Cultural weed management through intercropping helps in weed suppression, resulting in improved crop productivity. Cereal–legume intercropping is one of the major eco-friendly approaches to suppress weeds and improve crop performance and soil fertility. Therefore, a two-year field experiment was carried out at the campus of Ramakrishna Mission Vivekananda Educational and Research Institute, Ranchi, Jharkhand during the monsoon season of 2023 and 2024 in a randomized block design with three replications using eight cropping systems. Results revealed that sole black gram ensured highest weed control efficiency (55.9%), followed by intercropping system of finger millet and black gram (1:2) (49.5%). Finger millet + black gram (1:2) and sole black gram recorded higher growth attributes and yields of finger millet and black gram, respectively. However, finger millet + black gram (1:2) also recorded high growth and yield attributes of black gram. System productivity was maximum in sole black gram (4730 kg/ha), followed by intercropping system of finger millet and black gram (1:2) (3900 kg/ha), along with protein content (23.4%) and consequently, the production economics (net return: Rupees 56830/ha; benefit: cost of 1.90). It also resulted in the highest residual soil fertility. Additionally, the combined land equivalent ratio (1.44) was higher in the 1:2 intercropping system of finger millet and black gram, indicating a 44% yield advantage. Thus, in Eastern Plateau and Hill Zone of India, an intercropping system of finger millet and black gram (1:2) is recommended for cultivation in monsoon to achieve high weed suppression, crop productivity, and economic profitability.