Hostname: page-component-74656f9884-j7cmm Total loading time: 0 Render date: 2026-11-09T07:30:30.885Z Has data issue: false hasContentIssue false

Birefringent strands drive the flow of viscoelastic fluids past obstacles

Published online by Cambridge University Press:  02 September 2022

O. Mokhtari
Affiliation:
Institut de Mécanique des Fluides de Toulouse (IMFT), CNRS & Université de Toulouse, 31400 Toulouse, France TotalEnergies E&P, CSTJF, 64018 Pau, France
J.-C. Latché
Affiliation:
Institut de Radioprotection et de Sûreté Nucléaire (IRSN), 13115 Saint-Paul-Lez-Durance, France
M. Quintard
Affiliation:
Institut de Mécanique des Fluides de Toulouse (IMFT), CNRS & Université de Toulouse, 31400 Toulouse, France
Y. Davit*
Affiliation:
Institut de Mécanique des Fluides de Toulouse (IMFT), CNRS & Université de Toulouse, 31400 Toulouse, France
*
†Email address for correspondence: yohan.davit@imft.fr

Abstract

The flow of polymer solutions past solid obstacles or through porous media gives rise to rich physical phenomena over a wide range of spatial and temporal scales. Viscoelasticity, in particular, can induce a strong nonlinear response with an increase of flow resistance even for a solution whose viscosity decreases in simple shear flow. Various hypotheses have been proposed to explain this phenomenon but a clear picture of the pore-scale mechanisms involved and their impact upon larger scales is still lacking. Here, we show that localized zones of large polymeric stress, known as birefringent strands, drive the flow of an Oldroyd-B fluid through two-dimensional arrays of cylinders. Combining a recently developed numerical scheme with high performance computing, we find that these strands generate a complete reorganization of the flow with an increase of stagnation zones, a reinforcement of preferential paths and a splitting of flow channels. Furthermore, we show that this reorganization is the source of an increase in the viscous dissipation of the solvent and also that the stretching of polymer molecules in the strands is associated with entropy production. Both these phenomena yield a global increase in dissipation that can be directly linked to the increase of flow resistance. Our results demonstrate that the birefringent strands – not the elongational viscosity – drive the flow of viscoelastic fluids through porous media and that the increase of flow resistance can occur even at steady state, before the transition to elastic turbulence.

Information

Type
JFM Papers
Creative Commons
Creative Common License - CCCreative Common License - BY
This is an Open Access article, distributed under the terms of the Creative Commons Attribution licence (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted re-use, distribution and reproduction, provided the original article is properly cited.
Copyright
© The Author(s), 2022. Published by Cambridge University Press.
Figure 0

Figure 1. Examples of experimental observations of the formation of birefringent strands in the literature, with (a,d,f) cases with one cylinder; (c,e,g) cases with two cylinders; and (b) a cross-slot device. In (f,h,g,i), the results correspond to two different regimes of flow with (f,g) steady symmetric and (h,i) steady asymmetric. Panels (a,c) are reproduced from Haward, Toda-Peters & Shen (2018) with permission. Panel (b) is reproduced from Haward & McKinley (2013) with permission. Panels (d,e) are reproduced from Sun & Huang (2016) with permission. Panels (f–i) are reproduced from Hopkins, Haward & Shen (2020) with permission. In all panels, birefringence is characterized by the retardation, $R(\text {nm})$, between two optical paths, which stems from differences in refractive index due to polymer molecules. This local change in the optical property of the polymer solution is also a proxy for visualizing stress as it can be linked to the local principal stress difference through the stress–optic law, which states that there is a linear relationship between $R$ and the difference in principal stresses.

Figure 1

Figure 2. Example simulations of the flow of an Oldroyd-B fluid through an array of cylinders in the case with a Weissenberg number ${\simeq }5$ and $\beta =1$ (see § 2.1 for definitions). Plots of (a) the trace of the conformation tensor ${\rm tr}(\boldsymbol{\mathsf{c}})$, which represents the stretching of the polymer chains, and (b) velocity magnitude $\Vert \,\boldsymbol {u}\Vert$.

Figure 2

Figure 3. Typical geometry with boundary conditions. The boundary conditions are top–bottom periodicity and $\boldsymbol {u}=(0,0)^{\mathrm {T}}$ on the cylinder. Two types of boundary conditions are used for left- and right-hand sides, either (a) an inlet condition on the left-hand side, $\boldsymbol {u}=(1,0)^{\mathrm {T}}$ and $\boldsymbol{\mathsf{c}}=\boldsymbol{\mathsf{I}}$, and an outlet condition on the right-hand side, $p_{ext}=0$ (see (2.9)), or (b) periodic boundary conditions with the flow generated through a body force $\boldsymbol {F}$. (a) Inlet/outlet. (b) Biperiodic.

Figure 3

Figure 4. Schematic of mesh and unknowns corresponding to the RT element for quadrilateral cells. The degrees of freedom for the pressure and the conformation tensor are located at the centre of the cells. The degrees of freedom for the velocity components are located at the centre of the faces of the mesh and associated with the dual cells. For a rectangular mesh and each face of it, the dual cell is the union of the cones with basis the face and vertex the mass centre of an adjacent cell. The dual cell corresponding to the face between the two rectangular cells is shown in grey.

Figure 4

Table 1. Characteristics of the meshes used for the calculations. Lengths are non-dimensionalized with the radius of the cylinder as a reference.

Figure 5

Figure 5. Schematic of the geometry for a single cylinder. The length scales of the system are $H=20$ the height of the domain, $L_{in}=25$ the distance from the inlet to the centre of the cylinder and $L$ the total length of the domain. The length $L=L_{in}+30Wi$ is chosen sufficiently large so that the conformation tensor relaxes to its equilibrium value $\boldsymbol{\mathsf{c}}=\boldsymbol{\mathsf{I}}$ before reaching the boundary condition on the right-hand side. The boundary conditions are top–bottom periodicity and $\boldsymbol {u}=\boldsymbol {0}$ on the cylinder. Left/right boundary conditions are either inlet/outlet conditions or periodicity depending on the calculation.

Figure 6

Table 2. Summary of parameters and dimensionless numbers used for flow past a single cylinder.

Figure 7

Figure 6. Flow past a single cylinder in the case $\beta =1$ and inlet/outlet boundary conditions; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,c,e,g,i) and $\Vert \,\boldsymbol {u}\Vert$ (b,d,f,h,j) for different $Wi$. Panels (a,b) to (i,j) show $Wi=1$, $Wi=2$, $Wi=4$, $Wi=8$ and $Wi=16$. For ease of visualization, the range of the colour bar for the velocity field has been fixed to the interval $[0,1.6]$ with $1.6$ corresponding to the maximum value in the case $Wi=16$.

Figure 8

Figure 7. Flow past a single cylinder in the case $\beta =0$. (a) Value of ${\mathsf{c}}_{xx}$ along the line $x=1$ for different values of $Wi$. (b) Maximum of ${\mathsf{c}}_{xx}$ along the line $x=1$ as a function of $Wi$ (log–log axes). (c) Value of $\textrm {tr}(\boldsymbol{\mathsf{c}}-\boldsymbol{\mathsf{I}})$ along the centreline in the wake of the cylinder for different values of $Wi$ (log–linear axes). (d) Maximum of $\textrm {tr}(\boldsymbol{\mathsf{c}}-\boldsymbol{\mathsf{I}})$ along the centreline in the wake as a function of $Wi$ (log–log axes).

Figure 9

Figure 8. Flow past one cylinder in the case $\beta =0$ and $Wi\simeq 9$. Magnified areas near (a,c,e) and away (b,d,f) from the cylinder for the first and second components of $\boldsymbol {\nabla }\boldsymbol {\cdot}\boldsymbol{\mathsf{c}}^{0}$.

Figure 10

Figure 9. Flow past one cylinder with $Wi\simeq 9$ and biperiodic boundary conditions. Plots of (a) the trace of the zero-order conformation $\boldsymbol{\mathsf{c}}^{0}$ and (b) the longitudinal component of the first-order velocity $u_{x}^{1}$ with streamlines.

Figure 11

Figure 10. Flow past a single cylinder in the case $Wi=4$; (a) $\textrm {tr}(\boldsymbol{\mathsf{c}}-\boldsymbol{\mathsf{I}})$ normalized by its max and (b) $1-u_{x}$ along the centreline in the near wake of the cylinder for different values of $\beta$.

Figure 12

Figure 11. Schematic of the geometry for two cylinders aligned with the flow. The length scales of the system are $H=20$ the height of the domain, $D$ the distance between the cylinders centres, $L_{in}=25$ the distance from the inlet to the centre of the cylinder and $L$ the total length of the domain. The length $L=L_{in}+D+30Wi$ is chosen sufficiently large so that the conformation tensor relaxes to its equilibrium value $\boldsymbol{\mathsf{c}}=\boldsymbol{\mathsf{I}}$ before reaching the boundary condition on the right-hand side. The boundary conditions are top–bottom periodicity and $\boldsymbol {u}=\boldsymbol {0}$ on the cylinder. Left/right boundary conditions are either inlet/outlet conditions or periodicity, depending on the calculation. Meshes are uniform structured grids where the cylinders are defined by holes.

Figure 13

Figure 12. Flow past two cylinders aligned with the flow with $\beta =1$. Value of $\textrm {tr}(\boldsymbol{\mathsf{c}})$ as a function of $Wi$ in the case $D=3$ (a,c,e) and $D=20$ (b,d,f). From (a,b) to (e,f), $Wi=5$, $Wi=10$ and $Wi=20$. Boundary conditions are inlet/outlet conditions.

Figure 14

Table 3. Summary of parameters and dimensionless numbers used for flow past two cylinders aligned with the flow.

Figure 15

Figure 13. Flow past two cylinders aligned with the flow in the case $\beta =1$, $D=7$ and inlet/outlet boundary conditions; (a,c,e,g,i) $\textrm {tr}(\boldsymbol{\mathsf{c}})$ and (b,d,f,h,j) velocity magnitude with streamlines magnified between the cylinders, as a function of $De$. From (a,b) to (i,j), $De=0.7$, $De=1.4$, $De=1.8$, $De=2.1$ and $De=2.8$.

Figure 16

Figure 14. Flow past two aligned cylinders with $Wi\simeq 9$, $De\simeq 1.5$ and biperiodic boundary conditions. Plots of (a) the trace of the zero-order conformation $\boldsymbol{\mathsf{c}}^{0}$ and (b) the longitudinal component of the first-order velocity $u_{x}^{1}$ with streamlines.

Figure 17

Figure 15. Flow past two cylinders aligned with the flow with $Wi=20$, $De=3.33$ and inlet/outlet boundary conditions; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,c,e,g) and velocity magnitude with streamlines (b,d,f,h) as a function of $\beta$. Panels (a,b) to (g,h), $\beta =0$, $\beta =0.1$, $\beta =0.2$ and $\beta =0.4$.

Figure 18

Figure 16. Schematic of the geometry for two cylinders orthogonal to the direction of the flow. The length scales of the system are $H=20$ the height of the domain, $D$ the distance between the cylinders centres, $L_{in}=25$ the distance from the inlet to the centre of the cylinder and $L$ the total length of the domain. The length $L=L_{in}+30Wi$ is chosen sufficiently large so that the conformation tensor relaxes to its equilibrium value $\boldsymbol{\mathsf{c}}=\boldsymbol{\mathsf{I}}$ before reaching the boundary condition on the right-hand side. This geometry is characterized by the gap ratio, $G=({D-2})/({H-(D+2)})$. The boundary conditions are top–bottom periodicity and $\boldsymbol {u}=\boldsymbol {0}$ on the cylinder. Left/right boundary conditions are either inlet/outlet conditions or periodicity, depending on the calculation. Meshes are uniform structured grids where the cylinders are defined by holes.

Figure 19

Table 4. Summary of parameters and dimensionless numbers used for flow past two cylinders orthogonal to the flow.

Figure 20

Figure 17. Flow past two cylinders orthogonal to the flow in the case with $\beta =1$, $G=0.6$ and inlet/outlet boundary conditions; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,c,e,g) and velocity magnitude (b,d,f,h) as a function of $Wi$. Panels (a,b) to (g,h), $Wi=1$, $Wi=5$, $Wi=10$ and $Wi=20$.

Figure 21

Figure 18. Flow past two cylinders orthogonal to the flow. Flow rate between the cylinders, normalized by the Newtonian value, for different values of the gap ratio $G$ as a function of (a) $Wi$ in the case $\beta =1$ and (b) the viscosity ratio $\beta$ in the case $Wi=10$.

Figure 22

Figure 19. Flow past two cylinders orthogonal to the flow in the case with $\beta =0$, $Wi=10$ and inlet/outlet boundary conditions; $\textrm {tr}(\boldsymbol{\mathsf{c}}^{0})$ as a function of $G$; (a,c,e,g) $G<1$, from top to bottom $G=0$, $G=0.14$, $G=0.33$ and $G=0.6$, (b,d,f,h) $G\geq 1$, from top to bottom $G=1$, $G=1.67$, $G=3$ and $G=7$.

Figure 23

Figure 20. Flow past two cylinders orthogonal to the flow with $Wi\simeq 8$, $G=0.23$ and biperiodic boundary conditions. Plots of (a) the trace of the zero-order conformation $\boldsymbol{\mathsf{c}}^{0}$ and (b) the longitudinal component of the first-order velocity $u_{x}^{1}$ with streamlines.

Figure 24

Figure 21. Flow past two cylinders orthogonal to the flow with $Wi=10$, $G=0.23$ and inlet/outlet boundary conditions; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,c,e,g) and velocity magnitude (b,d,f,h) as a function of $\beta$. From (a,b) to (g,h), $\beta =0$, $\beta =0.5$, $\beta =1$ and $\beta =4$.

Figure 25

Figure 22. Schematic of the $10\times 10$ crystalline cylinder structure and example of random displacement (blue cylinder) with a maximum displacement $\varepsilon$. Boundary conditions are biperiodic and the flow is imposed through a body force $\boldsymbol {F}$. Meshes are uniform structured grids where the cylinders are defined by holes.

Figure 26

Table 5. Summary of parameters and dimensionless numbers used for flow in a lattice of cylinders.

Figure 27

Figure 23. Flow through arrays of cylinders for $\beta =1$. Fields of $\textrm {tr}(\boldsymbol{\mathsf{c}})$ as a function of $Wi$ and of the maximum displacement, $\varepsilon$, of each cylinder.

Figure 28

Figure 24. Flow through an array of cylinders in the case $\beta =1$ and $\varepsilon =3$; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,c,e) and velocity magnitude (b,d,f) as a function of $Wi$. From (a,b) to (e,f), $Wi\simeq 1.5$, $Wi\simeq 5$ and $Wi\simeq 11.5$.

Figure 29

Figure 25. Flow through an array of cylinders in the case $\beta =1$ and $\varepsilon =3$. Magnified areas for $\textrm {tr}(\boldsymbol{\mathsf{c}})$ and the velocity magnitude presented in figure 24. These areas capture the three principal effects of the strands and envelopes on the flow through an array of cylinders with (a) an increase of the zones of stagnation, (b) an amplification of the preferential flow paths and (c) a splitting of flow channels. The top right figure positions each magnified area in the array.

Figure 30

Figure 26. Flow through an array of cylinders in the case $\beta =1$ and $\varepsilon =3$. Probability density functions for the longitudinal component of the velocity field, $u_{x}$, as a function of $Wi$. The inset is a magnification of the framed area.

Figure 31

Figure 27. Flow through an array of cylinders in the case $\beta =1$ and $\varepsilon =0$; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,b), viscous dissipation $\mathcal {E}_{v}$ (c,d) and polymeric dissipation $\mathcal {E}_{e}$ (e,f) as a function of $Wi$. For visualization purposes, the colour bar for dissipation starts at $0.1$, so all values below 0.1 are represented in dark blue.

Figure 32

Figure 28. Flow through an array of cylinders in the case $\beta =1$ and $\varepsilon =2$; $\textrm {tr}(\boldsymbol{\mathsf{c}})$ (a,b), viscous dissipation $\mathcal {E}_{v}$ (c,d) and polymeric dissipation $\mathcal {E}_{e}$ (e,f) as a function of $Wi$. For visualization purposes, the colour bar for dissipations starts at $0.1$, so all values below 0.1 are represented in dark blue.

Figure 33

Figure 29. Flow through an array of cylinders in the case $\varepsilon =2$. Evolution of the viscous and polymeric dissipations and their sum corresponding to the drag coefficient $\mathcal {C}$ as a function of $Wi$ for different values of $\beta$. The subscript $_\mathcal {N}$ indicates the normalization by the Newtonian value of $\mathcal {C}$ in the limit $Wi\rightarrow 0$; (a) $\beta =0.5$, (b) $\beta =1$, (c) $\beta =2$.

Figure 34

Figure 30. Flow through arrays of cylinders in the case $\beta =1$. Comparison of the drag coefficient evolution with $Wi$ between the cases $\varepsilon =0$ and $\varepsilon =2$. The subscript $_\mathcal {N}$ indicates the normalization by the Newtonian value of $\mathcal {C}$, corresponding to the limit $Wi\rightarrow 0$.

Figure 35

Figure 31. Biperiodic array of cylinder. (a) Schematics of the geometry and boundary conditions. The geometry consists of a single cylinder of radius $1$ in a square of size $4$. The boundary conditions are top–bottom and left–right periodicity and $\boldsymbol {u}=0$ on the cylinder. (b) Initial mesh in the case $N=10$. (c) Refinement in the case $r=2$. (d) Body-fitted mesh in the case $N=40$.

Figure 36

Figure 32. Biperiodic array of cylinder. Evolution of the drag coefficient as a function of $Wi$ for (a) different values of the mesh size $N$ with a constant refinement $r=1$ and a body-fitted mesh in the case $N=300$ and (b) different values of the refinement $r$ with a constant mesh size $N=100$.