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Gas-sheared falling liquid films beyond the absolute instability limit

Published online by Cambridge University Press:  25 September 2023

Misa Ishimura
Affiliation:
Université Paris-Saclay, CNRS, FAST, 91405 Orsay, FranceUniversité Savoie Mont Blanc, CNRS, LOCIE, 73000 Chambèry, FranceDepartment of Mechanical Engineering, Yokohama National University, Kanagawa 240-8501, Japan
Sophie Mergui
Affiliation:
Université Paris-Saclay, CNRS, FAST, 91405 Orsay, FranceSorbonne Université, UFR 919, 4 place Jussieu, F-75252 Paris CEDEX 05, France
Christian Ruyer-Quil
Affiliation:
Université Savoie Mont Blanc, CNRS, LOCIE, 73000 Chambèry, France
Georg F. Dietze*
Affiliation:
Université Paris-Saclay, CNRS, FAST, 91405 Orsay, France
*
†Email address for correspondence: dietze@fast.u-psud.fr

Abstract

We study the effect of a confined turbulent counter-current gas flow on the waviness of a weakly inclined falling liquid film. Our study is centred on experiments in a channel of 13 mm height, using water and air, where we have successively increased the counter-current gas flow rate until flooding. Computations with a new low-dimensional model and linear stability calculations are used to elucidate the linear and nonlinear wave dynamics. We find that the gas pressure gradient plays an important role in countering the stabilizing effect of the tangential gas shear stress at the liquid–gas interface. At very low inclination angles, the latter effect dominates and can suppress the long-wave Kapitza instability unconditionally. By contrast, for non-negligible inclination, the gas effect is linearly destabilizing, amplifies the height of nonlinear Kapitza waves, and exacerbates coalescence-induced formation of large-amplitude tsunami waves. Kapitza waves do not undergo any catastrophic transformation when the counter-current gas flow rate is increased beyond the absolute instability (AI) limit. On the contrary, we find that AI is an effective linear wave selection mechanism in a noise-driven wave evolution scenario, leading to highly regular downward-travelling nonlinear wave trains, which preclude coalescence events. In our experiments, where Kapitza waves develop in a protected region before coming into contact with the gas, flooding is eventually caused far beyond the AI limit by upward-travelling short-wave ripples. Based on our linear stability calculations for arbitrary wavenumbers, we have uncovered a new short-wave interfacial instability mode with negative linear wave speed, causing these ripples.

Information

Type
JFM Papers
Copyright
© The Author(s), 2023. Published by Cambridge University Press
Figure 0

Figure 1.Sketch of our experimental set-up. A falling liquid film of water flows down a glass plate inclined at an angle $\phi =5^{\circ }$, and enters into contact with a counter-current turbulent air flow within a rectangular channel of height $H^\star =13$ mm and width $W^\star =27$ mm. A loudspeaker is used to force Kapitza waves on the surface of the liquid film, which grow and saturate within a protected region.

Figure 1

Figure 2.Transition of the wavy falling liquid film under a counter-current gas flow: water/air, $Re_L^{as}=44.7$, $Re_L=43.1$, $f_0^\star =3$ Hz. Shadowgraphs of the liquid–gas interface for increasingly strong fan power: (a) zero fan power (aerostatic configuration), regularly-spaced Kapitza waves; (b) $Re_G=-5830$, coalescence of Kapitza waves; (c) $Re_G=-6760$, coexistence of Kapitza waves with upward-travelling short ripples.

Figure 2

Figure 3.Typical CCI film thickness measurements in the aerostatic configuration: water/air, $Re_L^{as}=33.7$, $f_0^\star =2.8$ Hz. (a) Film thickness time traces measured at different positions. From left to right: $x^\star =13.5$, 27.5, 49.5 and 62.5 cm. (b) Spatial profiles of averaged quantities (at least 100 waves). Open/filled circles indicate ensemble-averaged wave height $h_{max}^\star$ and minimum film thickness $h_{min}^\star$; crosses indicate time-averaged film thickness $\bar {h}^\star$. Error bars indicate standard deviation, and red arrows mark positions for the traces in (a).

Figure 3

Figure 4.Falling liquid film (subscript $L$) on an inclined wall subject to a counter-current turbulent gas flow (subscript $G$). The flow is confined by an upper wall (not shown) at $y^\star =H^\star$ (stars denote dimensional quantities), and a symmetry condition is imposed at the centreline of the average gas layer $y^\star =D^\star$. Gas–liquid coupling is expressed via the tangential gas shear stress $T_G$ and the gas pressure $P_G$ at the film surface $y^\star =h^\star$. Red dashed lines illustrate the orthogonal curvilinear coordinate system $(\eta, \xi )$, where $\eta =\underline {y}\bar {d}/d$.

Figure 4

Figure 5.Spatial linear stability calculations with the WRIBL-OS approach. Parameters based on experiments of Kofman et al. (2017): $Ka=3174$ (water and air I in table 1), $\phi =5^\circ$, $Re_L=45$. Circles: passive-gas limit, $\varPi _\rho =\varPi _\mu =0$ in (3.41). Values of $|Re_G|$ increase in the order diamonds, squares, crosses, pentagons. (a,c) Full model, (b,d) $\varPi _\rho =0$ in (3.41), with (a,b) $H^\star =19$ mm, (c,d) $H^\star =40$ mm. Here: (a) $Re_G=[-6234, -8145, -8490\ (\textrm {AI})]$, dashed line $Re_G=-8500$; (b) $Re_G=[-6234, -8145, -8490, -15\,000]$; (c) $Re_G=[-8145, -15\,000, -20\,430 \ (\textrm {AI\ limit})]$, dashed line $Re_G=-20\,440$; (d) $Re_G=[-8145, -15\,000, -20\,430, -35\,000]$. We have rescaled $\omega$ with $\mathcal {T}_\nu =2.207\times 10^{-3}$ s (see (3.34a–c)).

Figure 5

Table 1.Fluid combinations used in our computations. The Kapitza number is defined as $Ka=\sigma/(\rho_L g^{1/3} \nu_L^{4/3})$, where $\sigma$, $\rho _L$ and $\nu _L$ denote the surface tension, density and kinematic viscosity of the liquid, and $g$ designates the gravitational acceleration.

Figure 6

Figure 6.Temporal stability predictions from the OS-OS (solid curves) and WRIBL-OS (open symbols) approaches. Parameters similar to those in figure 5(a): $Ka=3174$, $H^\star =19$ mm, $\phi =5^\circ$, $Re_L=32.7$. Circles indicate passive-gas limit ($\varPi _\rho =\varPi _\mu =0$ in (3.41)); pentagons indicate $Re_G=-4123$; squares indicate ${Re_G=-6173}$; diamonds indicate $Re_G=-8220$. (a) Growth rate; (b) wave speed.

Figure 7

Figure 7.Spatial linear stability predictions obtained from WRIBL-LW (symbols) and WRIBL-OS (lines) calculations. Inclined falling liquid film sheared by a co-current gas based on parameters in Samanta (2014): $Ka=963$ (glycerol–water and air II in table 1), $\phi =4^\circ$, $H^\star =15$ mm, $Re_G=2000$. S/U indicate stable/unstable regions. Circles indicate full formulation; squares indicate $\varPi _\rho =0$ in (3.41); diamonds indicate $T_{G}=T_{{G}0}$, $\varPi _\rho =0$; crosses indicate $\varPi _{\mu }=\varPi _\rho =0$. (a) Wave speed $c_r=\omega /k_r$ around the long-wave limit $k_r\to 0$; (b) neutral stability bound, $k_i=0$.

Figure 8

Figure 8.Spatial linear stability predictions from (a,c) WRIBL-LW and (b,d) WRIBL-OS approaches. Parameters according to experiments of Kofman (2014): $Ka=3174$ (water and air I in table 1), $H^\star =19$ mm, $\phi =5^\circ$, $Re_L=32.7$. Open circles indicate passive-gas limit, $\varPi _\rho =\varPi _\mu =0$ in (3.41). Values of $|Re_G|$ increase in the order diamonds, squares, crosses/asterisks, pentagons, pluses. (a,b) Full model; (c,d) $\varPi _\rho =0$ in (3.41). Here: (a) $Re_G=[-4123,-6713,-9157]$; (b) $Re_G=[-4123,-6713,-8220]$; (c) $Re_G=[-6713,-9100,-11\,000,-15\,000]$; (d) $Re_G=[-6713,-9100,-11\,000,-15\,000]$. Red dot-dashed curves track growth rate maximum $\{-k_i\}_{max}$. We have rescaled $\omega$ with $\mathcal {T}_\nu =2.207\times 10^{-3}$ s (see (3.34a–c)).

Figure 9

Figure 9.Nonlinear computations (solid and dashed lines) with our WRIBL-LW model (3.6) versus experiments (symbols) of Kofman (2014): $Ka=3174$ (water and air I in table 1), $H^\star =19$ mm, $\phi =5^\circ$, $Re_L=32.7$, $f_0^\star =2.8$ Hz ($\omega _0^\star \mathcal {T}_\nu =0.039$). Film thickness time traces at fixed streamwise position. Solid green lines indicate TWS from numerical continuation; dashed black lines indicate open-domain computations with coherent inlet forcing ($\varepsilon _1=0.01$, $\varepsilon _2=0$). (a) Quiescent gas ($\varPi _\rho =\varPi _\mu =0$ in computations);(b) $Re_G=-4123$; (c) $Re_G=-6713$.

Figure 10

Figure 10.Top view snapshots from one of our experiments. Falling water film sheared by a counter-current air flow and subject to coherent inlet forcing: $H^\star =13$ mm, $\phi =5^\circ$, $Re_L^{as}=44.7$, $Re_L=43.1$, $f_0^\star =3.0$ Hz. The first snapshot indicates aerostatic configuration; the second snapshot and onwards indicate counter-current turbulent gas flow with increasing $|Re_G|$. Absolute instability limit from linear stability calculation in figure 12: $Re_G^{AI}=-5182$.

Figure 11

Figure 11.Gas effect on threshold of long-wave Kapitza instability. Linear stability predictions for a falling liquid film sheared by a counter-current gas flow: $Ka=3174$ (water and air I in table 1), $H^\star =13$ mm.(a) Neutral stability bounds. Black curves with circles indicate $\phi =5^\circ$; red curves with diamonds indicate $\phi =1^\circ$. Curves with filled symbols indicate WRIBL-LW/WRIBL-OS prediction for turbulent gas flow; curves with open symbols indicate fully coupled prediction for laminar gas flow (Tilley et al.1994); dot-dashed magenta curve indicates short-wave instability mode (§ 6.2) at $\phi =1^{\circ }$; shaded zone indicates turbulence transition, $Re_G \in [-1800, -1300]$. S/U denote stable/unstable regions. (b) Spatial growth rate dispersion curves from WRIBL-OS: $\phi =1^\circ$, $Re_L=1.5\ (5/6)\cot (\phi )$. Pentagons indicate $\varPi _\rho =\varPi _\mu =0$ in (3.41); squares to pluses indicate $Re_G=-1000, -2000, -3000, -3600$.

Figure 12

Figure 12.Transition to AI predicted by spatial linear stability analysis with our WRIBL-OS approach. Parameters according to experiment in figure 10: $Ka=3174$ (water and air I in table 1), $H^\star =13$ mm, $\phi =5^\circ$, $Re_L=43.1$. Circles indicate $\varPi _\rho =\varPi _\mu =0$ in (3.41); diamonds indicate $Re_G=-4000$; crosses indicate $Re_G=-5181$. (a) Growth rate $-k_i$ versus $\omega$. Inset shows $-k_i$ versus $k_r$. Dot-dashed line indicates $Re_G=-5180$; dot-dot-dashed line indicates $Re_G=Re_G^{AI}=-5182$. (b) Wave speed $c_r=\omega /k_r$. Vertical dashed line indicates forcing frequency $f_0^\star =3$ Hz from figure 10. We have rescaled $\omega$ with $\mathcal {T}_\nu =2.207\times 10^{-3}$ s (see (3.34a–c)).

Figure 13

Figure 13.Gas effect on nonlinear TWS obtained with our WRIBL-LW model (curves) versus experiments (empty symbols). Inclined falling liquid film sheared by counter-current turbulent gas flow: $Ka=3174$ (water and air I in table 1), $\phi =5^\circ$. Filled/open symbols distinguish number of capillary ripples (CR): diamonds indicate 0-CR; squares indicate 1-CR; triangles indicate 2-CR; circles indicate3-CR; dashed line indicates >3-CR. Solid curves indicate $f^\star =f_0^\star$; dot-dashed curves indicate $f^\star =f^\star _{max}$. Crosses indicate AI limit; asterisks indicate nonlinear limit points. Open/filled red arrows mark AI limits obtained from WRIBL-LW/WRIBL-OS. (a,c) Wave height; (b,d) wave speed scaled with $\hat {u}_{Nu}^\star =(3/2)q_{L 0}^\star /h_{Nu}^\star$, where $h_{Nu}^\star =(3q_{L0}^\star\nu_L/(g\sin(\phi)))^{1/3}$. (a,b) Versus our experiments: $H^\star =13$ mm, $f_0^\star =3.0$ Hz, with (a) $Re_L=44.2\pm 0.3$, (b) $Re_L=43.1$. Filled arrow indicates $Re_G^{AI}=-5194$; empty arrow indicates $Re_G^{AI}=-5366$. (c,d) Versus experiments of Kofman et al. (2017): $H^\star =19$ mm, $Re_L=45$, $f_0^\star =3.05$ Hz. Filled arrow indicates $Re_G^{AI}=-8490$; empty arrow indicates $Re_G^{AI}=-9633$.

Figure 14

Figure 14.Gas effect on streamwise evolution of the wavy liquid film. Compilation of our experiments: water/air, $H^\star =13$ mm, $\phi =5^\circ$, $Re_L^{as}=46$, $Re_L=44.2\pm 0.3$, $f_0^\star =3$ Hz, $Re_G^{AI}=-5194$.(a) Ensemble-averaged wave height $h_{max}^\star$. Error bars represent standard deviation, and check marks mark the start of the coalescence-dominated region. Filled symbols mark data points used in figure 13(a). Circles indicate aerostatic configuration; diamonds indicate $Re_G=-3040$; squares indicate $Re_G=-4190$; pentagons indicate $Re_G=-5200$; triangles indicate $Re_G=-5750$. (b) Frequency spectra of the film height $h^\star$, with $Re_G=-5750$, where $|\hat {h}^\star _i|$ denotes the amplitude of the Fourier mode with $f_i^\star$. Crosses mark primary and secondary peaks. Left, $x^\star =41.5$ cm; middle, $x^\star =51.5$ cm; right, $x^\star =58.5$ cm.

Figure 15

Figure 15.Wave coalescence event. Top-view snapshots from our experiment in figure 10 (parameters similar to pentagons in figure 14a): $Re_L=43.1$, $Re_G=-5200$. Time increases from top left to bottom right with increment 0.48 s. Solid red and dashed yellow lines highlight two consecutive wave fronts.

Figure 16

Figure 16.Wave trains for two data sets from figure 14(a). (a) Film thickness time traces at $x^\star =82.5$ cm. Solid line indicates aerostatic configuration (circles in figure 14a), $Re_L^{as}=46.0$; dashed line indicates counter-current configuration (triangles in figure 14a), $Re_L=44.2$, $Re_G=-5750$. (b,c) Corresponding frequency spectra, where $|\hat {h}^\star _i|$ is the amplitude of the Fourier mode with $f_i^\star$. (b) Aerostatic configuration; open circles mark peaks at $f_0^\star$ and its harmonics. (c) Counter-current configuration; open circle marks global peak at most-amplified frequency $f_{max}^\star /f_0^\star =0.49$.

Figure 17

Figure 17.Gas effect on the starting position $x_c^\star$ of the coalescence-dominated region. Compilation of our experiments: water/air, $H^\star =13$ mm, $\phi =5^\circ$, $f_0^\star =3$ Hz. Circles indicate $Re_L=32.5\pm 0.6$; squares indicate $Re_L=44.3\pm 0.3$; curves indicate polynomial fits to guide the eye.

Figure 18

Figure 18.Gas effect on spatial evolution of naturally-evolving Kapitza waves. Open-domain computations using our WRIBL-LW model on a domain of length $L^\star =1.50$ m. The gas flow is applied over the entire domain length. Noisy inlet perturbation according to (3.46): $\varepsilon _1=0$, $\varepsilon _2=5\times 10^{-5}$. Parameters according to experiments in figure 14(a) (circles, squares and triangles there): $Ka=3174$ (water and air I in table 1), $H^\star =13$ mm, $\phi =5^\circ$, $Re_L=43.1$. Plots for: (a) $\varPi _\rho =\varPi _\mu =0$ in (3.6a); (b) $Re_G=-4190$; (c) $Re_G=-5750$. The AI limits, obtained from WRIBL-LW and WRIBL-OS, are $Re_G^{AI}=-5347$ and $Re_G^{AI}=-5182$.

Figure 19

Figure 19.Spatio-temporal diagrams of the normalized film height $h/h_{max}$ for the computations in figures 18(b) and 18(c): (a) $Re_G=-4190$, (b) $Re_G=-5750$. The AI frequency is ${f_{AI}^\star =3.35}$ Hz, as obtained from linear stability analysis based on our WRIBL-LW model.

Figure 20

Figure 20.Computations according to figures 18(a) and 18(b), but with additional coherent inlet forcing (3.46): $f_0^\star =3$ Hz, $\varepsilon _1=0.01$, $\varepsilon _2=5\times 10^{-5}$. Plots for: (a) $\varPi _\rho =\varPi _\mu =0$ in (3.6a); (b) $Re_G=-4190$.

Figure 21

Figure 21.Summary of wave data from our computations in figures 18 and 20. Maximum wave height $h_{max}$ versus the streamwise location. Circles indicate $\varPi _\rho =\varPi _\mu =0$; crosses indicate $Re_G=-4190$; diamonds indicate $Re_G=-5750$. Naturally evolving versus forced waves. (a) Noisy inlet perturbation: $\varepsilon _1=0$, ${\varepsilon _2=5\times 10^{-5}}$ in (3.46). (b) Additional coherent inlet forcing: $f_0^\star =3.0$ Hz, $\varepsilon _1=0.01$, $\varepsilon _2=5\times 10^{-5}$ in (3.46).

Figure 22

Figure 22.Vertically falling liquid film sheared by a turbulent counter-current gas flow. Liquid-side conditions according to figure 3(a) in Lavalle et al. (2020): $Ka=509.46$ (DMSO–water and air II in table 1), $Re_L=15$, $f_0^\star =16$ Hz, $Re_G^{AI}=-6500$. WRIBL computation on an open domain of length $L^\star =0.843$ m. Snapshots of the film height profile $h(x)$ at $f_0 t=61.4$. (a) At AI limit: $Re_G=Re_G^{AI}=-6500$. (b) Beyond AI limit: ${Re_G=-7500}$. Dot-dashed red line indicates $f_0 t=61.6$; green dashed line indicates Lagrangian path of a wave crest.

Figure 23

Figure 23.Standing ripples beyond the AI limit $Re_G^{AI}=-6500$. Computation from figure 22(b): ${Re_G=-7500}$. (a) Spatio-temporal diagram of the normalized film height $h/h_{max}$. (b) Film height time trace $h(t)$ at $x/L=0.6$. (c) Spatial profile of the liquid flow rate $q_L(x)$ at $f_0 t=61.4$.

Figure 24

Figure 24.New short-wave instability mode. Falling liquid film sheared by a turbulent counter-current gas flow: $Ka=3174$ (water and air I in table 1), $H^\star =13$ mm, $\phi =5^\circ$, $Re_L=43.1$, $Re_G^{AI}=-5182$. Temporal linear stability predictions using the OS-OS approach. Dashed blue indicates new short-wave mode; dot-dashed red indicates long-wave Kapitza mode; solid black with filled symbols indicates unstable merged mode; solid green with open symbols indicates stable merged mode. Pluses indicate $\varPi _\rho =\varPi _\mu =0$ in (3.41); crosses indicate $Re_G=-4700$; pentagons indicate $Re_G=-5200$; diamonds indicate $Re_G=-5750$; squares indicate ${Re_G=-6400}$; circles indicate $Re_G=-6760$. (a,c) Growth rate; (b,d) wave speed. Shaded magenta bands and filled magenta circles with error bars represent our experiment from figure 10: $Re_L=43.1$, $Re_G=-6760$, $\varLambda _{ripples}^\star =(13\pm 3)$ mm, $c_{ripples}^\star =(-6.2\pm 1.5)$ cm s$^{-1}$.

Figure 25

Figure 25.First signature of upward-travelling ripples in our experiments. Spatio-temporal diagrams of the film surface slope $\|\boldsymbol {\nabla } h\|$ for parameters in figure 10, obtained with the synthetic schlieren technique (Kofman et al.2014): $H^\star =13$ mm, $\phi =5^{\circ }$, $Re_L=43.1$, $f_0^\star =3$ Hz, $x^\star _0=48$ cm, $z^\star =13$ cm. (a) For $Re_G=-5200$, ripples start to appear in between Kapitza wave humps. (b) For $Re_G=-6080$, ripples deform crests of Kapitza waves.

Figure 26

Figure 26.Details of OS-OS linear stability predictions from figure 24: $Ka=3174$, $Re_L=43.1$, $H^\star =13$ mm, $\phi =5^\circ$. (a) Merging between the short-wave and long-wave instability modes from figures 24(a) and 24(c). Diamonds indicate $Re_G=-5750$; lines without symbols indicate $Re_G=-5680$, pentagons indicate $Re_G=-5200$. (b) Primary-flow liquid velocity at the film surface. Solid line indicates $H^\star =13$ mm, ${Re_{G}^{AI}=-5182}$; dot-dashed line indicates $H^\star =19$ mm, $Re_{G}^{AI}=-8461$; dashed line indicates $H^\star =5$ mm, $Re_{G}^{AI}=-1501$. Asterisks indicate the AI limit from WRIBL-OS spatial linear stability calculations.

Figure 27

Figure 27.Eigenfunctions (4.13a,b) for different instability modes from figure 24. Turbulent counter-current gas flow: $Re_G=-5200$. Linearly most-amplified short-wave (dashed blue lines, $k=12.8$) and long-wave (solid red lines, $k=1.6$) instability modes. (a) Liquid film, $\phi$; (b) gas layer, $\psi$.

Figure 28

Figure 28.Validation of our WRIBL-OS approach (§ 4.1). Spatial linear stability predictions for parameters in figure 15 of Vellingiri et al. (2015): $Ka=2000$ (methanol and helium in table 1), $\phi =90^{\circ }$, $\underline {Re}_0=3Re_L/\sin (\phi )=10$, $H^\star =30$ mm, $\varPi _\rho =0$, (3.6a) truncated at ${O}(\epsilon )$. Quantities are scaled with $\underline {\mathcal {L}}=h_0^\star$ and $\underline {\mathcal {U}}=h_0^{\star 2}g\sin(\phi)/(2\nu_L)$. The counter-current gas shear stress is quantified via $\varTheta =\left|T^\star_{G 0}\right|\!/(\mu_L \underline{\mathcal{U}}/\underline{\mathcal{L}})$.

Figure 29

Figure 29.Validation of our WRIBL-OS (§ 4.1) and OS-OS (§ 4.2) approaches. Temporal linear stability predictions for a gas-sheared vertically falling liquid film. (a) Neutral stability curves for parameters according to figure 11 in Vellingiri et al. (2015): $Ka=2000$, $H^\star =300$ mm. Crosses indicate OS-OS; solid lines indicate WRIBL-OS; open circles indicate data from Vellingiri et al. (2015). Thin solid line, $\varTheta =0$; dashed line, $\varTheta =1$; dot-dashed line, $\varTheta =2$; dot-dot-dashed line, $\varTheta =3$; thick solid line, $\varTheta =3.5$. Same scaling as in figure 28. (b) Growth rate dispersion curves for parameters according to figure 4(e) in Schmidt et al. (2016): $H^\star =10$ mm, $\rho _{L}=1000$ kg m$^{-3}$, $\mu _{L}=0.5\times 10^{-3}$ Pa s, $\rho _{G}=1$ kg m$^{-3}$, $\mu _{G}=1\times 10^{-6}$ Pa s, $\sigma =1$ mN m$^{-1}$, $\delta _{L}=h_0^\star /H^\star =0.08$, $\widetilde {Fr}=\tilde {\mathcal {U}}/\sqrt {g\tilde {\mathcal {L}}}=3$, $Re_{L}=6166$, $Re_{G}=48\,322$. Tildes indicate scaling with $\tilde {\mathcal {L}}=H^\star$ and $\tilde {\mathcal {U}}=[\partial _{x^\star }P_{G 0}^\star H^\star /\rho _G]^{1/2}$. Solid blue line indicates long-wave Kapitza mode; dashed red line indicates short-wave Tollmien–Schlichting mode.

Figure 30

Figure 30.Accounting for temporal and spatial derivatives of $T_G$ and $P_G$ in (3.6a). Temporal linear stability predictions based on three approaches for conditions according to figure 24: $Ka=3174$ (water and air I in table 1), $H^\star =13$ mm, $\phi =5^{\circ }$, $Re_{L}=43.1$. Dot-dashed lines indicate WRIBL-OS (3.41); solid lines indicate OS-OS (4.20) and (4.21); dashed lines indicate WRIBL-OS, including derivatives of $T_G$ and $P_G$ in (3.6a). (a) Here, $Re_{G}=-4700$. Red lines indicate long-wave Kapitza mode, blue lines indicate short-wave mode.(b) Here, $Re_{G}=-6760$, merged mode.

Ishimura et al. Supplementary Movie 1

Gas-induced wave coalescence on a weakly-inclined falling liquid film subject to a counter-current turbulent gas flow. Parameters according to panel 18b: below the absolute instability limit.

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Ishimura et al. Supplementary Movie 2

Regular wave train produced by absolute instability (AI) on a weakly-inclined falling liquid film subject to a counter-current turbulent gas flow. Parameters according to panel 18c: beyond the AI limit.

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Ishimura et al. Supplementary Movie 3

Standing ripples generated by absolute instability on a vertically falling liquid film subject to an increasingly strong counter-current turbulent gas flow. Parameters according to figure 23.

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