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Suppressing capillary instability in falling liquid threads

Published online by Cambridge University Press:  28 November 2024

Chase T. Gabbard
Affiliation:
School of Engineering, Brown University, Providence, RI 02912, USA
James T. Rhoads
Affiliation:
Department of Mechanical Engineering, Clemson University, Clemson, SC 29631, USA
Joshua B. Bostwick*
Affiliation:
Department of Mechanical Engineering, Clemson University, Clemson, SC 29631, USA
*
†Email address for correspondence: jbostwi@clemson.edu

Abstract

A cylindrical liquid thread readily destabilizes into a series of drops due to capillary instability, which is also responsible for undesirable bead-on-fibre structures observed when coating a thin fibre. In this experimental study, we show how a falling liquid thread can be stabilized by internally distorting the cross-sectional shape using two vertically hung fibres. Below a critical flow rate $Q_c$, the dual-fibre system deforms the falling thread into a smooth column with a non-circular cross-section, thereby suppressing instability. Above $Q_{{c}}$, the cylindrical thread is left undeformed by the fibres and destabilizes into beads connected by a stable, non-cylindrical film. An empirical stability threshold is identified showing that flow delays the onset of capillary instability when compared with a marginally stable quasi-static coating. When the flow is unstable $Q>Q_c$, the bead velocity $v$ obeys a simple scaling law that is well supported by our experiments over a large parameter range. This suppression technique can be extended to other slender geometries, such as a ribbon, which shows similar qualitative results but exhibits a different stability threshold due to spontaneous dewetting about its short edge.

Information

Type
JFM Papers
Creative Commons
Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (http://creativecommons.org/licenses/by/4.0), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
© The Author(s), 2024. Published by Cambridge University Press.
Figure 0

Figure 1. Bead-on-fibre instabilities. (a) Symmetric beading pattern with silicone oil that diminishes as the fibre radius $r$ increases from left ($r=0.05$ mm) to right ($r=0.45$ mm). (b) Asymmetric beading patterns form for larger surface tension values, as shown for glycerol ($r=0.25$ mm). (c) Secondary instabilities can develop in the thin film connecting beads, known as the isolated regime ($r=0.05$ mm). (d) An applied cross-flow can change the pattern from symmetric to asymmetric, eventually causing bead detachment ($r=0.25$ mm).

Figure 1

Figure 2. (a) Experimental set-up with inset showing the internal design of the nozzle housing. (b) The falling thread shown in side and front views with thicknesses $d_s$ and $d_f$, respectively. (c) Typical experiment showing a flat fluid thread (left) for a flow rate $Q=75$ ml hr$^{-1}$ and wavy thread (right) for $Q=300$ ml hr$^{-1}$. Here, the fluid viscosity is $\mu =350$ m Pa s, fibre radius $r=0.3$ mm and fibre gap $w=0.4$ mm. (d) Dimensionless thread thickness $\bar {d}=d/r$ against dimensionless time $\bar {t}=t/t_{f}$, where $t_f$ is the duration of the recording, for the two experiments shown in (c). The best-fit curve for each experiment is shown in black and the locations of the maximum $d_{max}$ and minimum $d_{min}$ thicknesses are denoted by the solid and hollow triangles, respectively.

Figure 2

Figure 3. (a) Front view (left) and side view (right) of liquid deposited on two parallel fibres with radius $r=0.25$ mm and spacing $w=0.8$ mm at a flow rate $Q=100$ ml hr$^{-1}$. The dashed and solid lines denote the liquid–air interface of the front and side view, respectively. (b) Normalized thread diameter $d/d_n$ against distance from the nozzle $z/l_c$, where $d_n$ is the nozzle diameter and $l_c$ is the capillary length, as it depends on flow rate $Q$. Front view and side view measurements are distinguished using a dashed and solid line, respectively, with approximate cross-sectional shapes. (c) Thread eccentricity $\alpha =1-d^{s}/d^{f}$ against flow rate $Q$. (d) Normalized relative thread diameter $\hat {d}=(d_{ss}-d)/(d_{ss}-d_{n})$, with $d_{ss}$ the pre-instability steady-state thread diameter, against distance from the nozzle $z/l_{c}$ for the side and front views.

Figure 3

Figure 4. Illustration of instability mechanism showing a (a) non-circular cross-section $Q< Q_c$ and (b) circular cross-section for $Q>Q_c$ with associated perturbed interfaces. For $Q< Q_{c}$ the long edge is fixed by the edges of the fibres, such that perturbations only affect the radius of curvature $R$ along the short edge giving rise to a stabilizing capillary flow from the crest to the trough. For $Q>Q_{c}$ the circular thread is always unstable due to an increased pressure (decreased curvature) at the trough, thus driving the instability.

Figure 4

Figure 5. (a) Thread destabilization as the flow rate $Q$ increases from left to right showing stable and unstable threads. Here, $r=0.25$, $w=0.2$ mm and $\mu =339$ m Pa s. Scale bar is 3 mm long. (b) Maximum thread diameter $d_{max}$, (c) minimum thread diameter $d_{min}$ and (d) dimensionless amplitude $\tilde {a}=a/r_{t}$ against $Q$ as measured in front (grey circle) and side view (blue star). The vertical black line denotes the stability threshold $Q=Q_{c}$. Inset illustrations show the approximate cross-sectional shape for $Q< Q_{c}$ (purple) and $Q>Q_{c}$ (orange).

Figure 5

Figure 6. (a) Critical flow rate $Q_c$ against the characteristic length $r_{t}$, as it depends upon fibre radius $r$ for viscosity $\mu =47$ m Pa s. The data fall along the curve $Q_{c} \sim r_{t}^{4}$. (b) Value of $Q_c$ against $r_{t}$ as it depends upon $\mu$ for $r=0.25$ mm.

Figure 6

Figure 7. (a) Stability diagram showing stable (purple) and unstable (orange) threads by plotting dimensionless maximum diameter $\tilde {d}=d_{max}^{s} /r_{t}$ against visco-gravitational number $\beta = \rho g r_{t}^{4} /\mu Q$. The dashed line denotes the stability threshold $\widetilde {d_{c}} = 2.68 \pm 0.21$ with the shaded region showing the empirical overlap. Plot markers indicate the viscosity of each test. (b) Side view images for different $\beta$ with $\tilde {d}=4.8$, 2.5, 2.1 and 2, from left to right.

Figure 7

Figure 8. (a) Typical spatio-temporal diagram with beads shown in white for $r=0.25$ mm and $w=1$ mm. The thread profile is tracked at a fixed vertical location (horizontal orange line) and the power density (PD) is determined using an FFT. (b) Bead velocity $v$ against flow rate $Q$, as it depends upon viscosity $\mu$. (c) Dimensionless bead velocity $\tilde {v}=v / v_{t}$, where $v_{t}=Q / r_{t}^{2}$, against visco-gravitational number $\beta = \rho g r_{t}^{4} /\mu Q$ exhibits a power-law trend with exponent $n=2/5$ and coefficient of determination $R^{2}=0.96$. The colour bars in (b,c) indicate the characteristic length $r_t$.

Figure 8

Figure 9. (a) Silicone oil ($\mu =47$ m Pa s) flowing down a nylon ribbon of thickness $a=0.01$ mm and width $b=3$ mm exhibits instability as the flow rate increases from left to right. Scale bar is 3 mm long. (b) Maximum (grey circles) and minimum (blue star) thread diameter $d^{s}$ measured perpendicular to the ribbon width and ($c$) dimensionless wave amplitude $\tilde {a}=a/r_{t}$, with $r_{t}=b/2=1.5$ mm, against flow rate $Q$. For low $Q$, the maximum and minimum thread diameters are similar and $\tilde {a}$ is small. For high $Q$, the film is unstable causing the maximum and minimum thread diameter to diverge and $\tilde {a}$ to increase.

Supplementary material: File

Gabbard et al. supplementary movie 1

This movie shows the videos associated with the images in Figure 5(a). Here, thread destabilization occurs as the flow rate Q increases from left to right for fiber radius r = 0.25 mm, spacing w = 0.2 mm, and viscosity μ = 339 \ m Pa s.
Download Gabbard et al. supplementary movie 1(File)
File 8.3 MB
Supplementary material: File

Gabbard et al. supplementary movie 2

Silicone oil with viscosity μ = 339 \ m Pa s flowing down nylon fibers with radius r = 0.25 mm and spacing w = 1 mm. This video is associated with the spatiotemporal diagram in Figure 8(a).
Download Gabbard et al. supplementary movie 2(File)
File 8.8 MB