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The role of viscoplastic drop shape in impact

Published online by Cambridge University Press:  27 December 2023

Kindness Isukwem
Affiliation:
Mines Paris, PSL University, Centre for material forming (CEMEF), UMR CNRS 7635, rue Claude Daunesse, 06904 Sophia-Antipolis, France
Julie Godefroid
Affiliation:
Sciences et Ingénierie de la Matière Molle, ESPCI Paris, PSL Research University, UMR CNRS 7615, Sorbonne Université, Paris, France
Cécile Monteux
Affiliation:
Sciences et Ingénierie de la Matière Molle, ESPCI Paris, PSL Research University, UMR CNRS 7615, Sorbonne Université, Paris, France
David Bouttes
Affiliation:
Saint-Gobain CREE, 550 rue Alphonse Jauffret, Cavaillon 84300, France
Romain Castellani
Affiliation:
Mines Paris, PSL University, Centre for material forming (CEMEF), UMR CNRS 7635, rue Claude Daunesse, 06904 Sophia-Antipolis, France
Elie Hachem
Affiliation:
Mines Paris, PSL University, Centre for material forming (CEMEF), UMR CNRS 7635, rue Claude Daunesse, 06904 Sophia-Antipolis, France
Rudy Valette
Affiliation:
Mines Paris, PSL University, Centre for material forming (CEMEF), UMR CNRS 7635, rue Claude Daunesse, 06904 Sophia-Antipolis, France
Anselmo Pereira*
Affiliation:
Mines Paris, PSL University, Centre for material forming (CEMEF), UMR CNRS 7635, rue Claude Daunesse, 06904 Sophia-Antipolis, France
*
†Email address for correspondence: anselmo.soeiro_pereira@mines-paristech.fr

Abstract

The impact of fluid drops on solid substrates is a cardinal fluid dynamics phenomenon intrinsically related to many fields. Although these impacting objects are very often non-spherical and non-Newtonian, previous studies have mainly focused on spherical Newtonian drops. As a result, both shape and rheological effects on the drop-spreading dynamics remain largely unexplored. In the present work we use a mixed approach combining experiments with multiphase three-dimensional numerical simulations to extend the work reported by Luu & Forterre (J. Fluid Mech., vol. 632, 2009, pp. 301–327) by highlighting the fundamental role of shape in the normal impact of viscoplastic drops. Such complex fluids are highly common in various industrial domains and ideally behave either like a rigid body or a shear-rate-dependent liquid, according to the stress solicitation. Spherical, prolate, cylindrical and prismatic drops are considered. The results show that, under negligible capillary effects, the impacting kinetic energy of the drop is dissipated through viscoplastic effects during the spreading process, giving rise to three flow regimes: (i) inertio-viscous, (ii) inertio-plastic, and (iii) mixed inertio-visco-plastic. These regimes are deeply affected by the drop initial aspect ratio, which in turn reveals the possibility of using drop shape to control spreading. The physical mechanisms driving the considered phenomenon are underlined by energy budget analyses and scaling laws. The results are summarised in a two-dimensional diagram linking the drop maximum spreading, minimum height and final shape with different spreading regimes through a single dimensionless parameter, here called the impact number.

Information

Type
JFM Papers
Copyright
© The Author(s), 2023. Published by Cambridge University Press
Figure 0

Figure 1. Experimental snapshots showing the spreading evolution of a water drop (a) and bentonite-in-water drops at three particle mass fractions $\phi$ (b–d). The yield stress $\tau _0$ increases with $\phi$: (a) $\phi =0$, $\tau _0 = 0$ Pa; (b) $\phi =0.5$, $\tau _0 = 5$ Pa; (c) $\phi =0.55$, $\tau _0 = 50$ Pa; and (d) $\phi =0.6$, $\tau _0 = 500$ Pa. The impact velocity is $U_0 = 1.25\ {\rm m}\ {\rm s}^{-1}$. The diameter of the drops is $D_0 = 5$ mm, and the height of the prolate ones is $H_0 = 12.5$ mm. The interval $\Delta t$ between two images is 1.9 ms.

Figure 1

Figure 2. Experimental snapshots illustrating the spreading time evolution of three bentonite-in-water drops impacting a hydrophilic acrylic plate at ${{Re}_{m,D}} = 47$ and ${Pl} = 0.18$. The dimensionless interval $\Delta t^{\ast } = t/t_{max}$ between two images is 0.1428 ($t_{max}$ being the instant at which the drop achieves its maximum spreading $D_{max}$). Clearly, regardless of the volume of the drop $V_{total}$, $D_{max}/D_0$ is an increasing function of $H_0/D_0$: (a) $V_{total} = 1.64 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.24$; (b) $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.24$; (c) $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 1.91$.

Figure 2

Figure 3. Experimental snapshots showing the spreading evolution of two prolate mayonnaise drops impacting an acrylic plate at ${{Re}_{m,H}} = 18.6$ and ${Pl} = 0.126$. The dimensionless interval $\Delta t^{\ast } = t/t_{max}$ between two images is 0.3334 for the upper-line case, and 0.1667 ms for the bottom-line case. As observed, different initial aspect ratios induce distinct maximum relative spreading: (a) $H_0/D_0 = 3$, $D_{max}/D_0 = 2$; (b) $H_0/D_0 = 8$, ${D_{max}/D_0 = 2.6}$.

Figure 3

Figure 4. (a) Experimental set-up for the investigation of the role of viscoplastic drop shape in impact. The viscoplastic drop of height $H_0$ and diameter $D_0$ falls by gravity $\boldsymbol {g}$ from a nozzle and hits the solid acrylic plate at the instant $t_0$ at an impact velocity $U_0$ ($U_0$ being a function of the distance between the nozzle and the plate $H$; $U_0 \propto \sqrt {H}$). (b) After the impact, the drop spreads radially until it achieves a maximum diameter $D_{max}$ and a minimum height $H_{min}$ at the instant $t_{max}$. A ketchup drop is used for the illustrated impact event ($U_0 = 1.25\ {\rm m}\ {\rm s}^{-1}$, $D_0 = 5$ mm, $H_0 = 7.5$ mm, $\rho = 1250\ {\rm kg}\ {\rm m}^{-3}$, $k = 10\ {\rm Pa}\ {\rm s}^{m}$, $m = 0.5$, $\tau _0 = 12$ Pa and $D_{max}/D_0 = 1.82$). It is recorded by a high-speed camera ($ O ( 10^{4} )$ frames per second) with the aid of a LED backlight panel. A movie showing the mentioned impact event is available as a supplemental material at https://doi.org/10.1017/jfm.2023.926 (see supplementary movie 1).

Figure 4

Table 1. Details concerning the considered fluids for the experiments: ${\rm A} = \text {sodium}$ alginate in 40 % by weight zirconia-in-deionized-water solutions; ${\rm C} = \text {Carbopol}$-based microgels; $\text {B-W} = 5\ \mathrm {\mu }{\rm m}$ bentonite particles in deionized water; $\text {B-G-W} = 5\ \mathrm {\mu }{\rm m}$ bentonite particles in 50 % by weight glycerol-in-deionized-water solution; $\text {K-W} = 5\ \mathrm {\mu }{\rm m}$ kaolin particles in deionized water; ${\rm M} = {\rm Amora}$, Bénédicta and Hellmann's mayonnaises; ${\rm K} = {\rm Amora}$, Nature and Heinz ketchups. Impact velocities $U_0$ vary from $1\ {\rm m}\ {\rm s}^{-1}$ to $4\ {\rm m}\ {\rm s}^{-1}$.

Figure 5

Figure 5. Rheological characterisation using an ARES-G2 rheometer (TA Instruments) equipped with a cone-plate geometry. We employ standard ramp shear tests over a range of $10^{-3}\ {\rm s}^{-1}$ to $10^3\ {\rm s}^{-1}$ to obtain stress versus deformation rate levels (a) in addition to oscillatory tests at $10\ {\rm rad}\ {\rm s}^{-1}$ to obtain the storage modulus of the used fluids (b).

Figure 6

Figure 6. Four different drop initial shapes are numerically considered: (a) spherical, (b) prolate,(c) cylindrical and (d) prismatic. Their initial aspect ratio $H_0/D_0$ varies from 1 to 8. (e) Numerical configuration taken into account. The used mesh (composed of approximately $10^6$ elements) adapted around each interface (viscoplastic drop in red, and air in blue) and illustrated by the black lines. The drop of height $H_0$ and diameter $D_0$ falls by gravity and hits the solid plate at the instant $t_0$ at an impact velocity $U_0$. After the impact, the drop spreads until it achieves a maximum diameter $D_{max}$ and a minimum height $H_{min}$ at the instant $t_{max}$. A movie showing a typical numerical simulation is available as a supplemental material (see supplementary movie 2; $U_0 = 1.5\ {\rm m}\ {\rm s}^{-1}$, $D_0 = 3.15$ mm, $H_0 = 12.6$ mm, $\rho = 1585\ {\rm kg}\ {\rm m}^{-3}$, $k = 0.1\ {\rm Pa}\ {\rm s}^m$, $m = 1$, $\tau _0 = 948$ Pa).

Figure 7

Table 2. Details concerning the considered drops for the numerical simulations. Impact velocities $U_0$ vary from $0.5\ {\rm m}\ {\rm s}^{-1}$ to $10\ {\rm m}\ {\rm s}^{-1}$.

Figure 8

Figure 7. Six numerical snapshots of the spreading process for eight viscoplastic drops at two ${{Re}_{m,D}}-{Pl}$ couples: ${{Re}_{m,D}} = 50$ and ${Pl} = 0.6$ (figure 7a–d; left column); ${{Re}_{m,D}} = 150$ and ${Pl} = 0.07$ (figure 7e–h; right column). The interval $\Delta t$ between two subsequent images corresponds to 20 % of the necessary time to achieve the maximum spreading $t_{max}$ ($\Delta t^{\ast } = \Delta t / t_{max} = 0.2$). The drop volumes, their aspect ratio and their maximum relative spreading are respectively: (a) $V_{total} = 1.64 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.12$; (b) $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.12$; (c) $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 1.31$; (d) $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 1.31$; (e) $V_{total} = 1.64 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.8$; ( f) $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.8$; (g) $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 2.58$; (h) $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 2.58$. The red surface in both the first and the last snapshot indicates the 3-D drop–air interface. Contours of the norm of the instantaneous velocity $| u(x, y, z, t) |$ (made dimensionless by the maximum instantaneous velocity $| u_{max}(t) |$) on the centre $x$–$z$ plane are represented on the left side of the second through fifth snapshot of each displayed case. Yielded (flowing; $| \boldsymbol {\tau } | > \tau _0$; black) and unyielded (non-flowing; $| \boldsymbol {\tau } | \leq \tau _0$; grey) regions are illustrated on their right side.

Figure 9

Figure 8. Six numerical snaphots obtained at ${{Re}_{m,H}} = 150$ and ${Pl} = 0.07$ illustrate the spreading evolution of spherical and prolate drops: (a) $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$, $H_0/D_0 = 1$, $D_{max}/D_0 = 1.8$; (b) $V_{total} =1.64\ \times$ $ 10^{-8}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 2.37$; (c) $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$, $H_0/D_0 = 4$, $D_{max}/D_0 = 2.37$. The red surface in both the first and the last snapshot indicates the 3-D drop–air interface. Contours of the norm of the instantaneous velocity $| u(x, y, z, t) |$ (made dimensionless by the maximum instantaneous velocity $| u_{max}(t) |$) on the centre $x$–$z$ plane are represented on the left side of the second through fifth snapshot of each displayed case. Yielded (flowing; black) and unyielded (non-flowing; grey) regions are illustrated on their right side.

Figure 10

Figure 9. Instantaneous volume fraction of unyielded regions $V_{unyielded}/V_{total}\times 100[\%]$ plotted as a function of dimensionless time $t/t_{max}$ for spherical (open symbols) and prolate numerical objects ($H_0/D_0 = 4$; solid symbols). For each subfigure, both the Reynolds number and the plastic number are kept fixed: (a) ${{Re}_{m,D}} = 50$ and ${Pl} = 0.6$, (b) ${{Re}_{m,D}} = 150$ and ${Pl} = 0.07$, and (c) ${{Re}_{m,H}} = 150$ and ${Pl} = 0.07$. Each symbol form indicates a specific drop volume $V_{total}$: $V_{total} = 1.64 \times 10^{-8}\ {\rm m}^3$ (circles); $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$ (triangles); $V_{total} = 1.64 \times 10^{-7}\ {\rm m}^3$ (diamonds). Inset plots stressing the minimum $V_{unyielded}/V_{total}$ are also provided.

Figure 11

Figure 10. Instantaneous relative diameter $D(t)/D_0$ as a function of dimensionless time $t/t_{max}$ for spherical (a) and prolate numerical drops at $H_0/D_0 = 4$ (b) and $H_0/D_0 = 8$ (c). Their volume is fixed at $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$. In each subfigure, three ${{Re}_{m,D}}-{Pl}$ couples are explored: ${{Re}_{m,D}} = 80$ and ${Pl} = 0.002$ (grey circles), ${{Re}_{m,D}} = 80$ and ${Pl} = 0.03$ (blue triangles), and ${{Re}_{m,D}} = 80$ and ${Pl} = 0.7$ (red diamonds).

Figure 12

Figure 11. Energy percentage curves plotted as a function of dimensionless time $t/t_{max}$: kinetic energy (blue triangles), surface energy (grey circles), gravitational energy (green squares) and dissipation (red diamonds). The latter is divided into two parts: viscous dissipation (orange triangles) and plastic dissipation (black asterisks). The computed terms are made dimensionless by the total energy of the system and generically represented by variable $\varepsilon ^{*}$. Aspect ratio effects on the spreading dynamics are pointed out with the aid of four different numerical drops: $H_0/D_0 = 1$ and $V_{total} = 6.54 \times 10^{-8}\ {\rm m}^3$ (first line); $H_0/D_0 = 1$ and $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$ (second line); $H_0/D_0 = 4$ and $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$ (third line); and $H_0/D_0 = 4$ and $V_{total} = 6.54 \times 10^{-8} {\rm m}^3$ (fourth line). For each of them, three ${{Re}_{m,D}}-{Pl}$ couples are considered: ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.002$ (a,d,g,j); ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.05$ (b,e,h,k); and ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.5$ (c, f,i,l).

Figure 13

Figure 12. Spherical numerical drops ($H_0/D_0 = 1$) with the same volume $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$. Each subfigure is related to a specific ${{Re}_{m,D}}-{Pl}$ couple: (a) ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.002$; (b) ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.05$; (c) ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.5$. They are composed of six upper-line snapshots and six bottom-line snapshots ($\Delta t^{\ast } = t/t_{max} = 0.2$). The first one shows the 3-D drop–air interface in red. From the second to the last upper-line snapshot, $| \boldsymbol {{\dot {\gamma }}} |/(U_0/H_0)$ contours are displayed on the left side of the centre $x$–$z$ plane, while yielded (black) and unyielded (grey) regions are shown on the right side. Additionally, from the second to the last bottom-line snapshot, the dissipative process is stressed by $k {|\boldsymbol {{\dot {\gamma }}}|}^{m+1}/(\rho U_0^3/H_0)$ and $\tau _0 {|\boldsymbol {{\dot {\gamma }}}|}/(\rho U_0^3/H_0)$ contours on the left and right side of the centre $x$–$z$ plane, respectively.

Figure 14

Figure 13. Prolate numerical drops ($H_0/D_0 = 4$) with the same volume $V_{total} = 2.62 \times 10^{-7}\ {\rm m}^3$. Subfigures are related to specific ${{Re}_{m,D}}-{Pl}$ couples: (a) ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.002$; (b) ${{Re}_{m,D}} = 112.5$ and ${Pl= 0.05}$; (c) ${{Re}_{m,D}} = 112.5$ and ${Pl} = 0.5$. They are composed of six upper-line snapshots and six bottom-line snapshots ($\Delta t^{\ast } = t/t_{max} = 0.2$). The first snapshot shows the 3-D drop–air interface in red. From the second to the last upper-line snapshot, $| \boldsymbol {{\dot {\gamma }}} |/(U_0/H_0)$ contours are displayed on the left side of the centre $x$–$z$ plane, while yielded (black) and unyielded (grey) regions are shown on the right side. Additionally, from the second to the last bottom-line snapshot, the dissipative process is stressed by $k {|\boldsymbol {{\dot {\gamma }}}|}^{m+1}/(\rho U_0^3/H_0)$ and $\tau _0 {|\boldsymbol {{\dot {\gamma }}}|}/(\rho U_0^3/H_0)$ contours on the left and right side of the centre $x$–$z$ plane, respectively.

Figure 15

Figure 14. (a) Rescaled maximum spreading plotted using the scaling laws and the impact number definition given by Luu & Forterre (2009): $(D_{max}/D_0) / [ {{Re}_{m,D}} ]^{1/{2m+3}}$ against $(1/{Pl})^{1/3} (1/{{Re}_{m,D}})^{1/{2m+3}}$. (b) Rescaled maximum spreading plotted using the scaling laws and the impact number definition taking the drop aspect ratio into account (present work): $(D_{max}/D_0) / [ {{Re}_{m,D}} (H_0/D_0)^{m+1} ]^{1/{2m+3}}$ against $(1/{Pl})^{1/3} (1/{{Re}_{m,D}})^{1/{2m+3}} (H_0/D_0)^{-m/{6m+9}}$. The symbols denote aspect ratio values (for the numerical simulations) or intervals (for the experiments; asterisks). (c) Rescaled minimum height as a function of the impact number (only numerical results related to prolate drops are plotted, for clarity). (d) Comparisons between the spreading time $t_{max}$ obtained from numerical simulations using prolate drops, and the one predicted by combining (3.4) and (3.2).

Figure 16

Figure 15. Three-step deformation rate rheological tests: 57 % bentonite (a), 3 % Carbopol (b), ‘Nature’ ketchup (c) and ‘Amora’ mayonnaise (d). These tests were carried out using an ARES-G2 rheometer (TA Instruments) equipped with a cone-plate geometry. At each step, the shear viscosity is plotted as a function of time (over 60 s) at a specific deformation rate: $0.1\ {\rm s}^{-1}$ at steps 1 and 3; and $100\ {\rm s}^{-1}$ at step 2. The black arrows indicate the recovery process.

Supplementary material: File

Isukwem et al. supplementary movie 1

a typical experiment showing a ketchup prolate drop impacting an acrylic plate (U0 = 1.25m/s, D0 = 5mm, H0 = 7.5mm, ρ = 1250kg/m3, k = 10Pa.sm, m = 0.5, τ0 = 12Pa, and Dmax/D0 = 1.82). It is recorded by a high-speed camera [𝒪(104) frames per second] with the aid of a LED backlight panel.
Download Isukwem et al. supplementary movie 1(File)
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Supplementary material: File

Isukwem et al. supplementary movie 2

a typical numerical simulation illustrating the impact of a prolate drop on a solid (U0 = 1.5m/s, D0 = 3.15mm, H0 = 12.6mm, ρ = 1585kg/m3, k = 0.1Pa.sm, m = 1, τ0 = 948Pa).
Download Isukwem et al. supplementary movie 2(File)
File 16.1 MB