
, with
$n(\boldsymbol{x},t)$
denoting the number density of particles. Similarly, the macroscopic velocity vector is
$\boldsymbol{u}(\boldsymbol{x},t)=\langle \boldsymbol{c}\rangle$
, and a rank-2 anisotropic tensor,
representing the second moment of the fluctuation velocity, is treated as a separate hydrodynamic field, where
$\boldsymbol{C}=\boldsymbol{c}-\boldsymbol{u}$
is the peculiar velocity of particles; the granular temperature is
$T=\langle C^{2}/3\rangle =M_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FC}}/3$
, and
$\widehat{\unicode[STIX]{x1D648}}$
is the deviator (i.e. the trace-less part) of
$\unicode[STIX]{x1D648}$
. For the homogeneous shear flow, the macroscopic velocity of the particle phase is related to the imposed shear rate (
$\dot{\unicode[STIX]{x1D6FE}}$
) via
$\boldsymbol{u}=\dot{\unicode[STIX]{x1D6FE}}y\,\boldsymbol{e}_{x}$
, with uniform velocity gradient tensor,
$$\begin{eqnarray}\displaystyle \unicode[STIX]{x1D735}\boldsymbol{u}=\left[\frac{\unicode[STIX]{x2202}\mathit{u}_{\unicode[STIX]{x1D6FC}}}{\unicode[STIX]{x2202}x_{\unicode[STIX]{x1D6FD}}}\right]=\unicode[STIX]{x1D63F}+\unicode[STIX]{x1D652}=\left[\begin{array}{@{}ccc@{}}0 & \dot{\unicode[STIX]{x1D6FE}}/2 & 0\\ \dot{\unicode[STIX]{x1D6FE}}/2 & 0 & 0\\ 0 & 0 & 0\end{array}\right]+\left[\begin{array}{@{}ccc@{}}0 & \dot{\unicode[STIX]{x1D6FE}}/2 & 0\\ -\dot{\unicode[STIX]{x1D6FE}}/2 & 0 & 0\\ 0 & 0 & 0\end{array}\right], & & \displaystyle\end{eqnarray}$$
where
$\unicode[STIX]{x1D63F}$
and
$\unicode[STIX]{x1D652}$
are the strain-rate and vorticity tensors, respectively.
The balance equations for the set of
$10$
hydrodynamic fields
$(n,\boldsymbol{u},\unicode[STIX]{x1D648})$
follow from (2.1) by multiplying it with
$\unicode[STIX]{x1D713}=1$
,
$\boldsymbol{C}$
and
$\boldsymbol{C}\boldsymbol{C}$
, respectively, and integrating the resulting equations over the velocity space. For the steady unidirectional flow (2.3), the mass balance equation is identically satisfied. It is straightforward to verify that the momentum balance equation, with Stokes drag law, boils down to
implying that there is zero slip (i.e.
$\boldsymbol{u}=\boldsymbol{v}$
) between the particle phase and the gas phase. Note that for a dense suspension there is a hydrodynamic contribution to the particle-phase stress tensor (Batchelor Reference Batchelor1970; Hinch Reference Hinch1977) whose origin was originally thought to be tied to the particle stresslet (Nott & Brady Reference Nott and Brady1994) but has recently been reinterpreted (Lhuillier Reference Lhuillier2009; Nott, Guazzelli & Pouliquen Reference Nott, Guazzelli and Pouliquen2011). More specifically, Nott et al. (Reference Nott, Guazzelli and Pouliquen2011) showed that the net force due to hydrodynamic interactions in the particle-phase momentum equation can be decomposed into an interphase drag and the divergence of a hydrodynamic stress. It may be noted that the latter contribution in the momentum equation,
$\unicode[STIX]{x1D735}\boldsymbol{\cdot }\unicode[STIX]{x1D64B}^{h}$
, vanishes under homogeneous deformation (2.3).
Incorporating (2.4) and neglecting hydrodynamic stress, the balance equation for the second moment is (Saha & Alam Reference Saha and Alam2017)
where
$\unicode[STIX]{x1D64B}\equiv \unicode[STIX]{x1D70C}\langle \boldsymbol{C}\boldsymbol{C}\rangle +\unicode[STIX]{x1D723}(m\boldsymbol{C})=\unicode[STIX]{x1D64B}^{k}+\unicode[STIX]{x1D64B}^{c}$
is the stress tensor,
$\unicode[STIX]{x1D64C}\equiv \unicode[STIX]{x1D70C}\langle \boldsymbol{C}\boldsymbol{C}\boldsymbol{C}\rangle +\unicode[STIX]{x1D723}(m\boldsymbol{C}\boldsymbol{C})=\unicode[STIX]{x1D64C}^{k}+\unicode[STIX]{x1D64C}^{c}$
is the flux of the second moment, and
$\boldsymbol{\aleph }\equiv \boldsymbol{\aleph }(m\boldsymbol{C}\boldsymbol{C})$
is the collisional source of second moment. The first and second terms in
$\unicode[STIX]{x1D64B}$
and
$\unicode[STIX]{x1D64C}$
refer to the corresponding kinetic and collisional contributions, respectively. The integral expressions for
$\boldsymbol{\aleph }(\unicode[STIX]{x1D713})$
and
$\unicode[STIX]{x1D723}(\unicode[STIX]{x1D713})$
are given by (Jenkins & Richman Reference Jenkins and Richman1985; Saha & Alam Reference Saha and Alam2016)
$$\begin{eqnarray}\displaystyle \unicode[STIX]{x1D723}(\unicode[STIX]{x1D713}) & = & \displaystyle -\frac{\unicode[STIX]{x1D70E}^{3}}{2}\iiint _{\boldsymbol{g}\boldsymbol{\cdot }\boldsymbol{k}>0}(\unicode[STIX]{x1D713}_{1}^{\prime }-\unicode[STIX]{x1D713}_{1})\boldsymbol{k}\int _{0}^{1}f^{(2)}(\boldsymbol{c}_{1},\boldsymbol{x}-\unicode[STIX]{x1D714}\unicode[STIX]{x1D70E}\boldsymbol{k},\boldsymbol{c}_{2},\boldsymbol{x}+\unicode[STIX]{x1D70E}\boldsymbol{k}-\unicode[STIX]{x1D714}\unicode[STIX]{x1D70E}\boldsymbol{k})\nonumber\\ \displaystyle & & \displaystyle \times \,(\boldsymbol{k}\boldsymbol{\cdot }\boldsymbol{g})\,\text{d}\unicode[STIX]{x1D714}\,\text{d}\boldsymbol{k}\,\text{d}\boldsymbol{c}_{1}\,\text{d}\boldsymbol{c}_{2},\end{eqnarray}$$
respectively, where
$f^{(2)}(\cdot )$
is the two-particle distribution function,
$\unicode[STIX]{x0394}\unicode[STIX]{x1D713}=(\unicode[STIX]{x1D713}_{1}^{\prime }+\unicode[STIX]{x1D713}_{2}^{\prime }-\unicode[STIX]{x1D713}_{1}-\unicode[STIX]{x1D713}_{2})$
, and
$\unicode[STIX]{x1D714}$
in (2.7) represents a current coordinate. The second-moment balance (2.5) also contains an energy source term (Koch Reference Koch1990; Koch & Sangani Reference Koch and Sangani1999) that is proportional to the slip velocity
$\boldsymbol{u}_{s}=\boldsymbol{u}-\boldsymbol{v}$
. This source term is a consequence of long-range hydrodynamic interactions but it vanishes identically for homogeneous shear flow, see (2.4), and hence does not affect the following analysis. Also, the possible impact of the omission of the hydrodynamic stress in (2.5) on our predictions will be discussed in § 5.2.
At the continuum level, the hydrodynamic interactions are retained via the viscous dissipation term in (2.5) that follows from the relation (Sangani et al. Reference Sangani, Mo, Tsao and Koch1996)
where
$f_{diss}(\unicode[STIX]{x1D708})$
is the hindrance factor that accounts for the finiteness of the volume fraction of particles,
$\unicode[STIX]{x1D708}$
, in a dense system. Note that Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996) derived (2.8) by assuming a Maxwellian velocity distribution function. The possible impact of an anisotropic hydrodynamic force driven by the anisotropic particle velocity distribution on the rheology of suspensions is assumed to be negligible in this work. The closed-form expression of
$f_{diss}(\unicode[STIX]{x1D708})$
has been determined by Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996) as
where
$\unicode[STIX]{x1D716}_{m}=9.76\unicode[STIX]{x1D706}_{g}/\unicode[STIX]{x1D70E}$
is the lubrication cutoff,
$\unicode[STIX]{x1D706}_{g}$
is the mean free path of the gas molecules, and
which is known to hold up to a particle volume fraction close to the freezing-point density
$\unicode[STIX]{x1D708}=\unicode[STIX]{x1D708}_{f}\approx 0.5$
. The logarithmic divergence of
$f_{diss}(\unicode[STIX]{x1D708},\unicode[STIX]{x1D716}_{m})$
with
$\unicode[STIX]{x1D716}_{m}$
in (2.9) is due to the non-continuum lubrication flows in the narrow gap between two colliding particles (Hockling Reference Hockling1973). The effective dissipation function (2.9) may also depend on the particle Reynolds number
$Re_{p}$
(Verberg & Koch Reference Verberg and Koch2006) – the possible impact of such inertial effects on suspension rheology will be analysed in § 5.3.
For a finite-density suspension, our analysis is carried out based on a density-corrected effective Stokes number,
being an effective viscous time scale for a dense system. In the dilute limit
$(\unicode[STIX]{x1D708}\rightarrow 0)$
,
$f_{diss}(\unicode[STIX]{x1D708})\rightarrow 1$
and consequently we have
$St_{d}=St$
and
$\unicode[STIX]{x1D70F}_{vis}^{e}\rightarrow \unicode[STIX]{x1D70F}_{vis}$
.
3 Non-perturbative theory for a sheared finite-density suspension
3.1 Maximum entropy principle and the anisotropic Maxwellian distribution
To evaluate the collision integrals (2.6) and (2.7), information about the two-body distribution function is needed for which we adopt the well-known molecular chaos ansatz, which implies that the two-particle distribution function can be factored as
$f^{(2)}(\boldsymbol{c}_{1},\boldsymbol{x}-\unicode[STIX]{x1D70E}\boldsymbol{k},\boldsymbol{c}_{2},\boldsymbol{x})=g_{0}(\unicode[STIX]{x1D708})f(\boldsymbol{c}_{1},\boldsymbol{x}-\unicode[STIX]{x1D70E}\boldsymbol{k})\,f(\boldsymbol{c}_{2},\boldsymbol{x})$
, where
$g_{0}(\unicode[STIX]{x1D708})$
is the contact radial distribution function as given in (2.11).
Employing the maximum entropy principle (Jaynes Reference Jaynes1957) based on the constraints of 10 hydrodynamic fields
$(\unicode[STIX]{x1D70C},\boldsymbol{u},\unicode[STIX]{x1D648})$
, a variational problem can be set up for the entropy
$S=-\int \,f(\boldsymbol{c},\boldsymbol{x},t)\ln f(\boldsymbol{c},\boldsymbol{x},t)\,\text{d}\boldsymbol{c}$
in terms of Lagrange multipliers. It follows (see appendix A in Saha & Alam (Reference Saha and Alam2017)) that the single-particle velocity distribution is given by an anisotropic Maxwellian
with
$|\unicode[STIX]{x1D648}|=\det (\unicode[STIX]{x1D648})$
. For an isotropic second moment
$M_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}=T\unicode[STIX]{x1D6FF}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
, (3.1) boils down to the standard Maxwellian
$f(C)\propto \exp (-mC^{2}/2)\equiv f_{M}$
, which can also be derived from the maximum entropy principle for the five-field theory of
$(\unicode[STIX]{x1D70C},\boldsymbol{u},T)$
at the Euler or NS order.
The anisotropic Maxwellian (3.1) has been used in dry granular flows (Goldreich & Tremaine Reference Goldreich and Tremaine1978; Shukhman Reference Shukhman1984; Araki & Tremaine Reference Araki and Tremaine1986; Jenkins & Richman Reference Jenkins and Richman1988; Richman Reference Richman1989; Saha & Alam Reference Saha and Alam2014, Reference Saha and Alam2016; Alam & Saha Reference Alam and Saha2017) as well as in recent works on dilute gas–solid suspensions (Vié, Doisneau & Massot Reference Vié, Doisneau and Massot2015; Kong et al.
Reference Kong, Fox, Feng, Capecelatro and Desjardins2017; Saha & Alam Reference Saha and Alam2017). Following our previous work (Saha & Alam Reference Saha and Alam2017), the anisotropic Maxwellian
$f_{AM}$
is chosen as the leading distribution function for dense gas–solid suspensions under homogeneous shearing. Apart from providing an exact non-perturbative theory for the homogeneously sheared suspension, the ansatz of (3.1) is crucial for the quantitative validity of the present theory (dubbed ‘AME’ for anisotropic Maxwellian expansion) over a large range of Stokes numbers at any value of the restitution coefficient – we shall verify this in § 4. The latter assumption also makes the present work different from all previous moment theories (‘Grad-moment expansion’ (GME) theory, based on an Hermite expansion around the Maxwellian distribution function (Grad Reference Grad1949)) for gas–solid suspensions (Tsao & Koch Reference Tsao and Koch1995; Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996; Parmentier & Simonin Reference Parmentier and Simonin2012).
3.2 Balance of second moment
The second-moment balance equation (2.5) under homogeneous shearing condition (2.3) simplifies to
where
$\mathit{u}_{\unicode[STIX]{x1D6FC},\unicode[STIX]{x1D6FD}}=\unicode[STIX]{x2202}\mathit{u}_{\unicode[STIX]{x1D6FC}}/\unicode[STIX]{x2202}x_{\unicode[STIX]{x1D6FD}}$
is the velocity-gradient tensor (2.3) and
is the total stress tensor, with its collisional component being
$\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}^{c}=\unicode[STIX]{x1D6E9}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}\equiv m\unicode[STIX]{x1D6E9}_{\unicode[STIX]{x1D6FC}}[C_{\unicode[STIX]{x1D6FD}}]$
as defined in (2.7). The collisional source of the second moment
$\aleph _{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}=\aleph [mC_{\unicode[STIX]{x1D6FC}}C_{\unicode[STIX]{x1D6FD}}]$
, defined in (2.6), can be rewritten as
and the integral expressions of
$A_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
,
$\widehat{\unicode[STIX]{x1D640}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
and
$\widehat{\unicode[STIX]{x1D642}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
can be found in Saha & Alam (Reference Saha and Alam2016); note that the hatted tensors
$\widehat{\unicode[STIX]{x1D640}}$
and
$\widehat{\unicode[STIX]{x1D642}}$
are trace-less. Substituting (3.3) and (3.4) into (3.2) yields
where
$\unicode[STIX]{x1D6E4}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}=A_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}+\widehat{\unicode[STIX]{x1D640}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}+\widehat{\unicode[STIX]{x1D642}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
. The system of four equations (3.5) must be solved to analyse the hydrodynamics and rheology of a sheared gas–solid suspension under homogeneous shearing deformation.
3.3 Anisotropy of the second-moment tensor
$\unicode[STIX]{x1D648}$
For the homogeneous shear flow (2.3), the eigendirections of the strain-rate tensor
$\unicode[STIX]{x1D63F}$
are
$|\unicode[STIX]{x1D60B}_{1}\!\rangle =(1,1,0)$
,
$|\unicode[STIX]{x1D60B}_{2}\!\rangle =(-1,1,0)$
and
$|\unicode[STIX]{x1D60B}_{3}\!\rangle =(0,0,1)$
. Let (
$\unicode[STIX]{x1D614}_{1},\unicode[STIX]{x1D614}_{2},\unicode[STIX]{x1D614}_{3}$
) be the eigenvalues of
$\unicode[STIX]{x1D648}$
, with respective eigendirections being
$|\unicode[STIX]{x1D614}_{1}\!\rangle$
,
$|\unicode[STIX]{x1D614}_{2}\!\rangle$
and
$|\unicode[STIX]{x1D614}_{3}\!\rangle =|\unicode[STIX]{x1D60B}_{3}\!\rangle$
. In the Cartesian
$(x,y,z)$
coordinate frame, the second-moment tensor is completely characterized by (Saha & Alam Reference Saha and Alam2017)
$$\begin{eqnarray}\displaystyle \unicode[STIX]{x1D648}=T\left[\begin{array}{@{}ccc@{}}1+\unicode[STIX]{x1D706}^{2}+\unicode[STIX]{x1D702}\sin 2\unicode[STIX]{x1D719} & -\unicode[STIX]{x1D702}\cos 2\unicode[STIX]{x1D719} & 0\\ -\unicode[STIX]{x1D702}\cos 2\unicode[STIX]{x1D719} & 1+\unicode[STIX]{x1D706}^{2}-\unicode[STIX]{x1D702}\sin 2\unicode[STIX]{x1D719} & 0\\ 0 & 0 & 1-2\unicode[STIX]{x1D706}^{2}\end{array}\right], & & \displaystyle\end{eqnarray}$$
in terms of (i) the temperature anisotropy (
$\unicode[STIX]{x1D702}$
) or the difference between the principal eigenvalues on the shear (
$x,y$
) plane,
where
$T_{i}=\langle C_{i}^{2}\rangle$
is the temperature along the
$i$
th direction, (ii) the non-coaxiality angle (
$\unicode[STIX]{x1D719}$
), i.e. the angle between the principal eigendirections of the strain-rate tensor and the second-moment tensor,
(iii) the excess temperature (
$\unicode[STIX]{x1D706}^{2}$
) along the vorticity direction
and (iv) the scaled shear rate (
$R$
) or the Savage–Jeffrey parameter (Savage & Jeffrey Reference Savage and Jeffrey1981)
which is nothing but the inverse of the square root of the granular temperature. It follows from (2.2) and (3.6) that
$\widehat{\unicode[STIX]{x1D648}}=0$
when
$\unicode[STIX]{x1D702}=0=\unicode[STIX]{x1D719}=\unicode[STIX]{x1D706}^{2}$
, resulting in an isotropic second moment
$M_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}=T\unicode[STIX]{x1D6FF}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
. Therefore, three parameters (
$\unicode[STIX]{x1D702},\unicode[STIX]{x1D719},\unicode[STIX]{x1D706}^{2}$
) completely characterize the anisotropy of
$\unicode[STIX]{x1D648}$
for homogeneous shear flow.
3.4 Principal axes frame and transformed equations
Instead of the Cartesian
$(x,y,z)$
coordinates, the reference frame is shifted to the eigenspace of
$\unicode[STIX]{x1D648}$
, spanned by the respective orthonormal triad of eigendirections (
$|\unicode[STIX]{x1D614}_{1}\!\rangle ,|\unicode[STIX]{x1D614}_{2}\!\rangle ,|\unicode[STIX]{x1D614}_{3}\!\rangle$
), with
$|\unicode[STIX]{x1D614}_{1}\!\rangle =[\cos \unicode[STIX]{x1D703},\sin \unicode[STIX]{x1D703},0]$
and
$|\unicode[STIX]{x1D614}_{2}\!\rangle =[-\sin \,\unicode[STIX]{x1D703},\cos \unicode[STIX]{x1D703},0]$
, where
$\unicode[STIX]{x1D703}=\unicode[STIX]{x1D719}+\unicode[STIX]{x03C0}/4$
is the angle between the
$x$
-axis and new
$x^{\prime }$
-axis, and
$|\unicode[STIX]{x1D614}_{3}\!\rangle =[0,0,1]\equiv |\unicode[STIX]{x1D60B}_{3}\!\rangle$
is directed along the
$z$
-axis. The new coordinate axes
$(x^{\prime },y^{\prime },z^{\prime })$
system is called the principal axes frame (Richman Reference Richman1989; Saha & Alam Reference Saha and Alam2016, Reference Saha and Alam2017) on which the second-moment tensor becomes a diagonal matrix,
via the rotation matrix
${\mathcal{R}}(\unicode[STIX]{x1D703})=[|\unicode[STIX]{x1D614}_{1}\!\rangle ,|\unicode[STIX]{x1D614}_{2}\!\rangle ,|\unicode[STIX]{x1D614}_{3}\!\rangle ]$
.
By employing
${\mathcal{R}}(\unicode[STIX]{x1D703})$
, in the principal axes frame the second-moment balance equation (3.5) can be written as four independent equations:
representing, respectively, (i) the trace of (3.5), with
$A_{\unicode[STIX]{x1D6FC}^{\prime }\unicode[STIX]{x1D6FC}^{\prime }}=A_{x^{\prime }x^{\prime }}+A_{y^{\prime }y^{\prime }}+A_{z^{\prime }z^{\prime }}$
, (ii) the
$(z^{\prime },z^{\prime })$
component of the deviatoric part of (3.5), (iii) the difference between the
$(x^{\prime },x^{\prime })$
and
$(y^{\prime },y^{\prime })$
components and (iv) the off-diagonal
$(x^{\prime },y^{\prime })$
component of (3.5). The under-braced terms in (3.12)–(3.14) are the contributions from the gas phase. The expressions for various integrals
$A_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
,
$\widehat{\unicode[STIX]{x1D60C}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
,
$\widehat{\unicode[STIX]{x1D60E}}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
and
$\unicode[STIX]{x1D6E9}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
appearing in (3.12)–(3.15) remain the same as those for the dry granular flow, which have been evaluated explicitly by Saha & Alam (Reference Saha and Alam2016):
Inserting (3.16) into (3.12)–(3.15) results in a system of four nonlinear algebraic equations with four unknowns (
$\unicode[STIX]{x1D702},\unicode[STIX]{x1D719},\unicode[STIX]{x1D706}^{2},R$
) which are obtained by numerically solving (3.12)–(3.15) for specified values of (
$\unicode[STIX]{x1D708},e,St$
).
4 Results and discussion
Having solved the second-moment balance equations (3.12)–(3.15) for
$\unicode[STIX]{x1D702}(\unicode[STIX]{x1D708},e,St)$
,
$\unicode[STIX]{x1D719}(\unicode[STIX]{x1D708},e,St)$
,
$\unicode[STIX]{x1D706}^{2}(\unicode[STIX]{x1D708},e,St)$
and
$R(\unicode[STIX]{x1D708},e,St)$
, the kinetic part of the stress tensor
$\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}^{k}=\unicode[STIX]{x1D70C}M_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
is determined from (3.6) and its collisional part
$\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}^{c}=\unicode[STIX]{x1D6E9}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
from (3.16a
) – all components of the stress tensor (3.3) are thus determined. The transport coefficients of a sheared suspension are subsequently evaluated as functions of (
$\unicode[STIX]{x1D708},e,St$
):
and the first and second normal-stress differences
respectively, where
$p=\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FC}}/3$
is the pressure; the dimensionless granular temperature is
$T/\dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}=1/64R$
, where
$R$
is the Savage–Jeffrey parameter (i.e. dimensionless shear rate) defined in (3.10); the pressure is made dimensionless via
$p/\unicode[STIX]{x1D70C}_{p}\dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}$
.
4.1 Comparison with DSMC simulation
To validate theoretical predictions (4.1) and (4.2), we have solved the Boltzmann–Enskog equation (2.1) using the well-known stochastic algorithm, DSMC (Bird Reference Bird1994; Gupta & Alam Reference Gupta and Alam2017) – the related algorithmic details for the homogeneous shear flow of a dense hard-sphere system can be found in Montanero & Santos (Reference Montanero and Santos1997) and those for a dilute suspension in Tsao & Koch (Reference Tsao and Koch1995). The correction for excluded-volume effects is taken care of via the Enskog factor (2.11) while (i) calculating the collision frequency and (ii) choosing the collision pairs. Equation (2.1) is transformed to the Lagrangian frame, moving with the shear field (2.3), and the particles experience an effective Stokes’ drag force as in (2.8) and (2.9). The crucial point of choosing the time step in DSMC is done by satisfying
$\unicode[STIX]{x0394}t<\min (\unicode[STIX]{x1D70F}_{vis}^{e},\unicode[STIX]{x1D70F}_{col})$
where
$\unicode[STIX]{x1D70F}_{col}$
is the collision time scale, taken to be a small fraction of the mean free time of hard spheres, and
$\unicode[STIX]{x1D70F}_{vis}^{e}=\unicode[STIX]{x1D70F}_{vis}/f_{diss}(\unicode[STIX]{x1D708})$
is an effective viscous time scale for a dense suspension that follows from the definition of the density-corrected Stokes number
$St_{d}$
(2.12). Once the system reaches a statistical steady state, the macroscopic quantities are calculated – in addition to the kinetic contribution to the stress tensor (
$\unicode[STIX]{x1D64B}^{k}$
), its collisional part
$\unicode[STIX]{x1D64B}^{c}$
must be calculated (Montanero & Santos Reference Montanero and Santos1997). In all simulations the lubrication cutoff is set to
$\unicode[STIX]{x1D716}_{m}=0.01$
in (2.9), and choosing a different value of
$\unicode[STIX]{x1D716}_{m}\in (0.05,0.01,0.001)$
did not noticeably affect the predicted transport coefficients.
Figure 1 confirms the excellent agreement between the DSMC simulation data (marked by symbols) and the present theoretical predictions (solid lines) for (a) shear viscosity
$\unicode[STIX]{x1D707}$
, (b) pressure
$p$
, and (c) first (
${\mathcal{N}}_{1}$
) and (d) second (
${\mathcal{N}}_{2}$
) normal-stress differences at
$St=10$
. The dot-dashed and dashed lines correspond to the NS order theory (Garzo et al.
Reference Garzo, Tenneti, Subramaniam and Hrenya2012) and the 13-moment theory based on Grad’s moment expansion (dubbed ‘GME’ theory (Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996)), respectively. It is clear that the present theory fares remarkably well in correctly predicting both NS (
$\unicode[STIX]{x1D707}$
and
$p$
) and non-Newtonian (
${\mathcal{N}}_{1}$
and
${\mathcal{N}}_{2}$
) transport coefficients over the whole range of restitution coefficients even for a Stokes number of
$St=10$
at a finite density of
$\unicode[STIX]{x1D708}=0.2$
. According to the GME theory,
${\mathcal{N}}_{2}=0$
(see figure 1
d) and
${\mathcal{N}}_{1}>0$
(see figure 1
c), but the latter is overpredicted (compared to the simulation data) by a factor of approximately 2–4 over the whole range of restitution coefficients. The overall agreement in figure 1 between the AME theory and the simulation data also holds excellently for higher values of
$St$
(see § 4.2).
Predictions of AME (solid lines) for (a) shear viscosity, (b) pressure, (c)
${\mathcal{N}}_{1}$
and (d)
${\mathcal{N}}_{2}$
for the whole range of the restitution coefficient
$e$
; the particle volume fraction is set to
$\unicode[STIX]{x1D708}=0.2$
and the Stokes number is
$St=10$
(i.e.
$St_{d}\approx 2.5$
). The dashed lines represent the GME theory of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996), the dot-dashed lines in panels (a) and (b) represent the NS order theory of Garzo et al. (Reference Garzo, Tenneti, Subramaniam and Hrenya2012) and the symbols correspond to DSMC data.

Before presenting the results on the
$St$
dependence of transport coefficients, it is interesting to compare our predictions in figure 1 with previous works on dilute suspensions. Referring to figure 12 of Saha & Alam (Reference Saha and Alam2017), which corresponds to a particle volume fraction of
$\unicode[STIX]{x1D708}=0.01$
with other parameters as in figure 1, we recall that the quantitative predictions of the GME theory were found to be comparable to those of the AME theory for both the shear viscosity and the first normal-stress difference even for highly inelastic particles with
$e\geqslant 0.5$
. On increasing the volume fraction to a modest value of
$\unicode[STIX]{x1D708}=0.2$
, however, the predictions of the GME theory become poor at all restitution coefficients, as demonstrated in figure 1. In contrast, the predictions of the present theory (including the second normal-stress difference) remain superior at finite densities over the whole range of restitution coefficients.
4.2 Predictions at large and small Stokes numbers
Since the Stokes number and particle Reynolds number are related via
$St=(2/9)(\unicode[STIX]{x1D70C}_{p}/\unicode[STIX]{x1D70C}_{g})Re_{p}$
, the limit of rapid granular suspension (
$St\gg 1$
) is easily satisfied since
$\unicode[STIX]{x1D70C}_{p}/\unicode[STIX]{x1D70C}_{g}\gg 1$
in most gas–solid systems; it is also possible to reach the limit of
$St\sim O(Re_{p}\ll 1)$
if
$\unicode[STIX]{x1D70C}_{p}\sim \unicode[STIX]{x1D70C}_{g}$
, which corresponds to a liquid–solid suspension. Of course, the many-body hydrodynamic interactions are important in the latter limit, all of which are not incorporated in the present theory, as pointed out in § 2. Given that the theory and the DSMC simulation have identical assumptions, in this section our primary goals are (i) to analyse the performance of the present theory over existing theories over a wide range of
$St$
for different values of
$\unicode[STIX]{x1D708}$
and
$e$
, and (ii) to determine to what extent the theory can be used in the small-
$St$
regime. The effect of full hydrodynamic interactions on the predicted rheology will be discussed in §§ 5.1 and 5.2.
Figures 2 and 3 display the
$St$
dependence of (a) particle-phase shear viscosity
$\unicode[STIX]{x1D707}$
, (b) granular temperature
$T$
, and (c) first (
${\mathcal{N}}_{1}$
) and (d) second (
${\mathcal{N}}_{2}$
) normal-stress differences, for particle volume fractions of
$\unicode[STIX]{x1D708}=0.2$
and
$0.5$
, respectively; the related range of the effective Stokes number
$St_{d}$
(2.12) is marked on the top horizontal axis in each panel. Focusing on the high-
$St$
regime in figures 2 and 3, it is seen that the predictions of the GME theory (Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996) for all fields become poorer with decreasing restitution coefficient
$e$
. In particular, the first normal-stress difference (figures 2
c and 3
c) is overpredicted in the GME theory and its disagreement with the simulation data increases significantly in a denser suspension, as can be seen from a comparison between figures 2(c) (
$\unicode[STIX]{x1D708}=0.2$
) and 3(c) (
$\unicode[STIX]{x1D708}=0.5$
) at
$St\gg 1$
– this disagreement is noteworthy despite the negligible effects of hydrodynamic interactions in the high-
$St$
regime. In contrast, the present theory can quantitatively predict all transport coefficients (
$\unicode[STIX]{x1D707}$
,
${\mathcal{N}}_{1}$
and
${\mathcal{N}}_{2}$
) over a large range of Stokes numbers
$St\in (0.01,100)$
at
$\unicode[STIX]{x1D708}=0.2$
(figure 2) and
$0.5$
(figure 3) even for highly inelastic (
$e=0.5$
) particles.
Variations of the (a) particle-phase shear viscosity
$\unicode[STIX]{x1D707}$
, (b) granular temperature
$T$
, and (c) first
$({\mathcal{N}}_{1})$
and (d) second
$({\mathcal{N}}_{2})$
normal-stress differences plotted against Stokes number
$St$
; the axis on the top represents the effective Stokes number
$St_{d}$
; see (2.12). The solid and dashed lines, respectively, denote the present theory and the GME theory of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996); the magenta dot-dashed line refers to the NS theory of Garzo et al. (Reference Garzo, Tenneti, Subramaniam and Hrenya2012); the circles (
$e=0.9$
) and squares (
$e=0.5$
) denote DSMC results. The particle volume fraction is set to
$\unicode[STIX]{x1D708}=0.2$
.

Same as figure 2, but for a dense suspension with particle volume fraction
$\unicode[STIX]{x1D708}=0.5$
.

In the small-
$St$
regime, the predictions for shear viscosity (figures 2
a and 3
a), granular temperature (figures 2
b and 3
b) and
${\mathcal{N}}_{1}$
(figures 2
c and 3
c) based on the GME theory are qualitatively different from those of the present theory and DSMC simulation. For example, at
$St\rightarrow 0$
, the scaled viscosity (and also pressure) approaches some constant value in the present theory, while it decays linearly with
$St$
in GME theory. In figure 2(a,b), the dot-dashed lines represent the NS theory (Garzo et al.
Reference Garzo, Tenneti, Subramaniam and Hrenya2012) which closely follow the GME theory in the small-
$St$
limit (
$St\ll 1$
). Note that the quantitative predictions of the NS theory deteriorate with decreasing
$e$
in the high-
$St$
limit – this is a well-known defect of all NS models (Saha & Alam Reference Saha and Alam2016; Alam & Saha Reference Alam and Saha2017).
Let us now discuss about the behaviour of two normal-stress differences in terms of the second-moment anisotropy. From the definition of the kinetic stress
$\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}^{k}=\unicode[STIX]{x1D70C}M_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}$
and employing (3.6), the anisotropies of the second-moment tensor can be expressed as
where
$p^{k}=\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FC}}^{k}/3$
is the kinetic pressure. From the simulation data on
$\unicode[STIX]{x1D617}_{\unicode[STIX]{x1D6FC}\unicode[STIX]{x1D6FD}}^{k}$
, three anisotropy parameters have been calculated from (4.3), and their variations with
$St$
and
$St_{d}$
are shown by symbols in figure 4(a–c), with solid lines representing theoretical predictions at
$\unicode[STIX]{x1D708}=0.2$
. The related results at a higher volume fraction of
$\unicode[STIX]{x1D708}=0.5$
look similar (and hence are not displayed) – in general, the magnitudes of (
$\unicode[STIX]{x1D702},\unicode[STIX]{x1D719},\unicode[STIX]{x1D706}^{2}$
) decrease with increasing density and vice versa in the high-
$St$
regime. From figure 4 we find that
$\unicode[STIX]{x1D719}\rightarrow 0$
and
$\unicode[STIX]{x1D706}^{2}\rightarrow 1/3$
at
$St\rightarrow 0$
, and hence it follows from (4.3) that
The first normal-stress difference can be expressed in terms of the anisotropy parameters (Saha & Alam Reference Saha and Alam2016),
${\mathcal{N}}_{1}\propto \unicode[STIX]{x1D702}\sin 2\unicode[STIX]{x1D719}$
, and hence it vanishes at
$St\rightarrow 0$
due to
$\sin 2\unicode[STIX]{x1D719}\rightarrow 0$
(see figure 4
b) as confirmed in figures 2(c) and 3(c). Therefore, according to the present theory, the vanishing of
${\mathcal{N}}_{1}$
at
$St\rightarrow 0$
is tied to the collinearity (
$\unicode[STIX]{x1D719}\rightarrow 0$
) of the eigendirections of the second-moment and shear tensors in the same limit. On the other hand, the order-one value of the second normal-stress difference at
$St\rightarrow 0$
in figures 2(d) and 3(d) is tied to the fact that the temperature (
$T_{z}$
) in the vorticity direction is much different from those in the shear plane since
$T_{x}+T_{y}=8T_{z}$
in this limit.
Variations with
$St$
or
$St_{d}$
of the second-moment anisotropy parameters: (a)
$\unicode[STIX]{x1D702}$
(temperature anisotropy in the shear plane, equation (3.7)), (b)
$\unicode[STIX]{x1D719}$
(the non-coaxiality angle, equation (3.8)) and (c)
$\unicode[STIX]{x1D706}^{2}$
(the excess temperature, equation (3.9)) for
$\unicode[STIX]{x1D708}=0.2$
.

Comparison with the simulation data of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996) for
$e=1$
and
$\unicode[STIX]{x1D708}=0.1$
: (a) shear viscosity, (b) granular temperature and (c)
${\mathcal{N}}_{1}$
. The filled circles and open triangles refer to their data with and without full hydrodynamic interactions, respectively; the open squares represent our DSMC data, which incorporate an effective drag term (
$\propto f_{diss}(\unicode[STIX]{x1D708})$
) to update particle trajectories. The solid and dashed lines refer to the present theory and the GME theory of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996), respectively.

5 Discussion: hydrodynamic interactions, viscous scaling and inertial effects
5.1 Effect of hydrodynamic interactions
Recall that the present theory does not include all many-body hydrodynamic interactions: the long-range hydrodynamic interactions and the short-range lubrication force are incorporated only via the viscous dissipation term (calculated with an isotropic Maxwellian distribution function) in the second-moment equation. However, (i) the effects of the anisotropic particle distribution function on hydrodynamic interactions, (ii) the fluid flow affecting the particle distribution function and (iii) the interactions due to shear-induced particle stresslet are neglected. Such detailed hydrodynamic interactions with non-Maxwellian velocity distribution for both the particle and gas phases may impact the effective viscous dissipation terms that are neglected in the present theory. In any case, to check the possible implications of detailed hydrodynamic interactions in simple shear, we compare our theory in figure 5 with the simulation data of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996) that includes all hydrodynamic interactions – this refers to the case of elastically colliding (
$e=1$
) particles for a volume fraction of
$\unicode[STIX]{x1D708}=0.1$
. The filled circles and open triangles refer to their data with and without full hydrodynamic interactions, respectively; the open squares represent our DSMC simulation data which incorporate hydrodynamic interactions only via the effective drag force (equations (2.8) and (2.9)). It is seen that both sets of simulation data for (a)
$\unicode[STIX]{x1D707}$
, (b)
$T$
and (c)
${\mathcal{N}}_{1}$
overlap with each other as well as with two theories (AME and GME) at Stokes numbers of
$St_{d}>5$
(i.e.
$St>10$
). This implies that many-body hydrodynamic interactions do not noticeably affect the rheology of suspensions (
$e=1$
) at moderate to high values of the Stokes number – this overall conclusion also holds at higher volume fractions (as confirmed from a comparison of our theory with the simulation data for
$\unicode[STIX]{x1D708}=0.25$
and
$0.45$
obtained from figures 12 and 13 of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996)).
Focusing on the small-
$St$
regime of figure 5, we find that the quantitative predictions of the present theory are better than those of the GME theory even at a small value of
$St_{d}=2$
. On the other hand, the simulation data with full hydrodynamic interactions (filled circles in figure 5
c) indicate that the first normal-stress difference increases with decreasing
$St$
, reaching some finite value at
$St=0$
– this is known to be a consequence of many-body hydrodynamic interactions in dense suspensions (Brady & Bossis Reference Brady and Bossis1988; Nott & Brady Reference Nott and Brady1994; Boyer, Pouliquen & Guazzelli Reference Boyer, Pouliquen and Guazzelli2011). The latter may be contrasted with the non-monotonic variation of
${\mathcal{N}}_{1}$
with
$St$
, leading to
${\mathcal{N}}_{1}\rightarrow 0$
at
$St\rightarrow 0$
, according to our theory and DSMC simulation. This non-monotonic variation is also captured by the simulation data of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996), marked by the open triangles in figure 5(c) – note that the latter simulations incorporate only an effective drag term to update particle trajectories as in our DSMC simulations.
It is interesting to note in figure 5(c) that the GME theory (dashed line) seems to predict the correct
$St$
dependence of the hydrodynamic simulation data for
${\mathcal{N}}_{1}\neq 0$
at
$St\rightarrow 0$
; this prediction is incorrect. We have verified (Saha & Alam 2019, unpublished) that a consistent ‘second-order’ GME theory, which incorporates all second-order nonlinearities in the production and flux terms (equations (2.6) and (2.7)), yields a non-monotonic variation of
${\mathcal{N}}_{1}$
with
$St$
, similar to the present predictions of the AME theory.
Based on above comparisons between simulation and theory, we conclude that the detailed hydrodynamic interactions must be included in the present theory to recover the correct behaviour of the first normal-stress difference at
$St\rightarrow 0$
. In this regard, the (shear-induced) anisotropic microstructure is another missing link in the present theory which may be incorporated via the two-body distribution function.
5.2 Scaling of stress
Recall from figures 2(a) and 3(a) that the shear viscosity has two distinct plateaus at
$St\gg 1$
(high viscosity) and
$St\ll 1$
(low viscosity); the related variations of the particle pressure with
$St$
(not shown) are similar. In the high-
$St$
regime, the (dimensional) granular temperature scales like
$T\sim \dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}$
(see figures 2
b and 3
b), yielding a quadratic dependence of stress with the shear rate (i.e.
$\unicode[STIX]{x1D617}_{xy}\sim \dot{\unicode[STIX]{x1D6FE}}^{2}$
) – this is the well-known Bagnoldian or inertial scaling of stress that holds in rapid granular flows (
$St\rightarrow \infty$
).
In the small-
$St$
regime too, the present theory recovers the same inertial scaling of stress (
$\unicode[STIX]{x1D617}_{xy}\sim \dot{\unicode[STIX]{x1D6FE}}^{2}$
), and the (dimensional) particle-phase viscosity has a linear dependence on the shear rate (
$\tilde{\unicode[STIX]{x1D707}}_{AME}\sim \dot{\unicode[STIX]{x1D6FE}}\sim St/\unicode[STIX]{x1D70F}_{vis}$
). This can be understood from the energy balance equation by equating the shear work (
$\unicode[STIX]{x1D617}_{xy}\dot{\unicode[STIX]{x1D6FE}}$
) with the viscous dissipation (
$\unicode[STIX]{x1D6E4}_{vis}=2\unicode[STIX]{x1D70C}T/\unicode[STIX]{x1D70F}_{vis}^{e}$
) since inelastic dissipation is insignificant at
$St\ll 1$
. This yields an expression for the shear stress as
$\unicode[STIX]{x1D617}_{xy}\sim n\unicode[STIX]{x1D70E}\unicode[STIX]{x1D707}_{g}T/\dot{\unicode[STIX]{x1D6FE}}$
, which, together with the scaling for the temperature
$T\sim St\dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}$
(figure 2
b), leads to
$\unicode[STIX]{x1D617}_{xy}^{\,AME}\sim \unicode[STIX]{x1D70C}\dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}$
at
$St\ll 1$
. This scaling holds also in DSMC simulations as is evident from the simulation data on the low-viscosity branch in figures 2(a) and 3(a). These predictions are at odds with the well-known viscous scaling of stress,
$\lim _{St\rightarrow 0}\unicode[STIX]{x1D617}_{xy}\propto \unicode[STIX]{x1D707}_{g}\dot{\unicode[STIX]{x1D6FE}}$
, for Stokesian suspensions.
At a phenomenological level, the viscous scaling of stress can be recovered by incorporating the hydrodynamic contribution to the particle-phase stress tensor via
$\unicode[STIX]{x1D64B}=\unicode[STIX]{x1D64B}^{k}+\unicode[STIX]{x1D64B}^{c}+\unicode[STIX]{x1D64B}^{h}$
. For low-Reynolds-number suspensions, Nott & Brady (Reference Nott and Brady1994) suggested an expression for the hydrodynamic stress:
where
$\unicode[STIX]{x1D6F1}$
is the particle pressure,
$\unicode[STIX]{x1D63F}=(\unicode[STIX]{x1D735}\boldsymbol{u}+(\unicode[STIX]{x1D735}\boldsymbol{u})^{\dagger })/2$
is the strain-rate tensor,
$\unicode[STIX]{x1D707}_{r}(\unicode[STIX]{x1D708})$
is the relative viscosity, which is an increasing function of the particle volume fraction, and
$\unicode[STIX]{x1D729}$
is a fourth-rank tensor that takes care of normal-stress differences. In fact, (5.1) represents the dominant contribution to the particle stress tensor at
$St\rightarrow 0$
. Neglecting normal-stress differences in (5.1) and plugging it into the energy balance (2.5) yields
$T\sim \dot{\unicode[STIX]{x1D6FE}}^{2}\unicode[STIX]{x1D70E}^{2}$
– this is dubbed the ‘suspension’ temperature, which is tied with the non-affine motion of the particles. The above scaling is the same as that of Nott & Brady (Reference Nott and Brady1994), and would lead to a plateau in figure 2(b) at
$St\rightarrow 0$
– of course, the stress scaling now remains viscous. A detailed analysis would require constitutive relations for the particle pressure
$\unicode[STIX]{x1D6F1}=\unicode[STIX]{x1D6F1}_{0}+\unicode[STIX]{x1D707}_{g}p_{r}(\unicode[STIX]{x1D708})\dot{\unicode[STIX]{x1D6FE}}$
, the density dependence of the relative viscosity
$\unicode[STIX]{x1D707}_{r}(\unicode[STIX]{x1D708})$
and the fourth-rank tensor
$\unicode[STIX]{x1D729}$
(Nott & Brady Reference Nott and Brady1994; Lhuillier Reference Lhuillier2009; Guazzelli & Pouliquen Reference Guazzelli and Pouliquen2018). In summary, a phenomenological hybrid approach to incorporate the hydrodynamic stress in the manner of Nott & Brady (Reference Nott and Brady1994) could be useful to recover (i) the viscous scaling of stress and (ii) the correct shear-rate scaling of normal-stress differences at
$St\rightarrow 0$
.
Effects of particle Reynolds number (
$Re_{p}$
) on transport coefficients: (a) shear viscosity, and (b) first
$({\mathcal{N}}_{1})$
and (c) second
$({\mathcal{N}}_{2})$
normal-stress differences. The lines denote theoretical predictions for different values of
$Re_{p}$
with a particle volume fraction of
$\unicode[STIX]{x1D708}=0.5$
and
$e=0.9$
.

5.3 Effect of fluid inertia
As clarified in § 2, all the above results are applicable strictly for zero-Reynolds-number (
$Re_{p}=0$
) suspensions. In the context of the present theory, the possible effects of fluid inertia (
$Re_{p}>0$
) on the particle-phase rheology can be ascertained via a modified viscous dissipation function (2.8). In this regard, an approximate expression for the dissipation function has been suggested by Verberg & Koch (Reference Verberg and Koch2006):
Here
$Re_{T}$
is the thermal Reynolds number based on the granular temperature
with
$Re_{p}=\unicode[STIX]{x1D70C}_{g}\dot{\unicode[STIX]{x1D6FE}}\unicode[STIX]{x1D70E}^{2}/\unicode[STIX]{x1D707}_{g}$
being the particle Reynolds number, and
is a transition Reynolds number that demarcates two regimes defined via
We have incorporated (5.2) in the second-moment balance equations (3.12)–(3.15) that are solved for specified values of (
$Re_{p},\unicode[STIX]{x1D708},e,St$
). Figure 6 shows the influence of
$Re_{p}$
on transport coefficients predicted by the present theory; the particle volume fraction is set to
$\unicode[STIX]{x1D708}=0.5$
and the restitution coefficient is
$e=0.9$
. The qualitative behaviour of each transport coefficient with varying
$St$
remains the same as that for
$Re_{p}=0$
and also at other values of
$\unicode[STIX]{x1D708}$
. It is seen that the shear viscosity decreases but the normal-stress differences are enhanced with increasing fluid inertia at
$Re_{p}=10$
, and the changes are negligible at
$Re_{p}=1$
as well as at
$St<1$
(not shown). Increased viscous dissipation with increasing
$Re_{p}$
is responsible for the reduction of the particle-phase viscosity. On the whole, our predictions in § 4 would remain largely unaffected at small finite values of the particle Reynolds number.
6 Conclusion and outlook
The Boltzmann–Enskog kinetic theory has been employed to analyse the hydrodynamics and rheology of Stokesian gas–solid suspensions undergoing homogeneous shear flow by extending the anisotropic moment theory of Saha & Alam (Reference Saha and Alam2017) to the dense regime. The hydrodynamic interactions were accounted for in the second-moment balance equation via a density-dependent viscous dissipation term (with a lubrication cutoff) as in the work of Sangani et al. (Reference Sangani, Mo, Tsao and Koch1996) and the particles were subject to linear Stokes’ drag law. The anisotropic Maxwellian was chosen as the single-particle distribution function that follows from the maximum entropy principle (Jaynes Reference Jaynes1957; Saha & Alam Reference Saha and Alam2014, Reference Saha and Alam2016, Reference Saha and Alam2017) for an extended set of 10 hydrodynamic fields – the resulting non-perturbative theory includes normal-stress differences and holds for homogeneously sheared suspensions of arbitrary shear rate.
Based on the above assumptions, we showed that the present theory bridges the rapid granular limit (
$St\rightarrow \infty$
) and the small-Stokes-number (
$St\ll 1$
) limit of finite-density viscous gas–solid suspensions, providing quantitative agreements for the shear viscosity and two normal-stress differences with simulation data for (i) all values of the restitution coefficient,
$0<e\leqslant 1$
(figure 1), and (ii) a wide range of particle volume fractions,
$\unicode[STIX]{x1D708}\leqslant 0.5$
(figures 1–4). In contrast, the existing moment theories (Sangani et al.
Reference Sangani, Mo, Tsao and Koch1996; Parmentier & Simonin Reference Parmentier and Simonin2012), with identical assumptions about hydrodynamic interactions as in the present theory, are found to hold only for Stokes numbers of
$St\geqslant O(10)$
with nearly elastic (
$e\approx 1$
) particles (figures 1 and 5). The first normal-stress difference is markedly overpredicted in dense suspensions and the second normal-stress difference is zero in the existing theories, but the latter is finite according to the present theory and simulation.
The limitations of the present theory at
$St\rightarrow 0$
can be tied to the omission of detailed hydrodynamic interactions and the related microstructural anisotropies, both of which are important in dense suspensions. For example, the scaling of the stress remains Bagnoldian/inertial (i.e. the stress varies quadratically with the shear rate) and the first normal-stress difference is zero at
$St\rightarrow 0$
for any finite
$\unicode[STIX]{x1D708}$
– both predictions are at odds with known results on Stokesian suspensions. In the context of the present kinetic theory approach, the incorporation of full many-body hydrodynamic interactions, possibly via the two-body distribution function and an anisotropic (shear-induced) pair-correlation function, remains an open issue that should be addressed in future.
Acknowledgements
This work is funded by the Department of Science and Technology under ‘India–Netherlands’ project (Ref. DST/INT/NL/P-03/2016); S.S. was supported by this project via a postdoctoral fellowship. Theory was worked out by M.A. and S.S.; R.G. wrote the numerical (DSMC) code and S.S. carried out the analysis of the numerical data. The work was conceived, supervised and written by M.A.







