1 Introduction
Polymer solutions attract much experimental and theoretical attention which is naturally explained by their fascinating non-Newtonian behaviour (Bird, Armstrong & Hassager Reference Bird, Armstrong and Hassager1977). Dissolving even small amounts of polymers in an ordinary fluid may dramatically change its hydrodynamic and rheological properties due to the appearance of elastic degrees of freedom. One of the most striking manifestations of non-Newtonian dynamics is a chaotic fluid motion which is observed at low Reynolds number
$Re$
exhibiting three main features (Groisman & Steinberg Reference Groisman and Steinberg2000, Reference Groisman and Steinberg2001, Reference Groisman and Steinberg2004; Gerashchenko, Chevallard & Steinberg Reference Gerashchenko, Chevallard and Steinberg2005; Burghelea, Segre & Steinberg Reference Burghelea, Segre and Steinberg2006, Reference Burghelea, Segre and Steinberg2007): pronounced growth in flow resistance, algebraic decay of velocity power spectra over a wide range of scales and orders of magnitude more efficient mixing than in an ordered flow. Since these properties are analogous to those of hydrodynamic turbulence, the chaotic state of the polymer solution has been named elastic turbulence.
Despite the close similarity between hydrodynamic turbulence and elastic turbulence, the physical mechanisms that underlie the two kinds of random motion are different. The former is known to occur at large
$Re$
due to instabilities arising from the nonlinear inertia term in the Navier–Stokes equation. In contrast, elastic turbulence takes place at vanishingly small
$Re$
where the effects of fluid inertia play no role. The main source of instability leading to elastic turbulence is the elastic stress created by the polymer stretching in the flow. The transition from laminar flow to elastic turbulence is controlled by the so-called Weissenberg number
$Wi$
, that is a ratio of the polymer linear relaxation time to the characteristic time of the flow dynamics. At large values of
$Wi$
, the majority of the dissolved polymers are above the coil–stretch transition that guarantees their strong back reaction on the fluid motion provided the polymer concentration is high enough (Balkovsky, Fouxon & Lebedev Reference Balkovsky, Fouxon and Lebedev2000; Chertkov Reference Chertkov2000; Fouxon & Lebedev Reference Fouxon and Lebedev2003; Gerashchenko et al.
Reference Gerashchenko, Chevallard and Steinberg2005).
The first experiments on elastic turbulence used three flow geometries with curved streamlines (Groisman & Steinberg Reference Groisman and Steinberg2000, Reference Groisman and Steinberg2001, Reference Groisman and Steinberg2004): von Kármán swirling flow between two disks, Couette–Taylor flow between cylinders and Dean flow in a curvilinear channel. Recently, purely elastic instabilities have been observed experimentally in a straight channel (Pan et al. Reference Pan, Morozov, Wagner and Arratia2013; Bodiguel et al. Reference Bodiguel, Beaumont, Machado, Martinie, Kellay and Colin2015) and elastic turbulence has been demonstrated numerically for viscoelastic Kolmogorov flow (Berti et al. Reference Berti, Bistagnino, Boffetta, Celani and Musacchio2008; Berti & Boffetta Reference Berti and Boffetta2010). Although the streamline curvature is not a crucial ingredient, it allows us to reduce the critical Weissenberg number for the instability onset.
In which aspects does elastic turbulence considerably differ from its inertial counterpart due to the aforementioned difference in the sources of flow instability? Although the phenomenon of elastic turbulence has been known of for two decades, this issue still remains poorly understood. The present paper demonstrates that at least one such aspect is the relation between the mean and the fluctuating components of the flow in the boundary layer region. The general rule for hydrodynamic turbulence states that the typical magnitude of random motion is of the order of the mean velocity variation at the considered spatial scale (Landau & Lifshitz Reference Landau and Lifshitz1987). In the context of wall-bounded turbulence, this means that fluctuations in the viscous boundary sublayer are of the order of the mean flow velocity. As is shown below, this rule is completely wrong in the case of wall-bounded elastic turbulence.
Polymer solutions can be characterized at two distinct levels: macroscopic and microscopic. The macroscopic approach treats the system as a continuous medium and, thus, focuses on the bulk parameters, which are averages of microscopic variables over scales much larger than the inter-polymer distance. In particular, the macroscopic description of the fluid velocity field is based on the generalized Navier–Stokes equation incorporating the elastic stresses (Balkovsky et al. Reference Balkovsky, Fouxon and Lebedev2000; Balkovsky, Fouxon & Lebedev Reference Balkovsky, Fouxon and Lebedev2001; Fouxon & Lebedev Reference Fouxon and Lebedev2003). At the microscopic level one deals with individual polymer molecules advected by the fluid flow. The microscopic approach has been extensively used to study the dynamics and statistics of polymer conformation (Afonso & Vincenzi Reference Afonso and Vincenzi2005; Celani, Musacchio & Vincenzi Reference Celani, Musacchio and Vincenzi2005a ; Celani, Puliafito & Turitsyn Reference Celani, Puliafito and Turitsyn2005b ; Turitsyn Reference Turitsyn2007; Vincenzi et al. Reference Vincenzi, Perlekar, Biferale and Toschi2015; Ahmad & Vincenzi Reference Ahmad and Vincenzi2016). In this paper we consistently implement both microscopic and macroscopic approaches to understand the properties of the boundary layer of elastic turbulence.
The emergence of a boundary layer where the fluid velocity field is approximated by a steady shear flow with relatively small fluctuations has been revealed in the experimental studies of elastic turbulence in different flow geometries (Burghelea et al.
Reference Burghelea, Segre and Steinberg2006, Reference Burghelea, Segre and Steinberg2007; Jun & Steinberg Reference Jun and Steinberg2011). From the theoretical point of view, the boundary layer is the region immediately adjacent to the wall within which the viscous stresses in a fluid are much larger than the elastic stresses associated with hydrodynamic stretching of polymers. Qualitatively, suppression of elastic stresses near the wall occurs because the gradient of the wall-normal component of the random velocity vanishes at the wall due to the no-slip boundary condition. The viscosity smooths the fluid velocity field which still remains a random function of time due to the fluctuations induced by the bulk flow where elastic stresses are relevant. A high-
$Re$
analogue of the boundary layer in the Newtonian fluids is the well-known viscous boundary sublayer defined by the condition that the viscosity dominates over the fluid inertia (Landau & Lifshitz Reference Landau and Lifshitz1987).
Let us expose the logic of our analysis. Since the backward reaction of the polymers on the flow diminishes at the bottom of the boundary layer, the polymers passing near the wall can be considered as passive. That dictates peculiarities of the velocity field structure and allows us to describe the spatially non-uniform statistics of the polymer conformation which is determined by interplay of the average shear flow and velocity fluctuations. Next, we use this information to find the elastic stresses responsible for the polymer back reaction on the flow. This back reaction is negligible in comparison with the viscous forces at small distances from the wall, but it eventually comes into the game at larger scales. From the condition that the elastic stresses become comparable with the viscous stresses at the border of the boundary layer, we extract the ratio of the mean flow to the magnitude of flow fluctuations. At the end of the paper the applicability range of our theory is discussed.
2 Velocity field in the boundary layer
When considering the boundary layer properties, we treat the wall as flat. For the channel flow, it is correct if the thickness of the boundary layer
$L$
is of the order of or smaller than the channel radius and its curvature. This condition also guarantees that correlation functions of the statistically stationary in time flow are homogeneous along the wall. Below, we consider the stationary case where the mean flow and the statistical properties of the flow fluctuations are time-independent. Note that our analysis is also applicable to the near-disk boundary layer in the von Kármán swirling flow, provided we are interested in a region far enough from the rotation axis (Burghelea et al.
Reference Burghelea, Segre and Steinberg2006, Reference Burghelea, Segre and Steinberg2007).
The Reynolds decomposition for the fluid velocity
$\boldsymbol{v}$
reads
where
$\boldsymbol{U}(\boldsymbol{r})$
and
$\boldsymbol{u}(\boldsymbol{r},t)$
are the mean and fluctuating parts of the flow velocity, respectively. Due to the dominant role of viscosity inside the boundary layer, the velocity field can be regarded as a smooth and regular function of the coordinates. In particular, the mean velocity is approximated in the leading order by a shear flow
where
$z\ll L$
and
$s$
is the shear rate. Here and below we choose a Cartesian reference system in such a way that the
$z$
-axis is perpendicular to the wall, and the
$x$
-axis is directed along the velocity of the mean flow: see figure 1.
Sketch of the polymer orientation geometry.

For the fluctuating velocity
$\boldsymbol{u}$
the following proportionality laws are valid:
provided
$z\ll L$
. The laws are consequences of the fluid velocity smoothness, the no-slip boundary condition at the wall and the incompressibility condition
$\unicode[STIX]{x1D735}\boldsymbol{\cdot }\boldsymbol{u}=0$
. Note also that
$\boldsymbol{u}$
varies along the wall at distances of the order of
$L$
.
3 Single polymer statistics
In the dilute limit, we neglect the mutual interactions of the polymer molecules. At
$z\ll L$
a single polymer can be treated as a passive object whose dynamics is governed by the equations
where
$\boldsymbol{r}$
is the coordinate of the mass centre of the polymer;
$\boldsymbol{R}$
is the polymer end-to-end elongation vector;
$\unicode[STIX]{x1D6FE}(R)$
is the extension-dependent spring constant of the polymer;
$\unicode[STIX]{x1D743}$
and
$\unicode[STIX]{x1D73B}$
are the Langevin forces having zero means and time-decorrelated second moments
$\langle \unicode[STIX]{x1D709}_{i}(t_{1})\unicode[STIX]{x1D709}_{j}(t_{2})\rangle =2\unicode[STIX]{x1D705}\unicode[STIX]{x1D6FF}_{ij}\unicode[STIX]{x1D6FF}(t_{1}-t_{2})$
and
$\langle \unicode[STIX]{x1D701}_{i}(t_{1})\unicode[STIX]{x1D701}_{j}(t_{2})\rangle =2\unicode[STIX]{x1D702}\unicode[STIX]{x1D6FF}_{ij}\unicode[STIX]{x1D6FF}(t_{1}-t_{2})$
with
$\unicode[STIX]{x1D705}$
and
$\unicode[STIX]{x1D702}$
representing the diffusivity for translational and elongational degrees of freedom of polymer motion, respectively.
The physical picture behind (3.1) and (3.2) is very simple: the polymer is advected along the Lagrangian trajectory being stretched by the velocity gradient and relaxing to its equilibrium shape due to elasticity. Note that the specific form of the function
$\unicode[STIX]{x1D6FE}(R)$
is not essential in the scope of this work. The only information on the elastic properties of the polymer required for our analysis is the spring constant in the Hookean (linear) limit
$\unicode[STIX]{x1D6FE}_{0}=\unicode[STIX]{x1D6FE}(0)$
and the maximum polymer extensibility
$R_{m}$
. We imply that
$R_{m}$
is small compared with the boundary layer thickness
$L$
.
In this section we use (3.1) and (3.2) with the velocity field
$\boldsymbol{v}$
given by (2.1)–(2.3) to describe the statistics of the polymer conformation inside the boundary layer in its dependence on the distance from the wall
$z$
. Our analysis is based on several assumptions, to be justified: (i) the Lagrangian correlation time
$\unicode[STIX]{x1D70F}_{c}$
of the flow in the near-wall region is much smaller than the characteristic time scale of the polymer stretching dynamics, (ii) the characteristic time scale of the stretching dynamics is much smaller than the characteristic time of polymer translational motion in the wall-normal direction, (iii) the thermal force
$\unicode[STIX]{x1D73B}$
can be neglected in comparison with the effect of velocity gradient stretching and (iv) the polymer is strongly elongated along the mean velocity most of the time. A justification of these assumptions for the boundary layer region of high-
$Wi$
elastic turbulence will be given below.
Due to time scale separation (i) and (ii), the statistics of the polymer conformation at a given spatial position is determined by the local intensity of the flow fluctuations which can be treated as shortly correlated in time. The conditions (iii) and (iv) in their turn mean that the main stochastic contribution to the polymer dynamics comes from the gradient of the
$z$
-component of the fluctuating velocity. Then, one can apply the results of the theoretical works (Chertkov et al.
Reference Chertkov, Kolokolov, Lebedev and Turitsyn2005; Turitsyn Reference Turitsyn2007), where exactly the same model assumptions have been exploited to examine the polymer dynamics in large mean shear with relatively weak flow fluctuations. For the sake of completeness we briefly reproduce the line of argument used in these works.
The orientation of the polymer end-to-end vector
$\boldsymbol{R}$
can be parametrized by the spherical angles
$\unicode[STIX]{x1D711}$
and
$\unicode[STIX]{x1D703}$
, as shown in figure 1. As was discussed in Chertkov et al. (Reference Chertkov, Kolokolov, Lebedev and Turitsyn2005), in terms of these variables, equation (3.2) (with the Langevin force omitted due to assumption (iii)) transforms into the following set of equations:
where
$\unicode[STIX]{x1D70D}_{\unicode[STIX]{x1D711}}$
,
$\unicode[STIX]{x1D70D}_{\unicode[STIX]{x1D703}}$
and
$\unicode[STIX]{x1D70D}_{\Vert }$
are random terms related to the fluctuating component of the fluid velocity. Although these terms are spatially inhomogeneous, assumptions (i) and (ii) guarantee that statistics of the polymer elongation vector adjusts adiabatically to the local flow properties and, therefore, the internal degrees of freedom can be analysed separately from the translation motion.
The angular dynamics described by (3.3) and (3.4) is decoupled from the dynamics of the polymer length. Moreover, since the polymer is strongly elongated along the shear direction (assumption (iv)), the orientation angles are small most of the time, and the intensity of the random term
$\unicode[STIX]{x1D70D}_{\unicode[STIX]{x1D711}}$
does not depend on
$\unicode[STIX]{x1D703}$
in the leading-order approximation. This means that the angle
$\unicode[STIX]{x1D711}$
becomes decoupled from both
$R$
and
$\unicode[STIX]{x1D703}$
. Treating
$\unicode[STIX]{x1D70D}_{\unicode[STIX]{x1D711}}$
in (3.3) as a delta-correlated Gaussian process, we can write the Fokker–Plank equation
in which
$P(t,\unicode[STIX]{x1D711})$
is the probability density function of
$\unicode[STIX]{x1D711}$
, and
$D$
denotes the angular diffusion coefficient. Equation (3.6) should be supplemented by the periodic boundary condition
$P(t,-\unicode[STIX]{x03C0}/2)=P(t,\unicode[STIX]{x03C0}/2)$
and the normalization condition
$\int _{0}^{\unicode[STIX]{x03C0}}P(t,\unicode[STIX]{x1D711})\,\text{d}\unicode[STIX]{x1D711}=1$
. In the strong shear limit,
$s\gg D$
, the stationary solution of (3.6) is localized at small angles and the steady-state average value of
$\unicode[STIX]{x1D711}$
is given by (see Turitsyn (Reference Turitsyn2007) for details of the derivation)
Here and in what follows, the angle brackets denote averaging over time or over realizations of the chaotic flow.
The near-wall shear rate can be estimated as
$s\sim U_{L}/L$
where
$U_{L}$
is the mean velocity of the flow at the border of the boundary layer. Next, the angular diffusion coefficient is determined by the gradient of the wall-normal component of velocity fluctuations:
$D=(1/2)\int _{-\infty }^{0}\langle \unicode[STIX]{x2202}_{x}u_{z}(\boldsymbol{r}(t),t)\unicode[STIX]{x2202}_{x}u_{z}(\boldsymbol{r}(0),0)\rangle \,\text{d}t$
. Using (2.3) one obtains
$\unicode[STIX]{x2202}_{x}u_{z}\sim u_{L}z^{2}/L^{3}$
where
$u_{L}$
measures the characteristic (wall-normal) fluctuating velocity at
$z=L$
, and, therefore,
$D\sim (\unicode[STIX]{x2202}_{x}u_{z})^{2}\unicode[STIX]{x1D70F}_{c}\sim u_{L}^{2}\unicode[STIX]{x1D70F}_{c}z^{4}/L^{6}$
. Inserting the estimates of
$s$
and
$D$
into (3.7), we find the conditional average of
$\unicode[STIX]{x1D711}$
at a given distance
$z$
from the wall:
Next let us consider the dynamics of the polymer elongation
$R$
. Since typical orientation angles are small,
$\unicode[STIX]{x1D711},\unicode[STIX]{x1D703}\ll 1$
, we can replace
$\sin \unicode[STIX]{x1D711}$
in (3.5) by
$\unicode[STIX]{x1D711}$
, while
$\cos \unicode[STIX]{x1D711}$
and
$\cos \unicode[STIX]{x1D703}$
can be replaced by unity. Further, we neglect the term
$\unicode[STIX]{x1D70D}_{\Vert }$
in comparison with
$s\unicode[STIX]{x1D711}$
because the diffusion coefficient
$D_{\Vert }\sim (\unicode[STIX]{x2202}_{x}u_{x})^{2}\unicode[STIX]{x1D70F}_{c}\propto z^{2}$
associated with
$\unicode[STIX]{x1D70D}_{\Vert }$
is much smaller than
$s\langle \unicode[STIX]{x1D711}\rangle \propto z^{4/3}$
at
$z\ll L$
. Then in the main approximation the dynamics of
$R$
is described by the following equation:
For the statistically stationary state we immediately find
To proceed we need to relate the correlation time
$\unicode[STIX]{x1D70F}_{c}$
to the spatial scale
$L$
and the characteristic velocities
$U_{L}$
and
$u_{L}$
. It is natural to expect that
$\unicode[STIX]{x1D70F}_{c}$
is of the same order as the inverse Lyapunov exponent
$\unicode[STIX]{x1D706}_{L}^{-1}$
at the edge of the boundary layer. Whereas the distance between two fluid parcels evolves accordingly to (3.9) with
$\unicode[STIX]{x1D6FE}=0$
, the Lyapunov exponent defined as the mean logarithmic rate of divergence of neighbouring Lagrangian trajectories is given by
$\unicode[STIX]{x1D706}_{L}=s\langle \unicode[STIX]{x1D711}\rangle$
, where
$\langle \unicode[STIX]{x1D711}\rangle$
is taken at
$z=L$
. Imposing the condition
$\unicode[STIX]{x1D70F}_{c}\sim \unicode[STIX]{x1D706}_{L}^{-1}$
, we find from (3.8) that
$\unicode[STIX]{x1D70F}_{c}\sim L/\sqrt{U_{L}u_{L}}$
. That yields the following estimates:
According to (3.11) and (3.12), the resulting effect of the hydrodynamic stretching cannot be decomposed into the additive contributions of the stationary shear part and the fluctuating part of the flow. Instead, the polymer dynamics in the boundary layer is determined by the combined effect of regular and chaotic components: fluctuations of the velocity gradient provide polymer stretching in the wall-normal direction required for the polymer to ‘feel’ the presence of the mean shear.
4 Numerical simulations
To check the scaling laws (3.11) and (3.12) we performed the simulations with synthetic random flow which mimics the boundary layer of elastic turbulence. In the case of strong shear the stretching dynamics becomes essentially two-dimensional, so we restrict ourselves to two-dimensional simulations. Namely, the components of the planar velocity field
$(v_{x},v_{z})$
in the periodic domain
$x\in [0,L]$
,
$z\in [-L,L]$
are chosen to be
$v_{x}=U_{x}+u_{x}$
,
$v_{z}=u_{z}$
, where
$$\begin{eqnarray}\displaystyle \left.\begin{array}{@{}c@{}}\displaystyle U_{x}=\frac{U_{L}}{\unicode[STIX]{x03C0}}\sin \frac{\unicode[STIX]{x03C0}z}{L},\\ \displaystyle u_{x}=\frac{L^{2}}{\unicode[STIX]{x03C0}^{2}}\left[a_{1}(t)\cos \frac{2\unicode[STIX]{x03C0}x}{L}+a_{2}(t)\sin \frac{2\unicode[STIX]{x03C0}x}{L}\right]\sin \frac{\unicode[STIX]{x03C0}z}{L},\\ \displaystyle u_{z}=\frac{2L^{2}}{\unicode[STIX]{x03C0}^{2}}\left[a_{1}(t)\sin \frac{2\unicode[STIX]{x03C0}x}{L}-a_{2}(t)\cos \frac{2\unicode[STIX]{x03C0}x}{L}\right]\left(1-\cos \frac{\unicode[STIX]{x03C0}z}{L}\right).\end{array}\right\} & & \displaystyle\end{eqnarray}$$
The independent random variables
$a_{1}$
and
$a_{2}$
are telegraph processes, that is
$a_{1}$
and
$a_{2}$
remain constant during time slot
$\unicode[STIX]{x1D70F}_{c}$
and their values are chosen from identical normal distributions with zero mean and variances
$\langle a_{1}^{2}\rangle =\langle a_{2}^{2}\rangle =u_{L}^{2}/L^{4}$
. Let us stress that the velocity field
$(v_{x},v_{z})$
is incompressible (
$\unicode[STIX]{x2202}_{x}v_{x}+\unicode[STIX]{x2202}_{z}v_{z}=0$
) and that it reproduces the proportionality laws
$U_{x},u_{x}\propto z$
,
$u_{z}\propto z^{2}$
when
$|z|\ll L$
. In our numerics we chose
$L=1$
,
$U_{L}=1$
,
$u_{L}=0.1$
and
$\unicode[STIX]{x1D70F}_{c}=L/\sqrt{U_{L}u_{L}}$
. The polymer dynamics was modelled via a two-dimensional version of (3.1) and (3.2) supplemented by the finitely extendible nonlinear elastic (FENE) model:
$\unicode[STIX]{x1D6FE}(R)=\unicode[STIX]{x1D6FE}_{0}(1-R^{2}/R_{m}^{2})^{-1}$
. The parameters
$\unicode[STIX]{x1D6FE}_{0}$
,
$R_{m}$
,
$\unicode[STIX]{x1D705}$
and
$\unicode[STIX]{x1D702}$
were adjusted in such a way that
$R_{m}/R_{0}=10^{2}$
,
$Wi=10^{4}$
and
$Pe=10^{6}$
, where
$R_{0}=\sqrt{3\unicode[STIX]{x1D702}/\unicode[STIX]{x1D6FE}_{0}}$
is the radius of gyration of a polymer and
$Pe=U_{L}L/\unicode[STIX]{x1D705}$
is the Péclet number.
(a,b) The average orientation angle
$\langle \unicode[STIX]{x1D711}\rangle$
and the spring constant
$\langle \unicode[STIX]{x1D6FE}\rangle$
dependences on the distance from the wall
$z$
. The solid lines represent the results of numerical simulations and the dashed lines are the theoretical power-law profiles: see (3.11) and (3.12). (c) The mean square of the polymer elongation
$\langle R_{x}^{2}\rangle$
along the shear direction as a function of distance from the wall
$z$
. The dashed line represents the asymptotic value corresponding to the limit of infinitely large shear. (d) The statistical moment
$C=\langle \unicode[STIX]{x1D6FE}R_{x}R_{z}\rangle$
(solid line) versus the distance from the wall
$z$
. This plot demonstrates that
$\langle \unicode[STIX]{x1D6FE}R_{x}R_{z}\rangle$
depends on
$z$
in the same manner as
$\langle \unicode[STIX]{x1D6FE}\rangle \langle \unicode[STIX]{x1D711}\rangle R_{m}^{2}$
(dashed line).

Figure 2 shows the steady-state expected values of the orientation angle
$\langle \unicode[STIX]{x1D711}\rangle$
and spring constant
$\langle \unicode[STIX]{x1D6FE}\rangle$
in their dependence on
$z$
. In agreement with theoretical prediction,
$\langle \unicode[STIX]{x1D711}\rangle$
and
$\langle \unicode[STIX]{x1D6FE}\rangle$
exhibit power-law behaviour with exponent
$4/3$
starting from some small distance from the wall and continuing for a scale of the order of
$L$
. The mean square of the polymer elongation along the wall is approximately constant in this region,
$\langle R_{x}^{2}\rangle \approx 0.62R_{m}^{2}$
: see figure 2(c). This is because
$\langle R_{x}^{2}\rangle$
is close to its limiting value, corresponding to the limit of infinitely large shear, which is numerically found to be approximately
$0.65R_{m}^{2}$
for the FENE model. Note that the limiting value differs from
$R_{m}^{2}$
due to the ongoing tumbling of a polymer molecule (Turitsyn Reference Turitsyn2007).
5 Relation between mean flow and fluctuations
Having described the single polymer statistics inside the boundary layer, we now pass to the macroscopic level of description. The hydrodynamics of the low-
$Re$
polymer solution is governed by the interplay of viscous forces and elastic forces, while fluid inertia can be neglected. Namely, if the flow is incompressible, i.e. the mass density of the neat fluid
$\unicode[STIX]{x1D70C}$
is a constant and
$\unicode[STIX]{x1D735}\boldsymbol{\cdot }\boldsymbol{v}=0$
, the momentum conservation law (with the nonlinear inertial term omitted) reads
Here
$p$
is the pressure,
$\unicode[STIX]{x1D6F1}_{ij}^{v}$
is the viscous stress tensors and
$\unicode[STIX]{x1D6F1}_{ij}^{e}$
is the tensor of elastic stresses created by the polymer stretching in the flow. Equation (5.1) is applicable at scales much larger than the inter-polymer distance where the polymer solution can be regarded as a continuous medium.
The elastic stress is the source of instability leading to the turbulent-like state of a polymer solution. In the bulk region of elastic turbulence, where polymers provide strong back reaction on the velocity field, the elastic stresses are of the order of or larger than the viscous stresses existing in the flow. However, in the peripheral region, the polymers are relatively weakly stretched since fluctuations of the wall-normal velocity gradient diminish towards the no-slip wall. This is why a boundary layer is formed, where viscosity overcomes elasticity.
For the statistically stationary flow, the only component of the viscous stress tensor remaining non-zero after averaging is
$\langle \unicode[STIX]{x1D6F1}_{xz}^{v}\rangle =\unicode[STIX]{x1D708}\unicode[STIX]{x2202}_{z}U_{x}$
, where
$\unicode[STIX]{x1D708}$
is Newtonian viscosity of the neat fluid. The corresponding component of the polymer-induced elastic stress is given by (Bird et al.
Reference Bird, Hassager, Armstrong and Curtiss1987)
where
$n$
is the concentration of the polymers in solution, and
$\unicode[STIX]{x1D6E4}$
is the kinetic coefficient, which determines the polymer relaxation. In the two-bead-one-spring model of the polymer molecule one has
$\unicode[STIX]{x1D6E4}\sim (\unicode[STIX]{x1D70C}\unicode[STIX]{x1D708}R_{0})^{-1}$
.
It is difficult to derive a closed-form expression for the statistical moment
$\langle \unicode[STIX]{x1D6FE}R_{x}R_{z}\rangle$
entering (5.2). However, for the boundary layer region one can safely write the estimate
$\langle \unicode[STIX]{x1D6FE}R_{x}R_{z}\rangle \sim \langle \unicode[STIX]{x1D6FE}\rangle \langle \unicode[STIX]{x1D711}\rangle R_{m}^{2}$
, which is confirmed by numerical simulations: see figure 2(d). Then, using (3.11), (3.12) and (5.2), we obtain
$\langle \unicode[STIX]{x1D6F1}_{xz}^{e}\rangle \sim n\unicode[STIX]{x1D708}R_{0}R_{m}^{2}u_{L}z^{8/3}/L^{11/3}$
at
$z\ll L$
. By the definition of the boundary layer, the elastic stress must become of the order of the viscous stress
$\langle \unicode[STIX]{x1D6F1}_{xz}^{v}\rangle \sim \unicode[STIX]{x1D708}U_{L}/L$
at
$z=L$
. This condition produces the following relation:
which is the central result of this work. Equation (5.3) shows that in contrast to high-
$Re$
turbulence, where the fluctuating velocity is always of the order of the mean flow in the viscous sublayer, wall-bounded elastic turbulence possesses a non-trivial relation between the mean and the fluctuating velocity components.
It should be stressed that the line of argument presented here cannot give us the value of the numerical factor in (5.3) which may significantly differ from unity in hydrodynamic problems of this sort. This remark must be taken into account when making numerical predictions based on the above result. At the same time, equation (5.3) uncovers the parametric relation between the quantities
$U_{L}$
,
$u_{L}$
,
$n$
,
$R_{m}$
and
$R_{0}$
which can be tested experimentally.
Another important concern that may restrict the applicability of our results is the difference between the properties of the real polymer molecule and that of the idealized dumbbell-like model adopted here. In particular, one may expect that in high-
$Wi$
flow, the kinetic coefficient
$\unicode[STIX]{x1D6E4}$
in (5.2) should be estimated as
$(\unicode[STIX]{x1D70C}\unicode[STIX]{x1D708}R_{m})^{-1}$
since for the strongly stretched polymer molecule the force of hydrodynamic friction affecting the dynamics of the elongation vector
$\boldsymbol{R}$
is determined by the scale
$R_{m}$
. This leads to the relation
$U_{L}/u_{L}\sim nR_{m}^{3}$
which, in contrast to (5.3), does not contain the equilibrium size
$R_{0}$
of the polymers.
We are ready to justify the set of assumptions (i)–(iv) underlying the analytical procedure presented above. First of all, we note that the characteristic time of the extensional dynamics is
$\langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
. Then, as follows from (3.12) and from the estimate
$\unicode[STIX]{x1D70F}_{c}\sim L/\sqrt{U_{L}u_{L}}$
, assumption (i), which can be written as
$\unicode[STIX]{x1D70F}_{c}\ll \langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
, is self-consistent for any
$z\ll L$
. There is a simple explanation as to why the time scales
$\unicode[STIX]{x1D70F}_{c}$
and
$\langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
are well separated inside the boundary layer. In the bulk region of elastic turbulence, where fluid motion is strongly influenced by polymer back reaction, the velocity correlation time
$\unicode[STIX]{x1D70F}_{c}$
must be of the same order as the relaxation time of the elastic stresses
$\langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
. Since the flow fluctuations in the boundary layer are induced by bulk turbulence, then the correlation time
$\unicode[STIX]{x1D70F}_{c}$
near the wall is also determined by the value of
$\langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
in the bulk. At the same time, hydrodynamic stretching of polymers in close vicinity to the wall is much weaker than their stretching in the bulk. We thus conclude that
$\unicode[STIX]{x1D70F}_{c}\ll \langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
in the boundary layer.
Next, let us examine the range of validity for the ‘adiabatic’ assumption (ii). Since the centre of mass of the polymer is passively advected by the flow, the probability density function
$n(z,t)$
of its
$z$
-coordinate obeys the standard advection–diffusion equation
$\unicode[STIX]{x2202}_{t}n=\unicode[STIX]{x2202}_{z}[D_{zz}(z)\unicode[STIX]{x2202}_{z}n]$
, where
$D_{zz}(z)=\unicode[STIX]{x1D707}z^{4}+\unicode[STIX]{x1D705}$
and
$\unicode[STIX]{x1D707}\sim u_{L}^{2}\unicode[STIX]{x1D70F}_{c}/L^{4}$
(Lebedev & Turitsyn Reference Lebedev and Turitsyn2004; Chernykh & Lebedev Reference Chernykh and Lebedev2011). The time required for a polymer at distance
$z$
from the wall to ‘feel’ the inhomogeneity of the fluctuations is estimated as
$\tilde{\unicode[STIX]{x1D70F}}(z)\sim z^{2}/D_{zz}(z)$
. This time must be much larger than the characteristic time of the stretching dynamics, i.e.
$\tilde{\unicode[STIX]{x1D70F}}(z)\gg \langle \unicode[STIX]{x1D6FE}\rangle ^{-1}$
. Given equation (3.12), this leads to the following condition:
As for the assumption (iii), the Langevin force
$\unicode[STIX]{x1D73B}$
produces the correction of the order of
$\unicode[STIX]{x1D702}/R_{m}^{2}$
to the angular diffusion coefficient
$D$
. The correction is relatively small if
where
$Wi=U_{L}\unicode[STIX]{x1D6FE}_{0}^{-1}/L$
is the Weissenberg number.
Finally, the assumption (iv) is equivalent to the inequalities
$\langle \unicode[STIX]{x1D711}\rangle \ll 1$
and
$\langle \unicode[STIX]{x1D6FE}\rangle \gg \unicode[STIX]{x1D6FE}_{0}$
. The former is satisfied for any
$z\ll L$
provided
$u_{L}\lesssim U_{L}$
, while the latter can be rewritten as
Taking into account (5.3), we conclude from (5.4)–(5.6) that the spatial scales
$r_{\unicode[STIX]{x1D705}}$
,
$r_{\unicode[STIX]{x1D702}}$
and
$r_{\unicode[STIX]{x1D6FE}_{0}}$
are small in comparison with the width of the boundary layer
$L$
in the limit when both the Weissenberg number
$Wi$
and the Péclet number
$Pe$
are large. That ensures the self-consistency of our asymptotic theory.
6 Discussion
We have combined a microscopic description of the polymer statistics with a macroscopic description of the stresses in a polymer solution to investigate the boundary layer properties of elastic turbulence. This allowed us to derive the parametric relation between the magnitude of the velocity fluctuations and the mean flow in the high Weissenberg number limit: see (5.3). This relation follows from the condition that the elastic stresses become comparable with the viscous stresses at the border of the boundary layer.
Unfortunately, the experimental studies performed to date are beyond the applicability of the asymptotic analysis presented here. Say, for the typical experimental parameters
$nR_{0}^{3}\approx 0.1$
and
$R_{m}/R_{0}\approx 100$
one observes
$U_{L}/u_{L}\approx 10$
and, therefore, we need to take
$Wi\gtrsim 10^{4}$
to ensure the spatial scale separation
$r_{\unicode[STIX]{x1D705}},r_{\unicode[STIX]{x1D702}},r_{\unicode[STIX]{x1D6FE}_{0}}\ll z\ll L$
. At the same time, the maximum Weissenberg number in existing experiments is of the order of
$10^{3}$
. Moreover, the large values of Weissenberg number, which we need to justify our analytical scheme, are difficult to achieve in practice because of the too fast mechanical degradation of polymer molecules at high shear rates. Thus, the current lack of relevant experimental data does not allow us to test the scaling laws (3.11) and (3.12) and the parametric dependence predicted by (5.3).
Could the asymptotic results give us qualitatively correct insight into the boundary layer properties outside the relevant asymptotic regime? Although the systematic study of this issue requires much further experimental work, the already known data suggest that (5.3) properly captures the observed peculiarities of elastic turbulence. First of all, it is noteworthy that the boundary layer width
$L$
drops from (5.3). This is in accord with the experimental observation by Jun & Steinberg (Reference Jun and Steinberg2011) that
$L$
is determined by the system size rather than being merely a function of the properties of a polymer solution. Secondly, velocity fluctuations are always weaker than the average flow in elastic turbulence experiments. In qualitative agreement with this fact, our theory predicts that at
$nR_{0}^{3}\approx 0.1$
and
$R_{m}/R_{0}\approx 100$
the mean velocity is large compared to the fluctuating velocity provided the unknown numerical prefactor on the right-hand side of (5.3) is not too small. Finally, and most importantly, equation (5.3) tells us that the fluctuations become less pronounced with an increase of the polymer concentration. This result may seem to be somewhat paradoxical: although the phenomenon of elastic turbulence becomes possible due to polymer additives, the turbulence intensity decreases as the concentration of the additives grows. However, the recent experimental study of elastic turbulence in a von Kármán swirling flow supports this prediction: see figure 10 in Jun & Steinberg (Reference Jun and Steinberg2017). We hope that these remarks will stimulate the detailed experimental and numerical verification of the theoretical results presented here.
Acknowledgement
We are grateful to V. Steinberg for valuable discussions. This work was supported by the Russian Scientific Foundation, grant no. 14-22-00259.


