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Liquid toroidal drop in compressional Stokes flow

Published online by Cambridge University Press:  23 November 2015

Michael Zabarankin*
Affiliation:
Department of Mathematical Sciences, Stevens Institute of Technology, Castle Point on Hudson, Hoboken, NJ 07030, USA
Olga M. Lavrenteva
Affiliation:
The Wolfson Department of Chemical Engineering, Technion-Israel Institute of Technology, Haifa 32000, Israel
Avinoam Nir
Affiliation:
The Wolfson Department of Chemical Engineering, Technion-Israel Institute of Technology, Haifa 32000, Israel
*
†Email address for correspondence: mzabaran@stevens.edu

Abstract

The deformation of an immiscible toroidal drop embedded in axisymmetric compressional Stokes flow is analysed via the boundary integral formulation in the case of equal viscosity. Numerical simulations are performed for the drop having initially the shape of a torus with circular cross-section. The quasi-stationary dynamic simulations reveal that, when the viscous forces, proportional to the intensity of the flow, are relatively weak compared with the surface tension (the ratio of these forces is characterized by the capillary number, $Ca$ ), three different scenarios of drop evolution are possible: indefinite expansion of the liquid torus, contraction to the centre and a stationary toroidal shape. When the intensity of the flow is low, the stationary shapes are shown to be close to circular tori. Once the outer flow strengthens, the cross-section of the stationary torus assumes first an elliptic and then an egg-like shape. For the capillary number greater than a critical value, $Ca_{cr}$ , toroidal stationary shapes were not found. Remarkably, $Ca_{cr}$ is close to the critical capillary number found previously for a simply connected drop flattened in compressional flow. Thus, a new example of non-uniqueness of stationary drop shape in viscous flow is obtained. Approximate stationary solutions in the form of tori with circular and elliptic cross-sections are obtained by minimizing the normal velocity over the drop interface. They are shown to be in good agreement with the stationary shapes from quasi-dynamic simulations for the corresponding intervals of the capillary number.

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Papers
Copyright
© 2015 Cambridge University Press 
Figure 0

Figure 1.Toroidal drop: $R$ and $a$ are the major and minor radii respectively. The cross-section of the torus is shown in the $rz$ half-plane in the cylindrical coordinate system $(r,{\it\varphi},z)$, where the $z$-axis is the axis of revolution.

Figure 1

Figure 2.Time evolution of parameters of deforming initially circular tori. (a–c) Major radius of the toroid. (d–f) Taylor deformation factor of the torus. (g–i) Deformation factor of the torus cross-section. In (a,d,g), $Ca=0.18$; dashed curves, $R=0.82$; solid curves, $R=0.81$; dot-dashed curves, $R=0.8107$. In (b,e,h), $Ca=0.1$; dashed curves, $R=1.2$; solid curves, $R=1$; dot-dashed curves, $R=1.09327$. In (c,f,i), $Ca=0.04$; dashed curves, $R=1.9$; solid curves, $R=1.86$; dot-dashed curves, $R=1.86969$.

Figure 2

Figure 3.Dynamic deformation of the cross-section of an initially circular toroidal drop: $Ca=0.16$; (a) $R=0.86$; (b) $R=0.85236$; (c) $R=0.852$.

Figure 3

Table 1.Critical major radius, $R_{cr}$, for various values of $Ca$.

Figure 4

Figure 4.Dynamic deformation of the cross-section of an initially circular toroidal drop: (a) $Ca=0.04$, $R=1.2$; (b) $Ca=0.1$, $R=1$; (c) $Ca=0.15$, $R=0.86$.

Figure 5

Figure 5.Deformation parameters of the torus in two cases: (a–c) $Ca=0.2$ and (d–f) $Ca=0.5$. In (a–c), the dotted, dot-dashed, dashed and solid curves correspond to $R=1$, 0.786, 0.780438260324 and 0.780438260323 respectively, whereas in (d–f), they correspond to $R=0.8$, 0.7, 0.6846 and 0.6845 respectively.

Figure 6

Figure 6.Dynamic deformation of the initially circular cross-section of a toroidal drop for $Ca=0.2$ in three cases: (a) $R=0.780438260323$, (b) $R=0.780438260324$, (c) $R=0.8$.

Figure 7

Figure 7.Dynamic deformation of the initially circular cross-section of a toroidal drop for $Ca=0.5$ in two cases: (a) $R=0.8$ and (b) $R=0.7$.

Figure 8

Table 2.Outcomes of deformation of circular tori with initial radius $R$.

Figure 9

Figure 8.(a) Dynamic deformation of the initially circular cross-section of a toroidal drop for $Ca=0$ in four cases: $R/a=1.009$, $1.4$, $1.9$ and $2.1$. (b) The inner radius $R_{in}=\min _{\boldsymbol{x}\in S}r$ (dotted and solid curves) and $R_{in,\,z=0}=\min _{\boldsymbol{x}\in S,\,z=0}r$ (see inset) of the droplet normalized by its initial value for initial aspect ratios of 1.4 (dotted and dashed curves) and 1.9 (solid and dot-dashed curves). The physical parameters are taken from Pairam & Fernández-Nieves (2009): ${\it\mu}=30\,000~\text{cp}$, ${\it\sigma}=4~\text{mN}~\text{m}^{-1}$.

Figure 10

Table 3.Parameters in (3.7) approximating the cross-sections of the pointwise stationary-state shapes with $K=1$ (fitted ellipses), the corresponding fit error (3.9) and $\Vert u_{n}\Vert _{S}$ defined by (3.8).

Figure 11

Table 4.Parameters in (3.7) approximating the cross-sections of the pointwise stationary-state shapes with $K=5$, the corresponding fit error (3.9) and $\Vert u_{n}\Vert _{S}$ defined by (3.8).

Figure 12

Figure 9.Cross-sections of the pointwise stationary-state shapes (solid curves) and their approximations by (3.7) with $K=1$ (fitted ellipses, dashed curves) and with $K=5$ (circles) in two cases: (a) $Ca=0.16$ and (b) $Ca=0.19$. Triangles mark the cross-sections of corresponding ‘stationary’ elliptic tori found from the inverse problem (4.18) with $w=r^{-1}$.

Figure 13

Figure 10.Streamlines about the stationary-state toroidal shape for $Ca=0.05$.

Figure 14

Figure 11.Streamlines about the stationary-state toroidal shape for $Ca=0.15$.

Figure 15

Figure 12.Streamlines about the stationary-state toroidal shape for $Ca=0.19$.

Figure 16

Figure 13.Circular tori: $(Ca,R(Ca))$ with $R(Ca)$ minimizing $\mathscr{E}_{1}(u_{n}^{+},r^{-1};S)$ (solid curve), $(Ca(R),R)$ with $Ca(R)$ determined by (4.9) (dot-dashed curve) and $(Ca,R_{cr}(Ca))$ with the critical radius $R_{cr}(Ca)$ tabulated in table 1 (dashed curve). The dashed and dot-dashed curves are visually indistinguishable.

Figure 17

Figure 14.The curves $(Ca(R),R)$ and $(Ca(R),a(R))$ for ‘stationary’ circular tori determined by (4.9) (triangles), for the ‘stationary’ elliptic tori found from the inverse problem (4.18) with $w=r^{-1}$ (dashed curves), and for (3.7) approximating the cross-sections of the pointwise stationary-state shapes with $K=1$ (fitted ellipses, red circles) and with $K=5$ (solid curves).

Figure 18

Table 5.Parameters of the ‘stationary’ elliptic torus (4.16) found from the inverse problem (4.18) with $w=r^{-1}$ and the corresponding mean absolute value $\Vert u_{n}\Vert _{S}$ defined by (3.8).

Figure 19

Figure 15.The Taylor deformation factor $D=(R_{max}-z_{max})/(R_{max}+z_{max})$ for a simply connected stationary shape (diamonds) and for a toroidal stationary shape (circles) as a function of $Ca$. In the ‘circles’ curve, the short dashed curve at $Ca\sim 0$ does not follow from computations, but reflects the assumption that $R_{max}\rightarrow \infty$ as $Ca\rightarrow 0$.

Figure 20

Figure 16.Cross-sections of the stable simply connected stationary-state shape (dashed curves) and of the unstable toroidal stationary-state shape (solid curves) for (a) $Ca=0.1$, (b) $Ca=0.15$ and (c) $Ca=0.19$.